Results are presented for Floquet calculations of photodetachment rates from a one-dimensional model atom irradiated by intense laser light. Light-induced quasibound states are found to originate from the movement of poles of the multichannel scattering matrix on the Riemann energy surface. The appearance of new bound states of the negative Hydrogen ion, recently predicted, is related to the motion of resonance poles that correspond to autoionising states in the absence of the field. A number of pole trajectories, leading to light-induced states, are discussed for the one-dimensional model atom. The Floquet method allows one to represent the wave function of a quantum system in a laser field, as an infinite sum of harmonic basis functions. In any practical calculation this infinite sum must be truncated. The consequences of representing the wave function, via the Floquet method, by a finite sum of harmonics is addressed. An illustration of these consequences is made by way of a number of representative calculations performed on a one-dimensional model atom. Results are presented of calculations performed to determine the influence of a laser field, of low to moderate intensity, upon the partial and total photodetachment rates of the negative Hydrogen ion, H(^-). Using the R-matrix Floquet method, a study is undertaken into the detachment of an electron from the ion, via multiphoton transitions through one of several autodetaching resonances of the ion. The discussion focuses on the influence of the laser field upon auto detaching pathways. It is found that the laser may induce structure into the continuum that does not exist in the absence of the laser field, or, conversely, may suppress field-free structure. In the latter case, the suppression of structure is related to the appearance of laser-induced degeneracies.

Abstract The topic of this thesis is superconducting electric circuits. Technical advances have made possible the experimental study of Josephson junction based circuit elements which sustain quantum mechanical properties long enough to be denoted as quantum devices. The quantum state can be controlled with electronic variables and measured using standard electrical setups. The research is motivated by the possibility to examine quantum phenomena in circumstances that can be customized, prospects of new quantum devices, and the development of quantum information processing. This thesis presents theoretical studies on the nonlinear and stochastic driving of a superconducting quantum two-level system (qubit). We first investigate the energy level shifts a single-Cooper-pair transistor under large amplitude driving realized via the inherently nonlinear Josephson energy by using an external magnetic flux. The effective driving field substantially deviates from a circular polarization and linear coupling. The energy level shifts are compared to the cases of a vanishing and a weak driving field, measured as the Stark shift and the generalized Bloch-Siegert shift, respectively. We describe criteria for the natural basis of the analytical and the numerical calculations. In addition to that, we develop a formalism based on the Floquet method for the weak probe measurement of the strongly driven qubit. In the latter part of the thesis research, we study utilization of a stochastic driving field whose time evolution is not regular but follows probabilistic laws. We concentrate on the motional averaging phenomenon and show that it can be measured with an unparalleled accuracy by employing a flux-modulated transmon qubit. As the stochastically modulated qubit is simultaneously measured with a moderate driving field, we develop a theoretical description accounting the possible interference effects between the modulation and the drive. The comparison with experimental results shows good agreement. Motional averaging phenomenon can be applied to estimate the properties of fluctuation processes occurring in qubits, e.g., the quasiparticle tunneling or the photon shot noise. Resting on the motional averaging, we anticipate that the qubit dephasing times can be improved if one can accelerate the dynamics of two-level fluctuators. We apply a semiclassical formalism where the qubit is treated with quantum mechanical concepts whereas the driving fields are classical. In the solution procedure, the numerical results support the main analytical understanding. As the theoretical results are extensively compared to reflection measurements, we construct an explicit connection between the dynamics of the studied quantum devices and the measured reflection coefficient.

