Thesis (M.S.) -- University of Tennessee, Knoxville, 2005. / Title from title page screen (viewed on June 28, 2005). Thesis advisor: Wayne T. Davis. Document formatted into pages (ix, 82 p. : ill. (some col.), col. maps). Vita. Includes bibliographical references (p. 58-67).

Thesis (M. Phil.)--University of Hong Kong, 2000. / Includes bibliographical references (leaves 110-120).

Thesis (M. Sc.)--University of Hong Kong, 2000. / Includes bibliographical references.

Thesis (Ph. D.)--University of Texas at Austin, 2008. / Vita. Includes bibliographical references.

Thesis (M.S.)--University of Wisconsin-Madison, 1990. / eContent provider-neutral record in process. Description based on print version record. Includes bibliographical references (p. 105-110).

This thesis deals with the issues associated with the legal regulation of air quality protection. The main objective is to describe, analyse and evaluate the condition of the current legal regulation which is mainly represented by the Act no. 201/2012 Coll., on the protection of air. The introductory part of the thesis focuses on the historical development of the legal regulation, its primary milestones, as well as legal regulation according to International and European Law and its impact on the internal national legislation. Furthermore, the thesis also focuses on the currently valid legal regulation and its components and clarifies its basic terminology. The largest portion of the thesis focuses on the legal regulation of the individual instruments regulated primarily by the Act no. 201/2012 Coll., on the protection of air, with the primary focus being the stationary sources of pollution. These instruments are sorted into traditional groups, each respectively representing conceptual, administrative-legal and economic instruments. The chapter on conceptual instruments primarily focuses on the two fundamental instrumental programs, that is a) - The National Emission Reduction Program of the Czech Republic, and b) - programs aimed at improving air quality and their importance in legal regulation....

Black carbon (BC) is the light-absorbing component of soot, a combustion-generated aerosol that warms the climate by absorbing solar radiation. Its impacts on climate depend on its microphysical properties, which are modified by atmospheric processes including condensation, coagulation and wet removal. State of the art climate models consider soot in a concentric core/shell configuration, with a BC core coated by nonrefractory material such as organics or sulphate. Within this model, thicker coatings enhance visible light absorption, but also wet removal efficiency, and these have opposing effects on the total amount of light absorbed over BC’s lifetime. How well the core/shell model can calculate Mass Absorption Coefficient (MAC, the ratio of absorption to BC mass) is uncertain, as real soot forms more complex (often fractal) shapes, and detailed optical models using these morphologies predict the core/shell model may under- or over-estimate MAC depending on the precise properties of the particles. Few reliable measurements of variations in ambient MAC are available, as most older measurement techniques suffer from systematic uncertainties. In this work, a Single Particle Soot Photometer (SP2) and PhotoAcoustic Soot Spectrometer (PASS) were used to measure BC mass concentration and absorption, and these instruments do not suffer from such uncertainties. The SP2 was also used to report core size and coating thickness distributions that are required to test state of the art climate models. Firstly, a method was developed to minimise bias in the measured coating thicknesses related to the limited detection range of the SP2. The sensitivity of this technique to the assumed density and refractive index of the BC core was also explored, and the most appropriate parameters to use with ambient measurements were determined. Core and shell distributions were measured in Pasadena, California under a range of different photochemical ages. These were then used to calculate MAC, which was compared to that measured using the SP2 and PASS. The measured and modelled MAC agreed within 10% at 532 nm, though this was dependent on the assumed refractive index of the BC core. Overall MAC increased by 15 –25% in around one third of a day of photochemical ageing. This is quite modest compared to some climate models, but not compared to the previous best estimate, which predicted MAC may increase by a factor of ~1.5 over BC’s lifetime. Core and coating distributions were also measured in Canadian boreal biomass burning plumes. A case study was presented comparing the properties of BC in three plumes, one of which had passed through a precipitating cloud. It was demonstrated that larger and more coated BC-containing particles were removed more efficiently, in agreement with previous thermodynamic theory. By calculating MAC using the measured core/shell distributions and comparing to measured scattering, it was demonstrated that the MAC and single-scattering albedo in the plumes were likely not significantly affected by the wet removal, as greater differences were observed between the two plumes not affected by precipitation.