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Atmospheric aerosol particles also known as atmospheric particulate matter or particulate matter (PM) are microscopic particles (solid or liquid) suspended in air, which is one of six air pollutants in US air quality standard. PM is classified as coarse particles with diameters between 2.5 to 10 mm, fine particles with a diameter less than 2.5 mm (PM2.5), and ultrafine particles with the diameter less than 0.1 mm (PM0.1). Epidemiological studies have already showed the adverse health effects (such as asthma, lung cancer and respiratory and cardiovascular disease) resulted from exposure to the fine and ultrafine particles. Monitoring the PM concentration (i.e., either mass or surface area concentration of PM) is critical for the protection of public health and environment and for the regulatory control. Various PM sensors are now available in market. A majority of these PM sensors are optical sensors, whose readouts are highly depended on the physical property and composition of PM. Several PM monitors based on the measurement principle of electrical charging are also available. However, the empirical calibration of the readout of these electrical PM monitors via the use of standard dust particles makes it difficult to obtain the true mass concentration of PM when PM size distribution is different from that of standard dust. The overall objective of this dissertation is to advance our scientific knowledge on the performance of cost-effective PM monitors for measuring either mass or surface area concentration of fine and ultrafine PM. This thesis includes two parts: (1) is on the evaluation of existing PM sensor for PM mass concentration measurement; (2) is on the development of new PM monitor for PM surface area concentration measurement. For the first part of this dissertation, four low-cost optical sensors, one Personal Dust Monitor (PDM) and DustrakTM were experimentally evaluated. Particles in the size distribution having different mean size, standard deviation value and material were used as test aerosol particles. The readouts of these low-cost and portable sensors are compared to that of a standard TEOM (Tapered Element Oscillation Microbalance). For the second part of this dissertation, a new electrical PM monitor, consisting of a corona-based aerosol charger, a precipitator and high sensitive current meter, has been proposed for measuring surface area concentration of fine and ultrafine PM. Particles are electrically charged upon entering an electrical PM monitor. Instead of using Faraday cage and current meter to measure the charges carried by particles in existed electrical PM sensors, the new PM monitor measures the current carried by particles deposited directly on the wall of the precipitator. A thorough evaluation has been carried out to evaluate the fundamental performance of this new PM monitor. In addition, small cyclones (i.e., quadru-inlet and tapered-body cyclones) were also evaluated as the size-selective inlet of these PM sensors/monitors to minimize the potential interface from the presence of PM with large sizes in the air. The small quadru-inlet cyclone is to resolve the issue of directional sampling; and the tapered-body cyclones is to reduce the cyclone pressure drop while having small cyclone cutoff particle size. Each cyclone has been evaluated via the measurement of particle penetration curve and pressure drop. Semi-empirical models have been obtained for the prediction of cyclone performance.

The movement of tropical cyclones (TC) is studied numerically based on a two-dimensional barotropic model, using a previously developed non-oscillatory balanced scheme. The model of TC used here takes an exponential form, and its size and strength are selected to be of a middle scale. Without a background flow, TCs move in the northwest direction due to the beta effect. The amplitudes of high wavenumber modes of the asymmetric flow, that are believed to be responsible for the TC drift, are computed using Fourier analysis. The amplitude of wavenumber one and two modes are dominant, so they are indicators of beta conversion of energy. Also, the effect of the monsoon trough on the TC movement is investigated. The results show a sudden change of the TC propagation path, consistent with earlier work. These two studies correspond to previous works. Here, the effect of equatorially trapped waves such as Kelvin, Rossby, and Mixed Rossby Gravity, on the TC path is newly studied by varying the wavenumber and wave speed of the underlying waves. The effect of the waves is considered because they are believed to contribute to cyclogenesis. For studying the effect, the barotropic flow induced by these waves via momentum transport and its variation were simulated for 50 days, and some patterns are found in the change of maximum wind speed. At a given time during the simulation, a TC is injected and the effect of the background wave is analyzed. Using the wavefield of 11 cases from 10 days to 30 days, the trajectories are calculated, and their patterns appear to be stochastic. So, the patterns are identified by calculating the mean path and its spread. The trajectories of TCs are different for different time of the waves. Kelvin waves make small variations on the length and direction of the trajectory of TCs. On the contrary, Rossby waves cause a dramatic change in the TC path and yield longer trajectories. Meanwhile, TCs in MRG waves keep fairly the same direction and usually have longer traveling distance. These changes vary by wave conditions. Therefore, the three kinds of waves have different effects on the trajectories of the TC. For some peculiar cases, the movements are explained based on wavefields. / Graduate

