Mining of uranium ore and its extraction using the milling process generates solid and liquid waste, commonly termed uranium mine tailings. Uranium mine tailings is radioactive, as it consists of residual uranium, thorium, and radium, which amounts to 85% of the original ore’s radioactivity. Due to the extensively long half-lives of uranium (4.5x109 years), thorium (75,400 years), and radium (1,620 years) and their harmful radioactive, it is imperative to isolate uranium mine tailings from the environment for a longer period. Containment of uranium mine tailings in dam-like structures, called uranium mine tailings dam (UMTD), is the most followed disposal and storage method. Like a conventional water retention dam, UMTDs are also susceptible to failure, mainly due to adverse weather conditions. Once the UMTD fails, a fraction of the radioactive tailings infiltrates and migrate through the vadose zone contaminating the groundwater sources underlying it. Radionuclide behavior and migration in the subsurface are affected by several environmental factors. To minimize the uncertainty and improve current radionuclide fate and transport models, it is vital to study these factors and any interdependence existing between them. This study aims to understand these environmental factors by i) enlisting the factors affecting subsurface radionuclide migration through scoping review of articles and reports, and ii) analyzing the interdependence existing between the factors using the complex network theory (CNT) approach and identifying the dominant factors among them. Factors such as chemical and biological characteristics of soil stratigraphy, groundwater, and radioactive tailings plume, meteorological, and hydrogeological are found to influence radionuclide behavior and transport mechanisms in the vadose zone. CNT approach described soil microorganisms, fraction of organic carbon, infiltration rate of the soil, transmissivity, clay fraction in the soil, particulates in groundwater, and infiltrating rainwater as dominant factors in the NoF based on their centrality measures and sensitivity analysis of the network of factors (NoF). Any uncertainty associated with these factors will affect and propagate through the model. Hence, sufficient resources should be directed in the future to characterize these factors and minimize their uncertainty, which will lead to developing reliable fate and transport models for radionuclides. / Thesis / Master of Applied Science (MASc) / Waste products from uranium mining and milling operations are called uranium mine tailings, which are radioactive. Generally, uranium mine tailings are disposed of and isolated in dam-like structures referred to as uranium mine tailings dams (UMTD). One of the most common causes of UMTD failure is extreme weather conditions. When a UMTD fails, a part of tailings, consisting of radionuclides uranium, thorium, and radium, infiltrate into the subsurface through the vadose zone. Radionuclide behavior and transport in the subsurface is influenced by several environmental factors. The objective of the present study is to understand the factors affecting radionuclide migration by i) conducting a scoping review on radionuclide migration in the subsurface to describe the factors studied in the literature, and ii) understanding and analyzing any relation among the factors and deriving the most dominant factors based on their relation. This study can be used further to develop accurate and reliable radionuclide fate and transport models with minimal uncertainty.
| Identifer | oai:union.ndltd.org:mcmaster.ca/oai:macsphere.mcmaster.ca:11375/27576 |
| Date | January 2022 |
| Creators | Narayanan, Brinda Lakshmi |
| Contributors | Dickson-Anderson, Sarah, Guo, Peijun, Civil Engineering |
| Source Sets | McMaster University |
| Language | English |
| Detected Language | English |
| Type | Thesis |
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