The atmospheric radiative transfer model MOCARAT was developed and is presented in this thesis. MOCARAT employs a Monte Carlo Technique for the accurate modeling of band radiances and reflectances in an atmospheric system with a ruffled ocean surface as a lower boundary. The atmospheric radiative transfer is modeled with consideration of molecular Rayleigh scattering, Mie Scattering and absorption on particulate matter, as well as band absorption by molecules in the wavelength channels of interest. The bidirectional reflection of downwelling light at the ocean surface is computed using the empirical relationship between surface wind field and the slope distribution of wave facets derived by Cox and Munk (1954a). A method is proposed to use the oceanic sun glint for remote sensing applications. The sensitivity of channel correlations to aerosol burden and type as well as other atmospheric and observational parameters is assessed. Comparisons of observed correlations with model results are used to check the consistency of the calibration of the airborne Multichannel Cloud Radiometer (MCR) that was employed during the Indian Ocean Experiment (INDOEX). The MCR calibration exhibited large variability from flight to flight. The method was applied to MODIS observations. Unlike the MCR, MODIS was stable where expected, although numerical values for some of the wavelengths appear to depart from theory. / Graduation date: 2004