The vertical structures of tropospheric temperature and moisture over the oceans have not been well observed to date. The Atmospheric Infrared Sounder (AIRS) aboard NASA?s Aqua satellite offers the opportunity to provide observed soundings of these variables. This thesis focuses on the validation and application of AIRS soundings in the tropical troposphere over the Atlantic Ocean, with emphasis on the Saharan Air Layer (SAL). SAL outbreaks occur every few days, producing a warm air mass that is particularly dry at the middle levels. These westward-propagating plumes inhibit convection and are thereby thought to possess a detrimental effect on African easterly waves and tropical cyclones (TCs). First, AIRS soundings are compared with concurrent Global Positioning System (GPS) dropwindsonde data released from NOAA?s Gulfstream-IV jet aircraft, for three TC cases. In SAL environments, temperature soundings from both instruments are usually consistent. Additionally, AIRS is able to capture the very dry air in the middle levels, but it generally underestimates the moisture in the boundary layer and often misses the sharp vertical moisture gradient at the SAL base (~850 hPa). In the moist tropical boundary layer, AIRS also exhibits a dry bias. Cloud cover also prevents AIRS from accurately sampling the low-level moisture. Next, total precipitable water is derived from AIRS soundings and averaged over daily, monthly and seasonal timescales. The significant monthly and interannual variability of the moisture distribution is found to be consistent with expectations. A peak in the probability density function of mixing ratio corresponding to dry air is observed in the lower-mid troposphere in early summer, consistent with the increased frequency of SAL outbreaks during this period. Finally, the relationship between dry air derived from AIRS and TC intensity is explored. As the amount of dry air increases, particularly in the southeast and northeast quadrants of the TC, the TC becomes more likely to weaken. In the presence of high wind shear or low sea surface temperature, the likelihood of weakening increases further. While these results highlight some shortcomings of the AIRS data, their importance and uniqueness are emphasized via new applications of AIRS soundings over data sparse regions.

This thesis seeks to identify locations in which errors in numerical model initial conditions may compromise skill in tropical cyclone (TC) track forecasts. Two major TCs that made landfall in 2008 are analyzed: Hurricane Ike and Typhoon Sinlaku. In order to examine the sensitivity of the TC to selected synoptic features, a vorticity perturbation technique is developed. Within a chosen radius and atmospheric depth, the vorticity is amplified or decreased, followed by a re-balancing of the fields. The following questions are proposed: (1) How does the TC track vary with respect to initial perturbations of differing amplitude, spatial scale and distance to the storm? (2) How does the evolving perturbation act to modify the synoptic environment surrounding the TC, and thereby the track? (3) Is it best to follow an objective technique to determine the sensitive areas, or is it better to use a subjective method based on fundamental synoptic reasoning? Utilizing the Weather Research and Forecasting (WRF) model, the ?control? simulation for each TC is found to replicate forecast errors evident in the operational global models. For Sinlaku, this includes a premature recurvature in the forecast. For Ike, this comprises a landfall too far south along the Texas coast due to no recurvature being forecast. The size, magnitude and location of vorticity perturbations to the control analysis are chosen subjectively. For Sinlaku, these locations include a large mid-latitude shortwave trough around 3000 km to the north-northwest, a smaller upper-level shortwave immediately to the north, a low-level monsoon trough to the west-southwest, a weak tropical storm to the northeast, and a local perturbation in the immediate environment. It is found that WRF forecasts of Sinlaku exhibit high sensitivity, with large modifications to its track arising from the perturbation of each selected targets in the synoptic environment. The greatest improvement in the track forecast occurs by weakening the vorticity associated with each of two shortwaves to the north of Sinlaku, suggesting that either or both of the shortwaves may have been initialized too strongly in the model analysis, thereby contributing to an erroneous recurvature. For Ike, the perturbation locations include a large mid-latitude shortwave trough 2500 km to its north, an upper-level cutoff low to the east-northeast, a low-level shortwave trough to the northwest, a tropical storm in the East Pacific, and a local perturbation in the immediate environment. In contrast to Sinlaku, the perturbation of synoptic targets around Ike produces less sensitivity, likely due to the fact that Ike is not in a position of imminent recurvature. The only perturbation that leads to an accurate 4-day forecast of recurvature and landfall in North Texas is the strengthening of the large mid-latitude shortwave trough, suggesting that the shortwave may have been initialized too weakly in the operational models. Finally, a comparison of targets selected objectively by the Ensemble Transform Kalman Filter (ETKF) versus the above subjectively-chosen targets suggests that while the ETKF effectively indicates similar target regions to those selected subjectively, it may be less effective in ranking the relative sensitivities of those targets. Overall, it is found that the TC track is more sensitive to perturbations of larger amplitude and spatial scale, and less so to the distance between the perturbation and the TC, and sensitivity is confined to specific regions of the flow. The perturbation methodology employed here may be used to offer suggestions of locations in which extra high-density satellite data may be assimilated.

