Thesis (Ph. D.)--University of Texas at Austin, 2007. / Vita. Includes bibliographical references.

Thesis (M.S.)--California Polytechnic State University, 2009. / Title from PDF title page; viewed on January 13, 2010. Major professor: William Ahlgren, Ph.D. "Presented to the Electrical Engineering faculty of California Polytechnic State University, San Luis Obispo." "In partial fulfillment of the requirements for the degree [of] Master of Science in Electrical Engineering." "December 2009." Includes bibliographical references (p. 81-87).

Traditional approaches in gamma-ray spectroscopy for determining the absolute full-energy peak efficiencies of germanium detectors are primarily either too time consuming or not economically viable. In addition, these approaches are difficult to use for arbitrary source shapes and counting geometries. An open source software package, KMESS (Kevin's Mesh Efficiency Simulator Software), was developed to address these problems. KMESS uses a new semi-empirical mesh-grid method to predict the absolute full-energy peak efficiencies of n- and p-type germanium detectors in both coaxial and closed-ended configurations. The model assumes that any gamma-ray source shape can be treated as a collection of point sources. The code was written in a modular form, making it easy to adapt for other detector configurations and materials. A suite of webbased graphical front-end tools was also developed to make the execution of KMESS user-friendly. KMESS can predict most full-energy peak efficiencies to within 10% accuracy for the energy range 100-1800 keV in less than 10 minutes. / text

Thesis (MSc)--Stellenbosch University, 2015. / ENGLISH ABSTRACT: The coincident measurement of gamma-rays originating from nuclei excited in light-ion reactions and scattered alpha-particles presents interesting opportunities to characterize the decay path for low multi-polarity nuclear excitations. This coincident measurement at θlab = 0◦ was shown to be a powerful tool for the spectroscopy of isoscalar E1 transitions, being selective to distinct modes of bulk nuclear motions. Aided with the high resolution capabilities provided by the HPGe Clover detectors as well as the K600 magnetic spectrometer for both γ and charged particle detection, these experiments are motivated by the need to investigate E1 strength in stable nuclei around the particle emission threshold, more commonly referred to as the Pygmy Dipole Resonance (PDR). However, due to our detector configuration we find that higher effi- ciency detectors offer a better overall functionality in these α − γ coincidence measurements which specifically suffer from low statistics. The feasibility of the (α, α 0γ) reaction using high resolution Clover detectors and the high efficiency HAGAR detector is characterized through their effi- ciency to detect γ rays in coincidence with the K600 magnetic spectrometer at θlab = 0◦ . Through the construction of Eγ − EX coincidence matrices, decay transitions of closely lying nuclear excitations can be studied on a stateby-state basis. The result is a quantified representation of γ yield, of which optimization is the key focus in order to extract meaningful nuclear structure information. / AFRIKAANSE OPSOMMING: Die samevallende meting van gammastrale van kerne opgewek in die lig-ion reaksies en verspreide alfa-deeljties, bied interessante geleenthede aan om die verval pad vir lae multi-polariteit kern opwekkings te karakteriseer. Hierdie samevallende meting by θlab = 0◦ was getoon om ‘n kragtige instrument vir die spektroskopie van isoscalar E1 oorgange te wees, as gevolg van die vermoë om selektief te onderskei tussen modes van kollektiewe kern ossillasies. Aangehelp met die hoë resolusie moontlikhede wat deur die HPGe Clover detektors asook die K600 magnetiese spektrometer vir beide γ en gelaaide deeltjie opsporing, hierdie eksperimente is gemotiveer deur die behoefte om E1 krag te ondersoek in stabiele kerne rondom die deeltjie emissie drumpel, meer algemeen na verwys as die Pygmy Dipool Resonansie (PDR). Maar as gevolg van die detektor opset, vind ons dat ’n hoër doeltreffendheid detector ’n beter algehele funksionaliteit aanbied wat in hierdie samevallende metings veral belangrik is weens lae statistiek. Die haalbaarheid van die reaksie wat gebruik maak van hoë resolusie Clover detektors en die hoë doeltreffendheid HAGAR detektor word gekenmerk deur hul doeltreffendheid om gammastrale optespoor in toeval met die K600 magnetiese spektrometer by θlab = 0◦ . Deur die konstruksie van toeval Eγ − EX matrikse, verval oorgange van kern opwekkings kan op ’n staat-by-staat basis bestudeer word. Die resultaat is ’n gekwantifiseerde verteenwoordiging van γ opbrengs, waarvan optimalisering die sleutel fokus is om betekenisvolle kernstruktuur inligting te kan onttrek

