<p>Polygeneration plants are proposed as an attractive solution to today’s challenging economic and political climate, whereby fossil fuels (e.g.: coal, natural gas) can be co-processed to obtain multiple products, such as electricity, gasoline and diesel. To this end, this thesis investigates the feasibility of the operation and control of a novel cooling system which incorporates steam methane reformer (SMR) tubes into a gasifier radiant syngas cooler (RSC). This approach capitalizes on available exergy by producing valuable H<sub>2</sub>-rich synthesis gas (syngas) for liquid fuel production. As the device is still in the conceptual phase, a detailed multi-scale, two-dimensional, heterogeneous model has been developed in prior work to accurately predict the unit’s operation.</p> <p>A base case design was developed for both counter-current and co-current flow configurations, wherein a PI control structure designed to achieve performance objectives. Key trade-offs were found between the configurations: the counter-current design was more robust and effective in rejecting moderate and severe disturbances, while providing greater cooling duty and natural gas throughput, but at the expense of dangerously high tube wall temperatures, which can greatly reduce tube lifetime. The co-current design operates in a safer temperature range and satisfactorily rejects moderate disturbances, but requires feedforward control to handle extreme gasifier upsets.</p> <p>An offset-free linear model predictive controller (MPC) was developed for the co-current system to address process interactions. The MPC model was identified from ‘data’ derived from the rigorous plant model, with a Luenberger observer used to estimate and eliminate the plant-model mismatch. MPC offered superior set point tracking relative to discrete-PI control, especially in cases where discrete-PI destabilized the system. Using the co-current design, the flexibility of the device to adjust natural gas throughput based on variations in downstream syngas demand was demonstrated.</p> / Master of Applied Science (MASc)
| Identifer | oai:union.ndltd.org:mcmaster.ca/oai:macsphere.mcmaster.ca:11375/15346 |
| Date | 22 April 2015 |
| Creators | Seepersad, Dominik |
| Contributors | II, Thomas Adams, Christopher L.E. Swartz, Prashant Mhaskar, Chemical Engineering |
| Source Sets | McMaster University |
| Detected Language | English |
| Type | thesis |
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