Tropical cyclone (TC) intensity change is governed by internal dynamics (e.g. eyewall contraction, eyewall replacement cycles, interactions of the inner-core with the rainbands) and environmental conditions (e.g. vertical wind shear, moisture distribution, and surface properties). This study aims to gain a better understanding of the physical mechanisms responsible for TC intensity changes with a particular focus to those related to the vertical wind shear and surface properties by using high resolution, full physics numerical simulations. First, the effects of the vertical wind shear on a rapidly intensifying storm and its subsequent weakening are examined. Second, a fully coupled atmosphere-wave-ocean model with a sea spray parameterization is used to study the impact of sea spray on the hurricane boundary layer. The coupled model consists of three components: the high resolution, non-hydrostatic, fifth generation Pennsylvania State University-NCAR mesoscale model (MM5), the NOAA/NCEPWAVEWATCH III (WW3) ocean surface wave model, and theWHOI threedimensional upper ocean circulation model (3DPWP). Sea spray parameterizations were developed at NOAA/ESRL and modified by the author to be introduced in uncoupled and coupled simulations. The model simulations are conducted in both uncoupled and coupled modes to isolate various physical processes influencing TC intensity. The very high-resolutionMM5 simulation of Hurricane Lili (at 0.5 km grid resolution) showed a rapid intensification associated with a contracting eyewall. Changes in both the magnitude and the direction of the vertical wind shear associated with an approaching upper-tropospheric trough were responsible for the weakening of the storm before landfall. Hurricane Lili weakened in a 5-10 m/s vertical wind shear environment. The simulated storm experienced wind shear direction normal to the storm motion, which produced a strong wavenumber one rainfall asymmetry in the downshear-left quadrant of the storm. The rainfall asymmetry was confirmed by various observations from the TRMM satellite and the WSR-88D ground radar in the coastal region. The increasing vertical wind shear induced a vertical tilt of the vortex with a time lag of about 5-6 hours after the wavenumber one rainfall asymmetry was first observed in the model simulation. Other key factors controlling intensity and intensity change in tropical cyclones are the air-sea fluxes. Accurate measurement and parameterization of air-sea fluxes under hurricane conditions are challenging. Although recent studies have shown that the momentum exchange coefficient levels off at high wind speed, little is known about the high wind behavior of the exchange coefficient for enthalpy flux. One of the largest uncertainties is the potential impact of sea spray. The current sea spray parameterizations are closely tied to wind speed and tend to overestimate the mediated heat fluxes by sea spray in the hurricane boundary layer. The sea spray generation depends not only on the wind speed but also on the variable wave state. A new spray parameterization based on the surface wave energy dissipation is introduced in the coupled model. In the coupled simulations, the wave energy dissipation is used to quantify the amount of wave breaking related to the generation of sea spray. The spray parameterization coupled to the waves may be an improvement compared to sea spray parameterizations that depends on wind speed only.

Thesis (Ph. D.)--Texas State University-San Marcos, 2006. / Vita. Appendices: leaves 119-142. Includes bibliographical references (leaves 143-147).

To design a cyclone abatement system for particulate control, it is necessary to accurately estimate cyclone performance. In this cyclone study, new theoretical methods for computing travel distance, numbers of turns and cyclone pressure drop have been developed. The flow pattern and cyclone dimensions determine the travel distance in a cyclone. The number of turns was calculated based on this travel distance. The new theoretical analysis of cyclone pressure drop was tested against measured data at different inlet velocities and gave excellent agreement. The results show that cyclone pressure drop varies with the inlet velocity, but not with cyclone diameter. Particle motion in the cyclone outer vortex was analyzed to establish a force balance differential equation. Barth??s "static particle" theory, particle (with diameter of d50) collection probability is 50% when the forces acting on it are balanced, combined with the force balance equation was applied in the theoretical analyses for the models of cyclone cut-point and collection probability distribution in the cyclone outer vortex. Cyclone cut-points for different dusts were traced from measured cyclone overall collection efficiencies and the theoretical model for calculating cyclone overall efficiency. The cut-point correction models (K) for 1D3D and 2D2D cyclones were developed through regression fit from traced and theoretical cut-points. The regression results indicate that cut-points are more sensitive to mass median diameter (MMD) than to geometric standard deviation (GSD) of PSD. The theoretical overall efficiency model developed in this research can be used for cyclone total efficiency calculation with the corrected d50 and PSD. 1D3D and 2D2D cyclones were tested at Amarillo, Texas (an altitude of 1128 m / 3700 ft), to evaluate the effect of air density on cyclone performance. Two sets of inlet design velocities determined by the different air densities were used for the tests. Experimental results indicate that optimal cyclone design velocities, which are 16 m/s (3200 ft/min) for 1D3D cyclones and 15 m/s (3000 ft/min) for 2D2D cyclones, should be determined based on standard air density. It is important to consider the air density effect on cyclone performance in the design of cyclone abatement systems.

