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Study of nonlinear optical properties of fullerenes and related compounds by optical Kerr effect: 應用光學克爾效應硏究足球烯分子及有關化合物之非線性光學性質. / 應用光學克爾效應硏究足球烯分子及有關化合物之非線性光學性質 / Study of nonlinear optical properties of fullerenes and related compounds by optical Kerr effect: Ying yong guang xue ke er xiao ying yan jiu zu qiu xi fen zi ji you guan hua he wu zhi fei xian xing guang xue xing zhi. / Ying yong guang xue ke er xiao ying yan jiu zu qiu xi fen zi ji you guan hua he wu zhi fei xian xing guang xue xing zhiJanuary 1997 (has links)
Yung, Man Fai. / Thesis (M.Phil.)--Chinese University of Hong Kong, 1997. / Includes bibliographical references. / Yung, Man Fai. / Acknowledgements --- p.iii / Abstract --- p.iv / Preface --- p.vi / Contents --- p.vii / List of Figures --- p.x / List of Tables --- p.xii / Chapter Chapter 1. --- Introduction --- p.1 / Chapter 1.1 --- Physical Origin of Optical Nonlinearity --- p.3 / Chapter 1.1.1 --- Mathematical Description --- p.3 / Chapter 1.1.2 --- Anharmonic Oscillator Model --- p.4 / Chapter 1.2 --- Nonlinear Optical Susceptibility --- p.4 / Chapter 1.2.1 --- Molecular Hyperpolarizability --- p.4 / Chapter 1.2.2 --- Macroscopic Nonlinear Susceptibility --- p.5 / Chapter 1.2.3 --- Kleinman Conjecture --- p.6 / Chapter 1.3 --- Third-Order Nonlinear Optical Process --- p.7 / Chapter 1.3.1 --- Intensity Dependent Refractive Index --- p.7 / Chapter 1.3.2 --- Physical Mechanisms --- p.8 / Chapter 1.3.3 --- Tensor Nature of Third-Order Susceptibility x(3) --- p.10 / Chapter 1.3.4 --- Conventions for Nonlinear Susceptibility --- p.11 / References --- p.12 / Chapter Chapter 2. --- Optical Kerr Effect --- p.13 / Chapter 2.1 --- Introduction --- p.13 / Chapter 2.2 --- Theoretical Background --- p.14 / Chapter 2.2.1 --- Pump-Probe Technique --- p.14 / Chapter 2.2.2 --- Description of Induced Birefringence --- p.15 / Chapter 2.2.3 --- Signal Transmitted through OKE --- p.17 / Chapter 2.2.4 --- Resonant OKE --- p.18 / Chapter 2.2.5 --- Third-Order Autocorrelation --- p.19 / Chapter 2.3 --- Applications --- p.20 / References --- p.21 / Tables --- p.23 / Figure Captions --- p.24 / Chapter Chapter 3. --- Nonlinear Optical Properties of Fullerenes --- p.26 / Chapter 3.1 --- Introduction --- p.26 / Chapter 3.2 --- Second Harmonic Generation --- p.27 / Chapter 3.3 --- Third-Order Effects --- p.28 / Chapter 3.4 --- Reverse Saturable Absorption and Optical Limiting --- p.29 / References --- p.32 / Figure Captions --- p.34 / Chapter Chapter 4. --- Excited State Enhancement --- p.38 / Chapter 4.1 --- Introduction --- p.38 / Chapter 4.2 --- Origin and Properties of Excited State Enhancement --- p.39 / Chapter 4.3 --- Experimental Demonstrations --- p.42 / References --- p.44 / Chapter Chapter 5. --- Experimental Setup --- p.46 / Chapter 5.1 --- Introduction --- p.46 / Chapter 5.2 --- Laser System --- p.46 / Chapter 5.3 --- Optical Layout --- p.48 / Chapter 5.4 --- Sample Preparation --- p.50 / Chapter 5.5 --- Detection System --- p.51 / Chapter 5.6 --- Third-Order Autocorrelation Measurement --- p.52 / Chapter 5.7 --- Optical Limiting Measurement --- p.53 / Chapter 5.8 --- Excited State Enhancement Measurement --- p.54 / References --- p.56 / Figure Captions --- p.57 / Chapter Chapter 6. --- Results and Discussion --- p.69 / Chapter 6.1 --- Introduction --- p.69 / Chapter 6.2 --- Results of Pure Liquids --- p.69 / Chapter 6.2.1 --- Carbon Disulfide (CS2) --- p.69 / Chapter 6.2.2 --- Toluene --- p.71 / Chapter 6.2.3 --- Nitrobenzene --- p.71 / Chapter 6.3 --- Third-Order Autocorrelation of CS2 --- p.74 / Chapter 6.4 --- Results of Fullerenes C60 and C70 --- p.75 / Chapter 6.5 --- Optical Limiting of C60 --- p.78 / Chapter 6.6 --- Excited State Enhancement of Fullerenes --- p.79 / References --- p.82 / Tables --- p.85 / Figure Captions --- p.90 / Chapter Chapter 7. --- Conclusion --- p.108
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