Accelerated carbonation is a new CO2 storage method under development as a solution for climate change caused by anthropogenic activities. In accelerated carbonation an alkaline source such as minerals or industrial residues react with carbon dioxide in a presence of slightly acidic solution to produce stable solid carbonates. There are varieties of accelerated carbonation routes which differ in process condition.</p><p>The aim of this study was to evaluate and compare the potential of a slurry route process and a wet route process for the carbonation of basic oxygen furnace (BOF) slag using the CO2 emitted by a conventional natural gas power plant.</p><p>For this purpose a life cycle assessment (LCA) study was performed based on principles and guidelines provided by ISO 14040:2006 and routines and data provided by the SimaPro v8 software package. The material and energy requirements for each of the steps involved in the carbonation process, i.e. pre-treatment of raw material, CO2 compression, transportation, carbonation step, after-treatment and landfill, were calculated and included in the LCA study.</p><p>The slurry and wet route resulted in net CO2 reduction of 87.4% and 72.3% respectively. However, a positive contribution to other environmental issues was observed with the wet route leading to higher impact mainly due to high heating requirement. An exception was contribution of slurry route to abiotic resource depletion, which was higher for the slurry route due to high water requirement. A general conclusion was that the electricity consumption is the main cause of environmental issues. Sensitivity analyses showed that the environmental impacts are dependent on the transportation distance and electricity source, while no dependence was observed with respect to construction of the carbonation plant.
| Identifer | oai:union.ndltd.org:UPSALLA1/oai:DiVA.org:kth-180552 |
| Date | January 2015 |
| Creators | Ghasemi, Sara |
| Publisher | KTH, Skolan för kemivetenskap (CHE) |
| Source Sets | DiVA Archive at Upsalla University |
| Language | English |
| Detected Language | English |
| Type | Student thesis, info:eu-repo/semantics/bachelorThesis, text |
| Format | application/pdf |
| Rights | info:eu-repo/semantics/openAccess |
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