<p>Nonlinear transmission lines (NLTLs) are of great interest for high power microwave (HPM) generation because they can sharpen pulses to create an electromagnetic shockwave to produce oscillations from 100 MHz to low GHz. NLTLs provide frequency agility, compactness, durability and reliability, providing a solid-state radiofrequency (RF) source for producing HPM. The essential component of NLTLs is the nonlinear material, typically a dielectric that varies with voltage or a magnetic material whose permeability varies with current, incorporated in the transmission line in various topologies. This thesis presents an alternative approach involving designing composites comprised of nonlinear dielectric inclusions (barium strontium titanate (BST)) and/or nonlinear inductive inclusions (nickel zinc ferrites (NZF)) in a polymer base host material, analogous to electromagnetic interference designs that incorporate stainless steel inclusions of various shapes in a plastic to tune the composite’s electromagnetic properties at GHz. Appropriately designing NLTL composites requires predicting these effective properties both in linear (for a fixed and low voltage and current) and nonlinear regions (permittivity and permeability become voltage dependent and current dependent, respectively) prior to designing HPM systems comprised of them. As a first step, this thesis evaluates and benchmarks composites models in the commercial software CST Microwave Studios (CST MWS) to various effective medium theories (EMTs) to predict the permittivity and permeability of composites of BST and/or NZF inclusions in the linear regime, compared with experimental measurements. The manufacturing and measurement of the nonlinear composites will be briefly discussed with an analysis of the homogeneity of a composite sample using 3D X-ray scan. Long-term application of these approaches to predicting the effective nonlinear composite permittivity and permeability and future work will be discussed.</p>