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Abstract In this paper, the optical properties of magnetic fluid thin films are studied. We present the experimental observation of optical linear birefringence and dichroism in magnetic fluid thin film induced by crossed magnetic field perpendicular to the direction of light propagation. According to our results, we ascertain that both the magnetic birefringence and dichroism are existed. Besides, we also find that the relations between magnetic field and magneto-optical effects changed with the applied magnetic field intensity.

<p>Microphotonics has been offering a body of ideas to prospective applicationsin optics. Among those, the concept of photonic integrated circuits (PIC’s) has recently spurred a substantial excitement into the scientific community. Relisation of the PIC’s becomes feasible as the size shrinkage of the optical elements is accomplished. The elements based on photonic crystals (PCs) represent promising candidacy for manufacture of PIC’s. This thesis is devoted to tailoring of optical properties and advanced modelling of two types of photonic crystals: (Bi₃Fe₅O₁₂/Sm₃Ga₅O₁₂)<em>^m</em> and (TiO₂/Er₂O₃)<em>^m</em> potentially applicable in the role optical isolators and optical amplifiers, respectively. Deposition conditions of titanium dioxide were first investigated to maximise refractive index and minimise absorption as well as surface roughness of titania films. It was done employing three routines: deposition at elevated substrate temperatures, regular annealing in thermodynamically equilibrium conditions and rapid thermal annealing (RTA). RTA at 500 ^oC was shown to provide the best optical performance giving a refractive index of 2.53, an absorption coefficient of 404 cm⁻¹ and a root-mean-square surface roughness of 0.6 nm. Advanced modelling of transmittance and Faraday rotation for the PCs (Bi₃Fe₅O₁₂/Sm₃Ga₅O₁₂)⁵ and (TiO₂/Er₂O₃)⁶ was done using the 4 × 4 matrix formalism of Višňovský. The simulations for the constituent materials in the forms of single films were performed using the Swanepoel and Višňovský formulae. This enabled generation of the dispersion relations for diagonal and off-diagonal elements of the permittivity tensors relating to the materials. These dispersion relations were utilised to produce dispersion relations for complex refractive indices of the materials. Integration of the complex refractive indices into the 4 × 4 matrix formalism allowed computation of transmittance and Faraday rotation of the PCs. The simulation results were found to be in a good agreement with the experimental ones proving such a simulation approach is an excellent means of engineering PCs.</p>

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In this thesis, the study of optical properties of magnetic fluid thin films is the main purpose. We measured the intensity of linear polarized laser beam, which passed through our sample, magnetic fluid thin film with external magnetism, to analyze the relationships between magnetic field intensity and magneto-birefringence and magneto-dichroism. According to our experimental results, we ascertain that both the magneto-birefringence and magneto-dichroism are existed. Besides, we found that the difference of index at magnetic fluid thin film changed with magnetic field intensity also. The phenomenon let us believe that magnetic fluid thin film is anisotropy. Moreover, we also applied the statement, which agreed by most physicists to explain what we found from our real measurements.

This work is comprised of the study of two magneto-optical phenomena: the Kerr effect and the Faraday effect. Neutron physics experiments often utilize polarized neutrons, and one method to generate or guide polarized neutrons involves the use of a system of magnetic super-mirrors. Experience shows that the magnetization of the super-mirror may decay with time; therefore, we implemented the surface magneto-optical Kerr effect (SMOKE) to study the temporal behavior of the magnetization of a magnetized remnant super-mirror sample, where a sensitivity of 0.1 mrad was obtained. Unique to our set-up was the method in which the various magnetization directions were probed. The sample was magnetized prior to insertion into the set-up, and a high precision rotational stage was used to manually rotate the sample to effectively generate a reversal of the magnetic field. Multiple samples from a larger super-mirror specimen were tested, in which no change in the magnetization was detected for one month after sample magnetization. Further studies could increase the sensitivity of the experiment, potentially rendering the method as an application for real-time magnetization monitoring. Polarized 3He nuclei are often used as an effective polarized neutron target at various laboratories, including Jefferson Lab, through the use of spin-exchange optical pumping in a glass cell constructed of GE-180. Utilizing the nuclear spin optical rotation to measure the Faraday effect of polarized 3He would develop a new procedure for polarization monitoring, establish a powerful tool to diagnose the wall properties and thicknesses of the cells used, and the determination of the frequency independent magnetic component of the polarizability would ultimately lead to the extraction of the spin polarizability of 3He. Furthermore, this study has the future implications of being the pioneer experiment for terrestrial dark matter studies. A new triple modulation technique was devised, where a sensitivity of 60 nrad was obtained, and the first ever extraction of the Verdet constant of GE-180 was recorded, an important factor in wall thicknesses and diagnostic investigations for Jefferson Lab. However, a measurement of the nuclear spin optical rotation of a polarized 3He target was not realized, as the measured polarization suggests a Faraday rotation just below the 60 nrad threshold. Nevertheless, the devised triple modulation method proves to be a very sensitive probe in Faraday effect studies, and additional examination of the polarized target for the production of a larger polarization, should yield a measurement of the nuclear spin optical rotation of polarized 3He.

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