Abstract Elementary experiments of atomic physics and quantum optics can be reproduced on a circuit board using elements built of superconducting materials. Such systems can show discrete energy levels similar to those of atoms. With respect to their natural cousins, the enhanced controllability of these ‘artificial atoms’ allows the testing of the laws of physics in a novel range of parameters. Also, the study of such systems is important for their proposed use as the quantum bits (qubits) of the foreseen quantum computer. In this thesis, we have studied an artificial atom coupled with a harmonic oscillator formed by an LC-resonator. At the quantum limit, the interaction between the two can be shown to mimic that of ordinary matter and light. The properties of the system were studied by measuring the reflected signal in a capacitively coupled transmission line. In atomic physics, this has an analogy with the absorption spectrum of electromagnetic radiation. To simulate such measurements, we have derived the corresponding equations of motion using the quantum network theory and the semi-classical approximation. The calculated absorption spectrum shows a good agreement with the experimental data. By extracting the power consumption in different parts of the circuit, we have calculated the energy flow between the atom and the oscillator. It shows that, in a certain parameter range, the absorption spectrum obeys the Franck-Condon principle, and can be interpreted in terms of vibronic transitions of a diatomic molecule. A coupling with a radiation field shifts the spectral lines of an atom. In our system, the interaction between the atom and the field is nonlinear, and we have shown that a strong monochromatic driving results in energy shifts unforeseen in natural or, even, other artificial atoms. We have used the Floquet method to calculate the quasienergies of the coupled system of atom and field. The oscillator was treated as a small perturbation probing the quasienergies, and the resulting absorption spectrum agrees with the reflection measurement.

Abstract In this thesis we study the interaction between radiation and matter using superconducting circuits that behave analogously with the conventional photon-atom interaction in quantum optics. The research is done with a system consisting of a waveguide resonator (radiation) strongly coupled to a transmon device (matter). We focus on the phenomena caused by strong coupling between the radiation and matter, and by driving the resonator to higher excited states with a strong monochromatic radiation. These have been studied little in the traditional radiation-matter systems. Increasing the strength of the monochromatic radiation drive, the dynamics of the system experiences a transition from the quantum to the classical regime. Also, the free-particle states of the transmon start being populated. In the weak driving limit, the transmon can be regarded as a two-state system. As a consequence, the resonator-transmon system is conventionally discussed in terms of the linear Jaynes–Cummings model. However, for strong coupling the Bloch–Siegert shift, caused by the terms neglected in the Jaynes–Cummings model, is strong and the Jaynes–Cummings model is insufficient for describing the dynamics of the system. We study the effects caused by strong coupling and the excitation of the higher transmon states instigated by the driving of the resonator. With reflection spectroscopy, we measure the absorption spectrum of the system and compare this with the spectrum calculated numerically using the Floquet–Born–Markov approach. We find that, in the region of the quantum-to-classical transition, the two-state approximation for the transmon is insufficient and the higher transmon states are necessary for accurate simulations. By calculating the average resonator occupation, we compare different numerical models: the Lindblad master equation, the Floquet–Born–Markov, and the semiclassical model. Coupling a transmon to a resonator shifts the energy levels of the resonator. This shift in the energy levels prevents the higher resonator states from being populated if the system is weakly driven with a frequency that is near the resonance frequency of the resonator. We simulate this photon blockade numerically and show that the blockade is substantially different for the two-state and multistate transmon approximations. / Original papers Original papers are not included in the electronic version of the dissertation. Pietikäinen, I., Danilin, S., Kumar, K. S., Vepsäläinen, A., Golubev, D. S., Tuorila, J., & Paraoanu, G. S. (2017). Observation of the Bloch-Siegert shift in a driven quantum-to-classical transition. Physical Review B, 96(2). https://doi.org/10.1103/PhysRevB.96.020501 http://jultika.oulu.fi/Record/nbnfi-fe201803073899 Pietikäinen, I., Danilin, S., Kumar, K. S., Tuorila, J., & Paraoanu, G. S. (2018). Multilevel Effects in a Driven Generalized Rabi Model. Journal of Low Temperature Physics, 191(5–6), 354–364. https://doi.org/10.1007/s10909-018-1857-8 http://jultika.oulu.fi/Record/nbnfi-fe2018061325770 Pietikäinen, I., Tuorila, J., Golubev, D. S., & Paraoanu, G. S. (2019) Quantum-to-classical transition in the driven-dissipative Josephson pendulum coupled to a resonator, Manuscript. https://arxiv.org/abs/1901.05655