The Environmental Radioactivity Laboratory (ERL) at iThemba LABS undertakes experimental work using a high purity germanium (HPGe) detector for laboratory measurements. In this study the Monte Carlo transport code, MCNPX, which is a general-purpose Monte Carlo N &minus / Particle code that extends the capabilities of the MCNP code, developed at the Los Alamos National Laboratory in New Mexico, was used. The study considers how various parameters such as (1) coincidence summing, (2) volume, (3) atomic number (Z) and (4) density, affects the absolute photopeak efficiency of the ERL&rsquo / s HPGe detector in a close geometry (Marinelli beaker) for soil, sand, KCl and liquid samples. The results from these simulations are presented here, together with an intercomparison exercise of two MC codes (MCNPX and a C++ program developed for this study) that determine the energy deposition of a point source in germanium spheres of radii 1 cm and 5 cm.<br /> <br /> A sensitivity analysis on the effect of the detector dimensions (dead layer and core of detector crystal) on the photopeak detection efficiency in a liquid sample and the effect of moisture content on the photopeak detection efficiency in sand and soil samples, was also carried out. This study has shown evidence that the dead layer of the ERL HPGe detector may be larger than stated by the manufacturer, possibly due to warming up of the detector crystal. This would result in a decrease in the photopeak efficiency of up to 8 % if the dead layer of the crystal were doubled from its original size of 0.05 cm. This study shows the need for coincidence summing correction factors for the gamma lines (911.1 keV and 968.1 keV) in the 232Th series for determining accurate activity concentrations in environmental samples. For the liquid source the gamma lines, 121.8 keV, 244.7 keV, 444.1 keV and 1085.5 keV of the 152Eu series, together with the 1173.2 keV and 1332.5 keV gamma lines of the 60Co, are particularly prone to coincidence summing. In the investigation into the effects of density and volume on the photopeak efficiency for the KCl samples, it has been found that the simulated results are in good agreement with experimental data. For the range of sample densities that are dealt with by the ERL it has been found that the drop in photopeak efficiency is less than 5 %. This study shows that the uncertainty of the KCl sample activity measurement due to the effect of different filling volumes in a Marinelli beaker is estimated in the range of 0.6 % per mm and is not expected to vary appreciably with photon energy. In the case of the effect of filling height on the efficiency for the soil sample, it was found that there is a large discrepancy in the trends of the simulated and experimental curves. This discrepancy could be a result of the use of only one sand sample in this study and therefore the homogeneity of the sample has to be investigated. The effect of atomic number has been found to be negligible for the soil and sand compositions for energies above 400 keV, however if the composition of the heavy elements is not properly considered when simulating soil and sand samples, the effect of atomic number on the absolute photopeak efficiency in the low energy (&lt / 400 keV) region can make a 14 % difference.

<p>The natural &sup2 / &sup3 / ⁸U, &sup2 / &sup3 / &sup2 / Th and ⁴&deg / K radioactive content of vineyard soil was measured with an in-situ gamma-ray detector. The activity concentration measured with the in-situ detector are normalized using the laboratory-determined activity concentrations of several samples from the vineyard site. To determine the activity concentration of a particular soil sample, the gamma-ray photopeak detection efficiencies are required. In this work, the detection efficiencies were derived for each soil sample using gamma-ray photopeaks associated with the radionuclide of &sup2 / &sup3 / ⁸U, &sup2 / &sup3 / &sup2 / Th present in the sample, and the ⁴&deg / K, 1460.8 keV gamma-ray peak, from KCl salt.</p>

The Environmental Radioactivity Laboratory (ERL) at iThemba LABS undertakes experimental work using a high purity germanium (HPGe) detector for laboratory measurements. In this study the Monte Carlo transport code, MCNPX, which is a general-purpose Monte Carlo N &minus / Particle code that extends the capabilities of the MCNP code, developed at the Los Alamos National Laboratory in New Mexico, was used. The study considers how various parameters such as (1) coincidence summing, (2) volume, (3) atomic number (Z) and (4) density, affects the absolute photopeak efficiency of the ERL&rsquo / s HPGe detector in a close geometry (Marinelli beaker) for soil, sand, KCl and liquid samples. The results from these simulations are presented here, together with an intercomparison exercise of two MC codes (MCNPX and a C++ program developed for this study) that determine the energy deposition of a point source in germanium spheres of radii 1 cm and 5 cm.<br /> <br /> A sensitivity analysis on the effect of the detector dimensions (dead layer and core of detector crystal) on the photopeak detection efficiency in a liquid sample and the effect of moisture content on the photopeak detection efficiency in sand and soil samples, was also carried out. This study has shown evidence that the dead layer of the ERL HPGe detector may be larger than stated by the manufacturer, possibly due to warming up of the detector crystal. This would result in a decrease in the photopeak efficiency of up to 8 % if the dead layer of the crystal were doubled from its original size of 0.05 cm. This study shows the need for coincidence summing correction factors for the gamma lines (911.1 keV and 968.1 keV) in the 232Th series for determining accurate activity concentrations in environmental samples. For the liquid source the gamma lines, 121.8 keV, 244.7 keV, 444.1 keV and 1085.5 keV of the 152Eu series, together with the 1173.2 keV and 1332.5 keV gamma lines of the 60Co, are particularly prone to coincidence summing. In the investigation into the effects of density and volume on the photopeak efficiency for the KCl samples, it has been found that the simulated results are in good agreement with experimental data. For the range of sample densities that are dealt with by the ERL it has been found that the drop in photopeak efficiency is less than 5 %. This study shows that the uncertainty of the KCl sample activity measurement due to the effect of different filling volumes in a Marinelli beaker is estimated in the range of 0.6 % per mm and is not expected to vary appreciably with photon energy. In the case of the effect of filling height on the efficiency for the soil sample, it was found that there is a large discrepancy in the trends of the simulated and experimental curves. This discrepancy could be a result of the use of only one sand sample in this study and therefore the homogeneity of the sample has to be investigated. The effect of atomic number has been found to be negligible for the soil and sand compositions for energies above 400 keV, however if the composition of the heavy elements is not properly considered when simulating soil and sand samples, the effect of atomic number on the absolute photopeak efficiency in the low energy (&lt / 400 keV) region can make a 14 % difference.

