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This study provides a detailed experimental evaluation of wheel-rail interaction for railroad vehicles, using the Virginia Tech Federal Railroad Administration (VT-FRA) Roller Rig. Various contact dynamics that emulate field application of railroad wheels on tracks are set up on the rig under precise, highly-controlled and repeatable conditions. For each setup, the longitudinal and lateral traction (creep) forces are measured for different percent creepages, wheel loads, and angles of attack. The tests are performed using quarter-scaled wheels with different profiles, one cylindrical and the other AAR-1B with a 1:20 taper. Beyond the contact forces, the wheel wear and the deposition of worn materials are measured and estimated as a function of time using a micron-precision laser optics measurement device. The change in traction versus amount of worn material at the contact surface is analyzed and related to wheel-rail friction. It is determined that the accumulation of the worn material at the contact surface, which appears as a fine gray powder, acts as a friction modifier that increases friction. The friction (traction) increase occurs asymptotically. Initially, it increases rapidly with time (and worn material accumulation) and eventually reaches a plateau that defines the maximum friction (traction) at a stable rate. It is estimated that the maximum is reached when the running surface is saturated with the worn material. Prior to the saturation, the friction increases directly with an increasing amount of deposited material. The material that accumulates naturally at the surface—hence, referred to as "natural third-body layer"—is estimated to be a ferrous oxide. It has an opposite effect from the Top of Rail (ToR) friction modifiers that are deposited onto the rail surface to reduce friction in a controlled manner. Additionally, the results of the study indicate that longitudinal traction decreases nonlinearly with increasing angle of attack (AoA), while lateral traction increases, also nonlinearly. The AoA is varied from -2.0 to 2.0 degrees, representing a right- and left-hand curve. Lateral traction increases at a high rate with increasing AoA between 0.0 – 0.5 degrees, and increases at a slow rate beyond 0.5 degree. Similarly, longitudinal traction reduces at a high rate for smaller AoA and at a slower rate for larger AoA. For the tapered wheel, an offset in lateral forces is observed for a right-hand curve versus a left-hand curve. The wheel taper generates a lateral traction that is present at all times. In one direction, it adds to the lateral traction due to the AoA, while in the opposite direction, it subtracts from it, resulting in unequal lateral traction for the same AoA in a right-hand versus a left-hand curve. The change in traction with changing wheel load is nearly linear under steady state conditions. Increasing the wheel load increases both longitudinal and lateral tractions linearly. This is attributed to the friction-like behavior of longitudinal and lateral tractions. An attempt is made to measure the contact shape with wheel load using pressure-sensitive films with various degrees of sensitivity. Additionally, the mathematical modeling of the wheel-roller contact in both pure steel-to-steel contact and in the presence of pressure-sensitive films is presented. The modeling results are in good agreement with the measurements, indicating that the pressure-sensitive films have a measurable effect on the shape and contact patch pressure distribution, as compared with steel-to-steel. / Doctor of Philosophy / This study provides a detailed experimental evaluation of wheel-rail interaction for railroad vehicles, using the Virginia Tech Federal Railroad Administration (VT-FRA) Roller Rig. Better understanding the dynamics and mechanics of wheel-rail interaction would significantly contribute to the development of technologies, materials, and operational methods that can further improve fuel efficiency, and reduce wheel and rail wear. Considering that the railroads are the backbone of cargo and passenger transportation and are critical to economic well-being, the results of this study are expected to contribute to the betterment of society. An attempt is made to emulate the field application of railroad wheels on tracks on the rig under precise, highly-controlled and repeatable conditions. For each set up, the contact forces are measured for different parameters, such as wheel loads. Beyond the contact forces, the wheel profile degradation and the deposition of worn materials are measured and estimated as a function of time using a micron-precision laser optics measurement device. It is determined that the accumulation of the worn material at the contact surface, which appears as a fine gray powder, increases contact forces. The effect of wheel load on contact forces is almost linear. Additionally, the results of the study indicate that the yaw angle between the wheel and the roller (AoA) changes the contact forces direction, which has a higher rate of change for a small AoA such as 0.0 – 0.5 degrees, compared to a larger AoA. An attempt is made to measure the contact shape with wheel load and AoA using pressure-sensitive films with various degrees of sensitivity. Additionally, the mathematical modeling of the wheel-roller contact in both pure steel-steel contact and in the presence of pressure-sensitive films is presented. As expected, both the model and test result indicate that the presence of a film at the contact surface changes both the dimensions and pressure distribution at the contact patch. Quantifying the distortion that occurs as a result of the pressure-sensitive film allows for a better assessment of the pressure distribution measurements that are made with the films in order to potentially discount the resulting distortions.