Nonlinear optics has had extensive application into a vast array of scientific fields. One such nonlinear process, two-photon absorption (TPA), has had a wildly successful adoption into the field of biological imaging and microscopy. As far and as fast as this field is progressing, limitations stemming from the use of ultrafast lasers are starting to appear. In this work, an alternative nonclassical light source will be motivated for the application of low photon-flux two-photon microscopy. The origin and properties of the chosen nonclassical source, spontaneous parametric downconversion (SPDC), will be discussed along with the spatial and spectral properties modelled. Nonlinear processes such as TPA and sum frequency generation (SFG) will be viewed as "ultrafast coincidence measurements" of two photons arriving at a molecule within the time window of excitation. These ultrafast coincidence measurements will be viewed in an alternative manner: in terms of the second-order coherence from a light source. This degree of second-order coherence can be subdivided into two categories arising from different combinations of correlations within and between entangled photon pairs. Of interest, the energy-time correlations within the photon pair allow for enhancements in ultrafast coincidence rates over coherent light sources. The makings of an experimental setup to demonstrate enhanced rates from ultrafast two-photon coincidences taking place in SFG in a nonlinear crystal will be discussed.

This thesis details two experimental tests that can be applied to particular quantum states to reveal important information. We begin by discussing the relevant background in quantum information. We introduce qubits and qudits as basic quantum states, and we discuss the evolution and measurement of quantum states. We then discuss quantum state tomography as a means by which to obtain complete information about a state, followed by a discussion of state discrimination as a means by which to determine the state given the promise that it is drawn from some known set. We then discuss relevant experimental techniques in quantum optics, including measurement, generation of entanglement, and generation of single photons from entanglement. The first experiment we discuss deals with the causal structure of a system, which is the description of the origin of correlations between two or more states. The causal structure can be direct-cause, meaning that one state causes the other; common-cause, meaning that both states are caused by another; or hybrid-cause, which is a combination of the two. We perform the first implementation of a new type of tomography to determine the causal structure; this is called causal tomography and functions regardless of whether two qubits are related by a common state, a process, or some combination thereof. We implement a process on two entangled photons so that we can select the exact causal structure that results, which ranges continuously between direct-cause and common-cause structures. Using causal tomography, we recover causal structures that closely match expected results and demonstrate that quantum mechanics provides an advantage in causal inference. The second experiment we discuss deals with the unambiguous discrimination of multiple quantum states. For the first time, we apply the principles of unambiguous state discrimination to high-dimensional systems. Given a state chosen randomly out of d possible states encoded in d dimensions, we implement a procedure for determining which state was chosen; this procedure in theory functions without error. We encode and detect the states in the orbital angular momentum degree of freedom up to dimension d=14. Although no experiment can provide perfectly error-free measurement due to inevitable imperfections, we obtain an error rate below the theoretical error rate of minimum-error state discrimination for dimensions up to d=12. At the time of submission of this thesis, this work has been accepted for publication in Physical Review Letters.

Quantum key-distribution (QKD) is a scheme for establishing shared secret key between remote parties. In such a scheme, quantum preparation and measurement devices (sources and detectors) are used. In existing theoretical treatments of QKD, the device models used do not capture all the imperfections which might occur in realistic devices. This creates a gap between the practical implementations and theoretical descriptions of QKD. In the present work, we contribute in bridging this gap by three methods: 1) Advancing the study of squashing models of measurement devices, 2) Devising an alternative to squashing models using statistical estimation in optical QKD, and 3) Modifying the security proof formalism of QKD to account for imperfect devices.

