Thesis (M. Phil.)--University of Hong Kong, 2010. / Includes bibliographical references (leaves 139-[147]). Also available in print.

Thesis (Ph. D.)--University of Wisconsin--Madison, 1975. / Vita. Typescript. eContent provider-neutral record in process. Description based on print version record. Includes bibliographical references.

Thesis (M. Phil.)--University of Hong Kong, 2010. / Includes bibliographical references (leaves 139-[147]). Also available online.

Thesis (Ph. D.)--University of Texas at Austin, 2008. / Vita. Includes bibliographical references.

A modified thin lens spectrometer has been used with improved geometry. The focussing properties of the instrument have been investigated for various geometries. Using this instrument the conversion electron spectra of Sn¹¹³ and Sb¹²⁵ have been taken. The intensity of the 256 kev conversion line in Sn¹¹³ spectrum showed that this transition is predominantly M1 in character and therefore the spin and parity of 648-kev level in In¹¹³ should be 1/2¯ or 3/2¯. The low energy part of the conversion spectrum of Sb¹²⁵showed the presence of the K conversion lines of 76 kev and 143 kev transitions, not observed before. The presence of these conversion lines confirmed the existence of a weak beta group feeding a level at 540 kev in the excited state of Te¹²⁵. The energy levels of Cs¹³³ have been studied through the decay of Ba¹³³. Scintillation spectra (using NaI(T1 ) crystal) together with photoelectron, conversion and e-gamma coincidence spectra have been taken. An analysis of the results indicate that the ground state and 81, 161, 383 and 437 kev levels in Cs¹³³ have spins and parities of 7/2⁺, 5/2⁺,5/2⁺,3/2⁺, 1/2⁺ respectively. The multipolarities of the connecting transitions are 383 kev (E2 ), 356 (E2 ) 302 kev (M1 with E2 admixture)} 276 kev (E2 ), 161 kev (probably M1 ) Electron capture from Ba¹³³ is limited almost entirely to the 437 and 383 kev levels in Cs¹³³, The decay energy available for capture to the 437 level is approximately 50 kev. / Science, Faculty of / Physics and Astronomy, Department of / Graduate

In this study, two methods of analysing activity concentrations of natural radionuclides (U, Th and K) in soil are critically compared. These are the Window Analysis (WA) and Full Spectrum Analysis (FSA). In the usual WA method, the activity concentrations are determined from the net counts of the windows set around individual &gamma / -ray peaks associated with the decay of U, Th and K. In the FSA method, the full energy spectrum is considered and the measured spectrum is described as the sum of the three standard spectra (associated with U, Th and K, respectively), each multiplied by an unknown concentration. The concentrations are determined from the FSA and correspond to the activity concentrations of U, Th and K in the soil. The standard spectra derived from separate calibration measurements using the HPGe detector, represents the response of the HPGe to a Marinelli sample beaker containing an activity concentration of 1 Bq/kg.

