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  • About
  • The Global ETD Search service is a free service for researchers to find electronic theses and dissertations. This service is provided by the Networked Digital Library of Theses and Dissertations.
    Our metadata is collected from universities around the world. If you manage a university/consortium/country archive and want to be added, details can be found on the NDLTD website.
11

Neutron and X-ray scattering study of magnetic manganites

Johnstone, Graeme Eoin January 2012 (has links)
This thesis presents three investigations of the magnetic and electronic proper- ties of manganese oxide materials. The investigations are performed using a variety of neutron scattering and x-ray scattering techniques. The electronic ground-state of Pr(Sr<sub>0.1</sub> Ca<sub>0.9</sub>)<sub>2</sub> Mn<sub>2</sub>O<sub>7</sub> an antiferromagnet with CE-type ordering, is determined using neutron spectroscopy, as opposed to the more usual approach of using diffraction. The Zener polaron model of the elec- tronic ground state of the CE-type magnetic phase is shown to be unsuitable for this material. The ground-state is shown to agree well with the electronic ground state proposed by Goodenough in the 1950’s, but without significant Mn<sup>3&plus;</sup>/Mn<sup>4&plus;</sup> disproportionation. The distribution of the magnetisation density within the unit cell of the CE-type antiferromagnet La<sub>0.5</sub>Sr<sub>1.5</sub>MnO<sub>4</sub> is determined from a polarised neutron diffraction experiment by analysing the results with the maximum entropy method. The majority of the magnetisation density is found to be located at the Mn site. The investigation shows tentative evidence of a small magnetic moment on the in-plane O site. However, a larger moment is observed at both the La/Sr site and the out-of-plane O site. The magnetic structure of the magnetoelectric multiferroic DyMn<sub>2</sub>O<sub>5</sub> is inves- tigated using resonant magnetic x-ray scattering. The magnetic structure is shown to be similar to other members of the RMn<sub>2</sub>O<sub>5</sub> series of multiferroics, but with the key difference that the magnetic moments are closely aligned parallel with the crystallographic b-axis, in contrast to the usual observation of the moments being close to parallel with the a-axis. This study also shows evidence that the electrical polarisation has a significant contribution from the valence electrons of the O ions, agreeing with previous work.
12

Gamma-ray bursts in the local universe

Chapman, Robert January 2009 (has links)
With energy outputs &gt;~10^51 erg in 0.1-1000 seconds, Gamma-ray Bursts (GRBs) are the most powerful events yet observed in the Universe. As such they are potential probes of the very early Universe, back to the era of re-ionisation and the first stars, but at the same time they have been observed to span a wide range in luminosity and redshift from the relatively local Universe (z~0.0085) out to z~6.29. GRBs divide into two classes based primarily on their duration as measured by T90 (the time taken to observe 90% of the total burst fluence). Long bursts (L-GRBs) have T90&gt;~2 seconds, and shorts (S-GRBs) T90&lt;~2 seconds. Though much has been learned regarding long duration GRBs since the first afterglow discovery in 1997 (including their likely association with massive core collapse supernovae), much remains unknown regarding short duration GRBs. In this work, after a brief historical introduction and review, we present analyses of the angular cross-correlation on the sky of short GRBs from the BATSE catalogue with galaxies in the local Universe sampled from the PSCz Redshift Survey and the Third Reference Catalogue of Bright Galaxies (RC3). In particular we show that 20%+/-8% (1 sigma) of all BATSE short duration bursts (localised to 10 degrees or better) show correlation with galaxy samples (morphological T-type&lt;=4) within ~112 Mpc. Our statistics thus provide evidence that a substantial fraction of BATSE short GRBs show a tendency to be associated with large scale structure on the sky traced by a variety of galaxy types. Short GRBs are believed to be produced in the final merger of compact object (neutron star-neutron star or neutron star-black hole) binaries, though other possible progenitors are known to exist. The short initial spike of a giant flare from a Soft Gamma Repeater (SGR) such as the December 27th 2004 event from SGR1806-20 would have been detectable by BATSE as a short GRB if it occurred in a galaxy within ~30-50 Mpc (assuming a distance to SGR1806-20 of 15 kpc). Using the observed luminosities and rates of Galactic SGR giant flares, as well as theoretical predictions for the rate of binary mergers, we investigate the ability of plausible Luminosity Functions (LF), singly and in combination, to reproduce our observed correlations and a cosmological S-GRB population. We find the correlations are best explained by a separate population of lower luminosity S-GRBs, with properties consistent with them being due to giant flares from extra-galactic SGRs. Overall predicted number counts are a good fit to the observed BATSE number counts, and furthermore, the wider redshift distribution is consistent with the early Swift S-GRB redshift distribution. The three closest GRBs which have been observed to date were all long duration bursts, and we have therefore also searched for cross-correlation signals between the BATSE long GRBs and local galaxies. The three nearby bursts shared several similar properties such as being under-luminous, spectrally soft and of low variability. We have therefore also investigated a subset of L-GRBs with light curve properties similar to these known nearby bursts. The whole sample is found to exhibit a correlation level consistent with zero (1 sigma upper limit=10%, equivalent to 144 bursts) out to a radius of ~155 Mpc, but a spectrally soft, low observed fluence and low variability subset shows a correlation level of 28%+/-16% (=50+/-28 bursts) within 155 Mpc. These results are consistent with low-luminosity, low-variability bursts being a separate sub-class of L-GRBs which may be much more prevalent in the local Universe than their high-luminosity, cosmologically distant counterparts. To investigate this further, we once again examined plausible luminosity functions for single and dual high and low luminosity populations, based on observed intrinsic rates from the literature. The local population was once again found only to be produced to a sufficient level (while maintaining consistency with the observed overall number counts) by a separate low luminosity population with intrinsic rates several hundred times greater than their cosmological counterparts. Constraining the models via the Swift overall redshift distribution instead of threshold-adjusted BATSE number counts showed that the dual LF models were able to produce excellent fits to the entire redshift distribution while adequately reproducing a local population. Finally, suggestions are made as to the direction future work may follow in order to build on these initial investigations, as well as to how observations with future missions and detectors such as Fermi (formerly GLAST), Advanced LIGO and LOFAR may shed further light on nearby GRBs.

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