In this thesis the orientation of macro-sized fibres in turbulent flows is studied, as well as the effect of nano-sized fibrils on hydrodynamic stability. The focus lies on enabling processes for new materials where cellulose is the main constituent. When fibres (or any elongated particles) are added to a fluid, the complexity of the flow-problem increases. The fluid flow will influence the rotation of the fibres, and therefore also effect the overall fibre orientation. Exactly how the fibres rotate depends to a large extent on the mean velocity gradient in the flow. In addition, when fibres are added to a suspending fluid, the total stress in the suspension will increase, resulting in an increased apparent viscosity. The increase in stress is related to the direction of deformation in relation to the orientation of the particle, i.e. whether the deformation happens along the long or short axis of the fibre. The increase in stress, which in most cases is not constant neither in time nor space, will in turn influence the flow. This thesis starts off with the orientation and spatial distribution of fibres in the turbulent flow down an inclined plate. By varying fibre and flow parameters it is discovered that the main parameter controlling the orientation distribution is the aspect ratio of the fibres, with only minor influences from the other parameters. Moreover, the fibres are found to agglomerate into streamwise streaks. A new method to quantify this agglomeration is developed, taking care of the problems that arise due to the low concentration in the experiments. It is found that streakiness, i.e. the tendency to agglomerate in streaks, varies with Reynolds number. Going from fibre orientation to flow dynamics of fibre suspensions, the influence of cellulose nanofibrils (CNF) on laminar/turbulent transition is investigated in three different setups, namely plane channel flow, curved-rotating channel flow, and the flow in a flow focusing device. This last flow case is selected since it is can be used for assembly of CNF based materials. In the plane channel flow, the addition of CNF delays the transition more than predicted from measured viscosities while in the curved-rotating channel the opposite effect is discovered. This is qualitatively confirmed by linear stability analyses. Moreover, a transient growth analysis in the plane channel reveals an increase in streamwise wavenumber with increasing concentration of CNF. In the flow focusing device, i.e. at the intersection of three inlets and one outlet, the transition is found to mainly depend on the Reynolds number of the side flow. Recirculation zones forming downstream of two sharp corners are hypothesised to be the cause of the transition. With that in mind, the two corners are given a larger radius in an attempt to stabilise the flow. However, if anything, the flow seems to become unstable at a smaller Reynolds number, indicating that the separation bubble is not the sole cause of the transition. The choice of fluid in the core flow is found to have no effect on the stability, neither when using fluids with different viscosities nor when a non-Newtonian CNF dispersion was used. Thus, Newtonian model fluids can be used when studying the flow dynamics in this type of device. As a proof of concept, a flow focusing device is used to produce a continuous film from CNF. The fibrils are believed to be aligned due to the extensional flow created in the setup, resulting in a transparent film, with an estimated thickness of 1 um. / <p>QC 20141003</p>
| Identifer | oai:union.ndltd.org:UPSALLA1/oai:DiVA.org:kth-153018 |
| Date | January 2014 |
| Creators | Kvick, Mathias |
| Publisher | KTH, Strömningsfysik, Stockholm |
| Source Sets | DiVA Archive at Upsalla University |
| Language | English |
| Detected Language | English |
| Type | Doctoral thesis, comprehensive summary, info:eu-repo/semantics/doctoralThesis, text |
| Format | application/pdf |
| Rights | info:eu-repo/semantics/openAccess |
| Relation | TRITA-MEK, 0348-467X ; 2014.22 |
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