Liquid water formation and flooding in PEM fuel cell gas distribution channels can significantly degrade fuel cell performance by causing substantial pressure drop in the channels and by inhibiting the transport of reactants to the reaction sites at the catalyst layer. A better understanding of the mechanisms of discrete water droplet transport by air flow in such small channels may be developed through the application of quantitative flow visualization techniques. This improved knowledge could contribute to improved gas channel design and higher fuel cell efficiencies. An experimental investigation was undertaken to gain better understanding of the relationships between air velocity in the channel, secondary rotational flows inside a droplet, droplet deformation, and threshold shear, drag, and pressure forces required for droplet removal. Micro-digital-particle-image-velocimetry (micro-DPIV) techniques were used to provide quantitative visualizations of the flow inside the liquid phase for the case of air flow around a droplet adhered to the wall of a 1 mm x 3 mm rectangular gas channel model. The sidewall against which the droplet was adhered was composed of PTFE treated carbon paper to simulate the porous GDL surface of a fuel cell gas channel. Visualization of droplet shape, internal flow patterns and Velocity measurements at the central cross-sectional plane of symmetry in the droplet were obtained for different air flow rates. A variety of rotational secondary flow patterns within the droplet were observed. The nature of these flows depended primarily on the air flow rate. The peak velocities of these secondary flow fields were observed to be around two orders of magnitude below the calculated channel-averaged driving air velocities. The resulting flow fields show in particular that the velocity at the air-droplet interface is finite. The experimental data collected from this study may be used for validation of numerical simulations of such droplet flows. Further study of such flow scenarios using the techniques developed in this experiment, including the general optical distortion correction algorithm developed as part of this work, may provide insight into an improved force balance model for a droplet exposed to an air flow in a gas channel.
| Identifer | oai:union.ndltd.org:LACETR/oai:collectionscanada.gc.ca:BVIV.1828/310 |
| Date | 17 January 2008 |
| Creators | Minor, Grant |
| Contributors | Djilali, Ned, Oshkai, Peter |
| Source Sets | Library and Archives Canada ETDs Repository / Centre d'archives des thèses électroniques de Bibliothèque et Archives Canada |
| Language | English, English |
| Detected Language | English |
| Type | Thesis |
| Rights | Available to the World Wide Web |
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