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Although many multi-component polymer systems are well characterised, the surface properties of polymers mixed with low surface energy additives have received little attention. In addition, the new branches of scanning probe microscopy that enable high resolution mapping and modification of surface charge distributions have been infrequently applied to polymer surfaces. The surface segregation of a fluorochemical additive directly from a polypropylene host matrix has been investigated by AFM and other surface analysis techniques. The level of surface enrichment was found to be governed by the temperature and duration of annealing. Further investigation revealed that the speed and extent of surface enrichment of the additive increases with polymer molecular weight. The effect of additive structure on surface segregation has also reported. A method of depositing charge onto polypropylene substrates from a high potential scanning AFM tip was developed. The relation between AFM tip- voltage and the level of charge deposited on the substrate suggested that a localised corona discharge was generated. AFM scanning parameters were found to effect the deposition of charge. The charging behavior of fluorochemical doped polypropylene surfaces was investigated on macroscopic scales using a scanning electrometer probe, and on microscopic scales using EFM. Fluorochemical domains at the surface have been found to preferentially accumulate both positive and negative charge. Surface charge distributions were found to become more uniform during annealing. Sub-micron particle capture by charged surfaces was investigated using EFM. In addition, spatially confined amine beads were deposited onto a patch of localised charge and subsequently functionalised to produce a metallic gold coating.

Thesis (Ph. D.)--University of Texas at Austin, 1999. / Vita. Includes bibliographical references (leaves 115-131). Available also in a digital version from Dissertation Abstracts.

No description available.

Thesis (PhD)-- University of South Australia, 1997

Thesis (Ph. D.)--University of Washington, 2007. / Vita. Includes bibliographical references (p. 74-80).

Thesis (Ph.D.)--University of Nebraska-Lincoln, 2009. / Title from title screen (site viewed October 13, 2009). PDF text: xiii, 127, 11 p. : ill. (some col.) ; 6 Mb. UMI publication number: AAT 3352608. Includes bibliographical references. Also available in microfilm and microfiche formats.

Thesis (M.S.)--Worcester Polytechnic Institute. / Keywords: purple membrane; photomechanics; photoinduced conformation change; photocycle; photoactive; photoinduced; bimetallic bending; bacteriorhodopsin; atomic force microscope; tip-sample interface; molecular conformation; PLDS; photoreactive; AFM. Includes bibliographical references (p. E-1-E-4).

Thesis (Ph. D.)--Ohio State University, 2005. / Title from first page of PDF file. Includes bibliographical references (p. 182-189).

No description available.