<p>The natural &sup2 / &sup3 / ⁸U, &sup2 / &sup3 / &sup2 / Th and ⁴&deg / K radioactive content of vineyard soil was measured with an in-situ gamma-ray detector. The activity concentration measured with the in-situ detector are normalized using the laboratory-determined activity concentrations of several samples from the vineyard site. To determine the activity concentration of a particular soil sample, the gamma-ray photopeak detection efficiencies are required. In this work, the detection efficiencies were derived for each soil sample using gamma-ray photopeaks associated with the radionuclide of &sup2 / &sup3 / ⁸U, &sup2 / &sup3 / &sup2 / Th present in the sample, and the ⁴&deg / K, 1460.8 keV gamma-ray peak, from KCl salt.</p>

Thesis (Ph. D.)--University of Nevada, Reno, 2008. / "May 2008." Includes bibliographical references. Online version available on the World Wide Web.

Magister Scientiae - MSc / The Environmental Radioactivity Laboratory (ERL) at iThemba LABS undertakes experimental work using a high purity germanium (HPGe) detector for laboratory measurements. In this study the Monte Carlo transport code, MCNPX, which is a general-purpose Monte Carlo N − Particle code that extends the capabilities of the MCNP code, developed at the Los Alamos National Laboratory in New Mexico, was used. The study considers how various parameters such as (1) coincidence summing, (2) volume, (3) atomic number (Z) and (4) density, affects the absolute photopeak efficiency of the ERL’s HPGe detector in a close geometry (Marinelli beaker) for soil, sand, KCl and liquid samples. The results from these simulations are presented here, together with an intercomparison exercise of two MC codes (MCNPX and a C++ program developed for this study) that determine the energy deposition of a point source in germanium spheres of radii 1 cm and 5 cm. A sensitivity analysis on the effect of the detector dimensions (dead layer and core of detector crystal) on the photopeak detection efficiency in a liquid sample and the effect of moisture content on the photopeak detection efficiency in sand and soil samples, was also carried out. This study has shown evidence that the dead layer of the ERL HPGe detector may be larger than stated by the manufacturer, possibly due to warming up of the detector crystal. This would result in a decrease in the photopeak efficiency of up to 8 % if the dead layer of the crystal were doubled from its original size of 0.05 cm. This study shows the need for coincidence summing correction factors for the gamma lines (911.1 keV and 968.1 keV) in the 232Th series for determining accurate activity concentrations in environmental samples. For the liquid source the gamma lines, 121.8 keV, 244.7 keV, 444.1 keV and 1085.5 keV of the 152Eu series, together with the 1173.2 keV and 1332.5 keV gamma lines of the 60Co, are particularly prone to coincidence summing. In the investigation into the effects of density and volume on the photopeak efficiency for the KCl samples, it has been found that the simulated results are in good agreement with experimental data. For the range of sample densities that are dealt with by the ERL it has been found that the drop in photopeak efficiency is less than 5 %. This study shows that the uncertainty of the KCl sample activity measurement due to the effect of different filling volumes in a Marinelli beaker is estimated in the range of 0.6 % per mm and is not expected to vary appreciably with photon energy. In the case of the effect of filling height on the efficiency for the soil sample, it was found that there is a large discrepancy in the trends of the simulated and experimental curves. This discrepancy could be a result of the use of only one sand sample in this study and therefore the homogeneity of the sample has to be investigated. The effect of atomic number has been found to be negligible for the soil and sand compositions for energies above 400 keV, however if the composition of the heavy elements is not properly considered when simulating soil and sand samples, the effect of atomic number on the absolute photopeak efficiency in the low energy (< 400 keV) region can make a 14 % difference. / South Africa