To design a cyclone abatement system for particulate control, it is necessary to accurately estimate cyclone performance. In this cyclone study, new theoretical methods for computing travel distance, numbers of turns and cyclone pressure drop have been developed. The flow pattern and cyclone dimensions determine the travel distance in a cyclone. The number of turns was calculated based on this travel distance. The new theoretical analysis of cyclone pressure drop was tested against measured data at different inlet velocities and gave excellent agreement. The results show that cyclone pressure drop varies with the inlet velocity, but not with cyclone diameter. Particle motion in the cyclone outer vortex was analyzed to establish a force balance differential equation. Barth??s "static particle" theory, particle (with diameter of d50) collection probability is 50% when the forces acting on it are balanced, combined with the force balance equation was applied in the theoretical analyses for the models of cyclone cut-point and collection probability distribution in the cyclone outer vortex. Cyclone cut-points for different dusts were traced from measured cyclone overall collection efficiencies and the theoretical model for calculating cyclone overall efficiency. The cut-point correction models (K) for 1D3D and 2D2D cyclones were developed through regression fit from traced and theoretical cut-points. The regression results indicate that cut-points are more sensitive to mass median diameter (MMD) than to geometric standard deviation (GSD) of PSD. The theoretical overall efficiency model developed in this research can be used for cyclone total efficiency calculation with the corrected d50 and PSD. 1D3D and 2D2D cyclones were tested at Amarillo, Texas (an altitude of 1128 m / 3700 ft), to evaluate the effect of air density on cyclone performance. Two sets of inlet design velocities determined by the different air densities were used for the tests. Experimental results indicate that optimal cyclone design velocities, which are 16 m/s (3200 ft/min) for 1D3D cyclones and 15 m/s (3000 ft/min) for 2D2D cyclones, should be determined based on standard air density. It is important to consider the air density effect on cyclone performance in the design of cyclone abatement systems.

Despite the numerous advantages associated with using compact cylindrical cyclone gas/liquid separators, particularly for upstream production operations, the lack of a full understanding of the complex hydrodynamic process taking place in it and its “unfamiliarity” to oil field personnel has hindered its widespread use. The complexity associated with this technology is attributed to two limiting physical phenomena, liquid carry-over and gas carryunder. While a lot of work has been done to better understand and predict the liquid carry-over operational envelope, little or no information about methods capable of adequately predicting or characterizing the gas carry-under performance of such separators is available. Traditionally, to mitigate the gas carry-under phenomena, the use of complex control algorithms and systems has been employed. These systems make the technology expensive (as opposed to the potential cost reduction it promises) and impractical for realistic use in the oil field where reliability is of critical importance. A simpler solution, the use of changeable or adjustable inlet-slots that regulate the artificial gravity environment created in the separator, could significantly improve the gas carry-under performance of cylindrical cyclone separators. This research has focused primarily on the use of adjustable inlet-slots. Theoretical analysis and experimental data investigating the benefits of variable inlet geometry have been provided. This work lays the foundation or validation required to perform more tests on a field-scale version to verify the results presented here. A modular design of such a variable inlet-slot inletsection has the potential of simplifying the design and specifications of cylindrical cyclone gas/liquid separators. From the results of this investigation, it was found that the gas carry-under performance of a cylindrical cyclone gas/liquid separator could be improved considerably over a wider range of operating conditions by adjusting the size of the inlet-slots. This contradicts earlier reports of liquid carry-over improvement in separator performance. Also, for the first time, a simple method for theoretically analyzing the percent improvement in separator gas carry-under performance using the optimum g-force concept is presented. This method could be incorporated into design software for determining the slot-size configuration required for varying separator-operating conditions.