In this thesis, we develop a number of operational tests and tools for benchmarking the quantum nature of optical quantum communication devices. Using the laws of quantum physics, ideal quantum devices can fundamentally outperform their classical counterparts, or even achieve objectives which are classically impossible. Actual devices will not be ideal, but they may still be capable of facilitating quantum communication. Benchmarking tests, based on the presence of entanglement, can be used to verify whether or not imperfect quantum devices offer any advantage over their classical analogs. The general goal in this thesis is to provide strong benchmarking tools which simultaneously require minimal experimental resources but also offer a wide range of applicability. Another major component is the extension of existing qualitative benchmarks (`Is it quantum or classical?') to more quantitative forms (`How quantum is it?'). We provide a number of benchmarking results applicable to two main situations, namely discrete remote state preparation protocols and continuous-variable quantum device testing. The theoretical tools derived throughout this thesis are also applied to the tasks of certifying a remote state preparation experiment and a continuous-variable quantum memory.

No description available.

Quantum information science has shown that computers which exploit the quantum nature of particles, namely quantum computers, can outperform contemporary computers in some computational tasks. The fundamental building blocks of a quantum computer are quantum logical gates and quantum bits (qubits). Previous research has shown that the optical approach to quantum computing is promising. However, linear optical quantum computing (LOQC) schemes require a huge amount of resource, which makes large scale LOQC impractical, and hence there have been renewed interests in nonlinear optical quantum computing schemes, where less resource is required. The performance of these quantum gates depends on the properties of the nonlinear media. However, requirements on some of the properties for high performance quantum gates are not fully known. This thesis intends to bridge this gap of knowledge and examines the necessary conditions on several types optical nonlinearities that are common in two-qubit quantum gates schemes. These types of nonlinearities are, namely two-photon absorption, $\chi^{(2)}$ nonlinearity and $\chi^{(3)}$ cross-Kerr nonlinearity. The two-photon absorption based quantum Zeno gate is modeled in this thesis. It is shown that for practical absorbers, the photon loss significantly lowers the quantum fidelity of the Zeno gate. Nevertheless, this thesis proposes to use the Zeno gate for fusing optical cluster states. With the best theoretical estimate of single photon loss in the absorbers, the Zeno gate can outperform linear optical schemes. This thesis also proposes to embed the Zeno gate in the teleportation-type of two-qubit gate, namely GC-Zeno gate, such that the success rate of the gate can be traded off for higher gate fidelity. The effect of some mode matching error and detector inefficiency on the GC-Zeno gate are also considered here. It is shown that the photon loss requirement as well as the mode matching requirement are both stringent for having a fault tolerant GC-Zeno gate. This thesis models some of the properties of a $\chi^{(3)}$ optical medium and explores how they affect the fidelity of the cross-Kerr nonlinearity based quantum gate. This thesis shows that for a cross-Kerr medium with fast time response but negligible wave dispersion, the medium would induce spectral entanglement between the input photons and this significantly lowers the fidelity of the quantum gate. Nevertheless, when the dispersion has a stronger effect than the time response, and if phase noise is negligible, it is possible to achieve a quantum gate with high fidelity. However, the noise is actually significant, and this thesis suggests that spectral filtering can be applied to prohibit the occurrence of the noise. The requirements on employing optical $\chi^{(2)}$ nonlinearity for quantum computing are also examined. This study models the spectral effects of a $\chi^{(2)}$ medium on its efficiency. It is shown in this thesis that since the Hamiltonian of the medium does not commute at different times, the unitary operation should be modeled by a Dyson series, which leads to undesired spectral entanglement that lowers the efficiency of the medium. However, in the case of periodical poling, the unitary operation can be modeled by a Taylor series, where under some phase matching conditions, the medium can have a high efficiency. Furthermore, this thesis proposes a Bell measurement scheme and a quantum gate scheme based on $\chi^{(2)}$ nonlinearity that can always outperform linear optics even when the nonlinearity strength is weak. In the case of sufficiently strong nonlinearity, a quantum gate with high success rate can be achieved. In summary, this thesis models some of the properties of two-photon absorbers, $\chi^{(2)}$ nonlinearity and $\chi^{(3)}$ nonlinearity, and shows that it is possible to achieve the conditions required for high performance quantum gates, however these conditions are experimentally challenging to meet.

