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  • About
  • The Global ETD Search service is a free service for researchers to find electronic theses and dissertations. This service is provided by the Networked Digital Library of Theses and Dissertations.
    Our metadata is collected from universities around the world. If you manage a university/consortium/country archive and want to be added, details can be found on the NDLTD website.
221

Synthetic studies in heterocyclic and aromatic systems : part I - thiazolines, part II - cyclopropabenzenes

Mansuri, Muzammil Mansoor January 1978 (has links)
No description available.
222

Mechanistic investigations on the pictet-gams isoquinoline synthesis

Oppong - Boachie, Francis Kwabena January 1976 (has links)
No description available.
223

The reactions of aliphatic amines with polyhaloalkanes in the presence of copper salts

Malik, Zubair Ahmad January 1969 (has links)
No description available.
224

Electron-transfer oxidations of aromatic compounds with copper(II) halides

Mancilla, J. M. January 1974 (has links)
No description available.
225

Electrochemical and photochemical reactions of aromatic amides, pyrazoles and 1,2,3-triazole

Mannus, David January 1978 (has links)
No description available.
226

Some new aspects of pyrrole chemistry

Marriott, Michael Thomas Patrick January 1979 (has links)
No description available.
227

Advances in alicyclic chemistry

McKervey, Michael Anthony January 1972 (has links)
No description available.
228

Disproportionation of olefins catalysed by group VI transition metal oxides

O'Neill, Philip Paschal Joseph January 1972 (has links)
No description available.
229

Stereoselective routes to the total synthesis of the polyene macrolide viridenomycin

Thirsk, Carl Edward January 2003 (has links)
Viridenomycin 11 is a polyene macrolide possessing a wealth of biological activity. As part of an ongoing program examining the stereoselective synthesis of polyene natural products, a strategy was explored to effect the total synthesis of viridenomycin 11.As a consequence of the adopted retrosynthetic strategy, the project was naturally divided into three main areas: efforts directed towards the southern (E, E, E, Z)-tetraene 210, towards the northern (E, Z, Z)-triene 209, and towards the core cyclopentenone 211.Both polyenic sections 209 and 210 were tackled with a view to utilizing palladium-coupling methodology developed in the group, whereby vinylboronates of type 122 undergo Heck coupling with alkenyl halides, affording polyenyl boronates that may then be converted into polyenyl iodides via stereoselective iodo-deboronation. The geometry of the new double bond is determined by the order of reagent addition during the iodo-deboronation. Vinylboronates such as 122 may thus be regarded as a vinyl dianion equivalent, permitting ready access to either alkene geometry, and allowing a polyene chain to be built up via an iterative process. Efforts towards 209 gave rise to a surprising reaction, in which it was discovered that iodoacrylates 214 are problematic Heck coupling partners due to a propensity to undergo novel Michael addition-elimination reactions with most amine bases, instead affording amino acrylates in excellent yields. Efforts towards 210 called for the development of new and robust methods for the elaboration of the amino acid phenylglycine, providing gready improved procedures for its conversion to the corresponding N-protected β-amino alcohol, N-protected β-amino-O-sulfonylates, N -protected β -amino iodides and N-protected β-amino nitriles, all valuable synthetic intermediates in their own right. An advanced synthon en route to 210 was prepared by Heck coupling of (Z)-iodide 214 with vinylboronate 272, representing a considerable in-road into the synthesis of this fragment. Markedly different chemistry was required to synthesize 211. Its retrosynthetic strategy called for a stereoselective aldol reaction, and as a consequence of this work it was found that novel oxazaborolidinone mediated Mukaiyama aldol additions between diene 4-(ferr-butoxy)-2,4-bis[(trimethylsilyl)oxy]-l,3-butadienyl methyl ether 335 and a wide range of electrophiles gave aldol products in isolated yields of up to 90%.
230

Photo-oxidation in the tetrapyrrole series

Chaney, B. D. January 1977 (has links)
No description available.

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