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Theory and large-scale numerical simulations of nucleation and growth

In this work we have re-examined the classical problem of nucleation and growth. We present a new model that combines steady-state homogeneous nucleation theory with the classical Lifshitz-Slyozov mechanism of growth. This model considers the substantial correlations between droplets and naturally incorporates the crossover from the early-stage, nucleation dominated regime to the scaling, late-stage, coarsening regime within a single framework, without ad-hoc assumptions. This is achieved by the development of a set of self-consistent interface equations which describe the decay of metastable states. The model is implemented numerically and some interesting dynamical behaviour is observed, including the reproduction of the expected late-time scaling and power-law growth laws for the key mean-field variables.

Identiferoai:union.ndltd.org:LACETR/oai:collectionscanada.gc.ca:QMM.27417
Date January 1996
CreatorsStinson O'Gorman, Dean.
ContributorsGrant, Martin (advisor)
PublisherMcGill University
Source SetsLibrary and Archives Canada ETDs Repository / Centre d'archives des thèses électroniques de Bibliothèque et Archives Canada
LanguageEnglish
Detected LanguageEnglish
TypeElectronic Thesis or Dissertation
Formatapplication/pdf
CoverageMaster of Science (Department of Physics.)
RightsAll items in eScholarship@McGill are protected by copyright with all rights reserved unless otherwise indicated.
Relationalephsysno: 001553749, proquestno: MQ29792, Theses scanned by UMI/ProQuest.

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