[Portion of abstract]: Sediment dynamics are influenced by transformed landscape connectivity in catchments worldwide. The upper Thina catchment, an important high rainfall resource in the northern Eastern Cape, South Africa, is an example of where ongoing subsistence farming on communal land has led to overgrazing and trampling that has initiated large erosive features (e.g. gullies) and river incision. The formation of gullies led to increased hillslope-channel connectivity and the resultant river incision decreased the channel-valley fill connectivity. These two changes in connectivity led to increased sediment export from the catchment that has various down-stream ecological and socio-economic impacts. This study investigates how the change in hillslope-channel and channel-valley fill connectivity has altered the sediment dynamics in the Vuvu catchment, a headwater tributary of the Thina River. A combination of methods were used to assess the changes in hillslope-channel and channel-valley fill connectivity. High resolution aerial images were used to map source features, such as fields, gullies, sheet erosion, landslides, roads and livestock tracks. Topographic and geological characteristics of the source features were extracted using a Geographic Information System. Furthermore, hillslope-channel pathways, such as the natural drainage network, continuous gullies, discontinuous gullies, roads and livestock tracks were mapped and analysed in terms of topographic and geological characteristics. Historic aerial images were assessed to calculate the date the larger gullies began forming. Recent aerial photos and cross sectional surveys of the valley fill were combined to map the various sediment sinks. Particle size and organic content were analysed for flood bench cores and terrace samples. The chronology of the flood benches was determined using unsupported Pb-210 and Cs-137 dating, and determined for the terraces using Optically Stimulated Luminescence dating. Quantitative and qualitative sediment tracing approaches, using mineral magnetic properties, were used to trace the origin of suspended sediment (collected during flood events), sediment stored in the flood benches and sediment stored in the terraces. Hydrological monitoring was used to assess the potential to store sediment on flood benches along the valley fill through flood bench inundation frequency. Hydrological and hydraulic modelling extended the measured inundation frequencies to a 73 year period and other cross sections along the valley fill. Furthermore, a future scenario of an increased vegetation cover and reduced hillslope-channel connectivity was assessed in terms of channel-valley fill inundation frequency.