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Mixed-linker approach in designing porous zirconium-based metal–organic frameworks with high hydrogen storage capacityNaeem, Ayesha, Ting, V.P., Hintermair, U., Tian, M., Telford, Richard, Halim, Saaiba, Nowell, H., Holynska, M., Teat, S.J., Scowen, Ian J., Nayak, Sanjit 17 May 2016 (has links)
Yes / Three highly porous Zr(IV)-based metal–organic frameworks, UBMOF-8, UBMOF-9, and UBMOF-31, were synthesized by using 2,2′-diamino-4,4′-stilbenedicarboxylic acid, 4,4′-stilbenedicarboxylic acid, and combination of both linkers, respectively. The mixed-linker UBMOF-31 showed excellent hydrogen uptake of 4.9 wt% and high selectivity for adsorption of CO2 over N2 with high thermal stability and moderate water stability with permanent porosity and surface area of 2552 m2 g−1. / University of Bath; Royal Society of Chemistry; Engineering and Physical Sciences Research Council
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