Quantum information science has shown that computers which exploit the quantum nature of particles, namely quantum computers, can outperform contemporary computers in some computational tasks. The fundamental building blocks of a quantum computer are quantum logical gates and quantum bits (qubits). Previous research has shown that the optical approach to quantum computing is promising. However, linear optical quantum computing (LOQC) schemes require a huge amount of resource, which makes large scale LOQC impractical, and hence there have been renewed interests in nonlinear optical quantum computing schemes, where less resource is required. The performance of these quantum gates depends on the properties of the nonlinear media. However, requirements on some of the properties for high performance quantum gates are not fully known. This thesis intends to bridge this gap of knowledge and examines the necessary conditions on several types optical nonlinearities that are common in two-qubit quantum gates schemes. These types of nonlinearities are, namely two-photon absorption, $\chi^{(2)}$ nonlinearity and $\chi^{(3)}$ cross-Kerr nonlinearity. The two-photon absorption based quantum Zeno gate is modeled in this thesis. It is shown that for practical absorbers, the photon loss significantly lowers the quantum fidelity of the Zeno gate. Nevertheless, this thesis proposes to use the Zeno gate for fusing optical cluster states. With the best theoretical estimate of single photon loss in the absorbers, the Zeno gate can outperform linear optical schemes. This thesis also proposes to embed the Zeno gate in the teleportation-type of two-qubit gate, namely GC-Zeno gate, such that the success rate of the gate can be traded off for higher gate fidelity. The effect of some mode matching error and detector inefficiency on the GC-Zeno gate are also considered here. It is shown that the photon loss requirement as well as the mode matching requirement are both stringent for having a fault tolerant GC-Zeno gate. This thesis models some of the properties of a $\chi^{(3)}$ optical medium and explores how they affect the fidelity of the cross-Kerr nonlinearity based quantum gate. This thesis shows that for a cross-Kerr medium with fast time response but negligible wave dispersion, the medium would induce spectral entanglement between the input photons and this significantly lowers the fidelity of the quantum gate. Nevertheless, when the dispersion has a stronger effect than the time response, and if phase noise is negligible, it is possible to achieve a quantum gate with high fidelity. However, the noise is actually significant, and this thesis suggests that spectral filtering can be applied to prohibit the occurrence of the noise. The requirements on employing optical $\chi^{(2)}$ nonlinearity for quantum computing are also examined. This study models the spectral effects of a $\chi^{(2)}$ medium on its efficiency. It is shown in this thesis that since the Hamiltonian of the medium does not commute at different times, the unitary operation should be modeled by a Dyson series, which leads to undesired spectral entanglement that lowers the efficiency of the medium. However, in the case of periodical poling, the unitary operation can be modeled by a Taylor series, where under some phase matching conditions, the medium can have a high efficiency. Furthermore, this thesis proposes a Bell measurement scheme and a quantum gate scheme based on $\chi^{(2)}$ nonlinearity that can always outperform linear optics even when the nonlinearity strength is weak. In the case of sufficiently strong nonlinearity, a quantum gate with high success rate can be achieved. In summary, this thesis models some of the properties of two-photon absorbers, $\chi^{(2)}$ nonlinearity and $\chi^{(3)}$ nonlinearity, and shows that it is possible to achieve the conditions required for high performance quantum gates, however these conditions are experimentally challenging to meet.

Thesis (Ph. D.)--University of Oregon, 2007. / Typescript. Includes vita and abstract. Includes bibliographical references (leaves 251-264). Also available for download via the World Wide Web; free to University of Oregon users.

Thesis (Ph. D.)--University of Texas at Austin, 2008. / Vita. Includes bibliographical references.

Thesis (Ph. D.)--University of Oregon, 1999. / Typescript. Includes vita and abstract. Includes bibliographical references (leaves 197-201). Also available for download via the World Wide Web; free to University of Oregon users. Address: http://wwwlib.umi.com/cr/uoregon/fullcit?p9948024.