This thesis reports an investigation into methods of determining the long term deposition field for atmospheric aerosols in areas of complex topography using the soil inventories of atmospherically derived radionuclides. Measurements of the radionuclides ²¹⁰Pb, ¹³⁷Cs, ¹³⁴Cs and ⁷Be in vegetation and soil have been made at five mountain locations in northern Britain. A description of the field sampling procedure, sample processing and y-ray analysis is given. Loss-on-ignition experiments to determine the organic fraction of sampled soils were also conducted on selected samples. The presence of frequent low level cloud shrouding mountain tops in the uplands of northern and western Britain leads to enhanced precipitation and also deposition of the major acidic ions, eg SO₃²⁻ and N0₃, due to the washout of the low level cloud by falling rain ('seeder-feeder scavenging') and also the direct deposition of cloud droplets ('occult deposition'). It is important to quantify the inputs of acidic deposition in these acid sensitive regions and direct measurements present many logistical problems. The radionuclide ²¹⁰Pb is attached to the same sub-micron aerosol size range in the atmosphere as the major acidic ions and following deposition attaches very strongly to organic matter in soils. In this study the soil inventory of atmospherically derived ²¹⁰Pb is used as a tracer of the deposition of acidic ions. As the half-life of ²¹⁰Pb is 22.3 years the soil inventory of ²¹⁰Pb(atmos), at a site undisturbed for - 100 years, represents deposition integrated over several decades. Initial sampling took place at the Merrick, an isolated mountain close to the coast in southwest Scotland, to test and develop the technique. Measurements showed the ²¹⁰Pb(atmos) inventory to increase with altitude at a greater rate than precipitation. Sampling at Great Dun Fell in Cumbria enabled the measured radionuclide inventories to be compared with detailed measurements of the variation of the wet deposition pattern with altitude, and also with a model of sulphate deposition. Close correspondence was found between the ²¹⁰Pb deposition profile and the deposition pattern, with altitude, for the major acidic ions. The three mountains Ben Cruachan, Beinn Dorain and Ben Lawers lie along an 80 km transect running roughly west to east from the western coast into the central Highlands. Sampling at these three mountains has yielded information on the change in the wet deposition field with distance inland. The measurements suggest that deposition of ²¹⁰Pb decreases, with distance from the western coast, at a greater rate than does precipitation. The soil inventory of ²¹⁰Pb(atmos) increases with altitude at a greater rate than rainfall at 4 of the 5 mountains. The results show that, around summits, on average, the concentration of ²¹⁰Pb in low level cloud is a factor of - 2 greater than in the frontal ('seeder') rain falling from higher altitude. This finding is in good agreement with detailed wet deposition measurements. The ²¹⁰Pb measurements are important in themselves as they help define the global and UK ²¹⁰Pb budget. From measurements made at 65 individual sites the mean ²¹⁰Pb(atmos) inventory is 0.44 ± 0.03 Bq cm⁻², with the mean of the average annual rainfall being 2,060 ± 70 mm yr⁻¹. These figures correspond to a mean concentration of ²¹⁰Pb in rainfall of 66 mBql⁻¹. The ¹³⁷Cs inventory has been separated into the fraction originating from nuclear weapons testing, ¹³⁷Cs(bomb), and the fraction due to the Chernobyl accident, ¹³⁷Cs(Chern). The measured ¹³⁷Cs(bomb) inventory ranges from a mean of 3,300 Bq m⁻² at Ben Lawers to 5,200 Bq m⁻² at Beinn Dorain. The ¹³⁷Cs(Chern) inventory is highly variable between locations ranging from a mean of 440 Bq m⁻² at Great Dun Fell to 14,900 Bqm⁻² at Ben Lawers reflecting the patchy nature of deposition, due largely to convective storms, during the passage of the radioactive plume. The radionuclide ¹³⁷Cs is shown to be relatively mobile in the organic soils which characterise the study areas. The cosmogenic radionuclide ⁷Be was measured in samples collected from the Merrick on 26th Oct 1988. The mean inventory was 0.039 Bq cm⁻², being associated with vegetation and the top few cm of the soil profile.

Rapid emergency response decisions from a radiation release are necessary in order to prevent the general public from being exposed to a potential radiation hazard. A one meter exposure rate measurement is all that is necessary to establish relocation and food control areas when the ground is contaminated at the Protective Action Guide minimum response levels. With the results of these calculations, a known one meter exposure rate is all that is necessary to establish relocation and food control areas for a release from the WNP-2 commercial nuclear power plant or a release from a waste tank at the Hanford site. The calculated one meter exposure rate for WNP-2 is 1.32 ��R/hr at twenty-four hours. The calculated one meter exposure rate for the Hanford tanks is 14.97 ��R/hr. / Graduation date: 1995

There are a variety of uses for reference neutron fields including detector response and dosimeter studies. The Georgia Institute of Technology has a 252Cf spontaneous fission source and an AmBe (α, n) source available for use in its research programs. In addition, it has iron, lead, beryllium, tantalum, heavy water, and polyethylene spheres to modify the neutron energy distributions from these neutron sources. This research characterized the neutron leakage spectra from the source inside spherical shells using a Bonner sphere spectrometer. All the neutron fields measured were also computed with a Monte Carlo code to determine the neutron fluence rate and ambient dose equivalent rate. The comparison of experimental data and calculations are used to provide further insight into the neutron spectra as modified by the spheres. The characterization of these modified sources will provide data to assist in using the resulting neutron fields in other research activities. To measure each neutron field combination, one of the two sources was placed in the center of an attenuating sphere. The neutron field was first measured at a variety of source-to-detector distances with a Bonner Sphere System. The spectrometer measurements, specifically the count rates of the different Bonner spheres, as a function of distance from the source is fitted to obtain corrections for room-scatter and air-scatter of neutrons using the Eisenhauer, Schwartz, and Johnson method. Using these corrections, the count rates free of room return is obtained at 1 m from the source and unfolded using the BUMS software to obtain the reported fluence and dose equivalent rates. These results are compared to those generated by the Monte Carlo Neutral Particle (MCNP) code. Models were made in MCNP for each of the source and moderating sphere combinations. The neutron fluence and dose rates were tallied during the MCNP simulation. The unfolded experimental data and the MCNP calculations showed good agreement for most of source-attenuating sphere combinations, thereby reinforcing the experimental results.

Thesis (Ph. D.)--Joint Program in Oceanography (Massachusetts Institute of Technology, Dept. of Earth, Atmospheric, and Planetary Sciences; and the Woods Hole Oceanographic Institution), 2002. / Includes bibliographical references.