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Slow Dynamics in Quantum Matter: The Role of Dimensionality, Disorder and Dissipation

A central goal in the study of modern condensed matter physics is the characterization of the dynamical properties of quantum systems. Many decades of effort towards this goal, studying a diverse range of (near-equilibrium) quantum matter, from Fermi liquids, to quantum two-level systems, to interacting spin models, and more, has revealed a remarkable pervasiveness of the simple dynamical description of these complex systems in terms of quasi-particles that carry spin, charge, and heat, and that are generally able to equilibrate systems.

This thesis is an examination of some exceptions to this rule. Specifically, we study a number of instances of quantum matter where equilibration phenomena happens at rather long time scales, or does not occur at all. Particular emphasis is laid on the role of dimensionality, disorder, and dissipation in engendering such novel dynamical behavior.

First, we consider non-equilibrium dynamics in one-dimensional quasi-condensates. Low dimensionality inhibits scattering in these systems, and low-energy excitations are long-lived phase fluctuations that exhibit an enriched conformal symmetry. Utilizing this symmetry, we generalize sudden quenches typically used to study non-equilibrium dynamics to quenches along general relativistic and conformal trajectories. Gases never truly equilibrate after such a quench; instead, they evolve into a `prethermal' state with thermal-looking correlations and a chiral asymmetry.

We then study the problem of the dynamical transition driven by disorder, from an ergodic to a non-ergodic phase, in one-dimensional quantum spin chains. In particular, in XXZ chains with on-site disorder, we find a unique intermediate phase straddling the boundary of the dynamical phase transition, wherein rare-region effects lead to long-time tails in equilibration and vanishing DC conduction before the onset of non-ergodicity. We propose generalizations of such `Griffiths' behavior to arbitrary dimensions. We also study the dynamics of random-bond Heisenberg chains by developing a strong-disorder renormalization group protocol for these systems. We discuss how magnetic noise from such disordered systems contains signatures of their anomalous dynamical properties.

Next, we re-examine the phenomenological theory of two-level systems in amorphous materials in the light of new experimental evidence that these states have large electric/magnetic dipole moments. We propose and justify an interpretation of the model as one of tunneling electrons slowed down by a large phonon drag and discuss the dynamical consequences of such polaronic effects.

Finally, we discuss how magnetic noise measurements can be used to non-invasively access the anomalous properties of systems such as those discussed above. In particular, we examine how scattering properties of isolated magnetic impurities and non-local transport in a variety of two-dimensional materials can be probed experimentally using NV centers as noise magnetometers. / Physics

Identiferoai:union.ndltd.org:harvard.edu/oai:dash.harvard.edu:1/33493505
Date25 July 2017
CreatorsAgarwal, Kartiek
ContributorsDemler, Eugene
PublisherHarvard University
Source SetsHarvard University
LanguageEnglish
Detected LanguageEnglish
TypeThesis or Dissertation, text
Formatapplication/pdf
Rightsopen

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