This dissertation begins with a study of some of the linear and nonlinear optical properties of composite materials consisting of CdSₓSe₁₋ₓ microcrystallites embedded in a host glass matrix. These studies investigate changes in absorption, refractive index and nonlinear response time under a variety of experimental conditions. The data demonstrates that this class of materials exhibit: a strong saturation of absorption due to band filling; a large n₂ which also saturates; response times which range from <100ps to many nanoseconds; and a permanent darkening and change of n₂ induced by extended exposure to high energy pulses. These measurements were used to identify the optimum sample of the semiconductor doped glasses to demonstrate an efficient degenerate four-wave mixing process within a planar waveguide. High quality single mode waveguides were fabricated from the semiconductor doped glass by K⁺-ion exchange. Four wave mixing was performed in the waveguide that produced a peak reflectivity of ≅.003, which is 8 orders of magnitude larger than that achieved previously in a similar experiment where CS₂ was used as the nonlinear medium.
| Identifer | oai:union.ndltd.org:arizona.edu/oai:arizona.openrepository.com:10150/184367 |
| Date | January 1988 |
| Creators | Gabel, Allan Harley. |
| Contributors | Stegeman, George |
| Publisher | The University of Arizona. |
| Source Sets | University of Arizona |
| Language | English |
| Detected Language | English |
| Type | text, Dissertation-Reproduction (electronic) |
| Rights | Copyright © is held by the author. Digital access to this material is made possible by the University Libraries, University of Arizona. Further transmission, reproduction or presentation (such as public display or performance) of protected items is prohibited except with permission of the author. |
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