Electrons not only have charges but also have spin. By utilizing the electron spin, the energy consumption of electronic devices can be reduced, their size can be scaled down and the efficiency of `read' and `write' in memory devices can be significantly improved. Hence, the manipulation of electron spin in electronic devices becomes more and more appealing for the advancement of microelectronics. In spin-based devices, the manipulation of ferromagnetic order parameter using electrical currents is a very useful means for current-driven operation. Nowadays, most of magnetic memory devices are based on the so-called spin transfer torque, which stems from the spin angular momentum transfer between a spin-polarized current and the magnetic order parameter. Recently, a novel spin torque effect, exploiting spin-orbit coupling in non-centrosymmetric magnets, has attracted a massive amount of attention. This thesis addresses the nature of spin-orbit coupled transport and torques in non-centrosymmetric magnetic semiconductors. We start with the theoretical study of spin orbit torque in three dimensional ferromagnetic GaMnAs. Using the Kubo formula, we calculate both the current-driven field-like torque and anti-damping-like torque. We compare the numerical results with the analytical expressions in the model case of a magnetic Rashba two-dimensional electron gas. Parametric dependencies of the different torque components and similarities to the analytical results of the Rashba two-dimensional electron gas in the weak disorder limit are described. Subsequently we study spin-orbit torques in two dimensional hexagonal crystals such as graphene, silicene, germanene and stanene. In the presence of staggered potential and exchange field, the valley degeneracy can be lifted and we obtain a valley-dependent Berry curvature, leading to a tunable antidamping torque by controlling the valley degree of freedom. This thesis then addresses the influence of the quantum spin Hall effect on spin orbit torque in nanoribbons with a hexagonal lattice. We find a dramatic modification of the nature of the torque (field like and damping-like component) when crossing the topological phase transition. The relative agnitude of the two torque components can be significantly modifies by changing the magnetization direction. Finally, motivated by recent experimental results, we conclude by investigating the features of spin-orbit torque in magnetic transition metal dichalcogenides. We find the torque is associated with the valley polarization. By changing the magnetization direction, the torque can be changed from a finite value to zero when the valley polarization decreases from a finite value to zero.

Thesis advisor: Vidya Madhavan / We present Scanning Tunneling Microscopy (STM) studies on several systems in which spin-orbit coupling leads to new and interesting physics, and where tuning by doping and/or strain can significantly modify the electronic properties, either inducing a phase transition or by sharply influencing the electronic structure locally. In the perovskite Iridate insulator Sr3Ir2O7, we investigate the parent compound, determining the band gap and its evolution in response to point defects which we identify as apical oxygen vacancies. We investigate the effects of doping the parent compound with La (in place of Sr) and Ru (in place of Ir). In both cases a metal-insulator transition (MIT) results: at x ~ 38% with Ru, and x ~ 5% with La. In the La-doped samples we find nanoscale phase separation at dopings just below the MIT, with metallic spectra associated with clusters of La atoms. Further, we find resonances near the Fermi energy associated with individual La atoms, suggesting an uneven distribution of dopants among the layers of the parent compound. Bi2Se3 is a topological insulator which hosts linearly dispersing Dirac surface states. Doping with In (in place of Bismuth) brings about topological phase transition, achieving a trivial insulator at x ~ 4%. We use high-magnetic field Landau level spectroscopy to study the surface state’s properties approaching the phase transition and find, by a careful analysis of the peak positions find behavior consistent with strong surface-state Zeeman effects: g~50. This interpretation implies, however, a relabeling of the Landau levels previously observed in pristine Bi2Se3, which we justify through ab initio calculations. The overall picture is of a g-factor which steadily decreases as In is added up to the topological phase transition. Finally, we examine the effects of strain on the surface states of (001) thin films of the topological crystalline insulator SnTe. When these films are grown on closely-related substrates—in this case PbSe(001)—a rich pattern of surface strain emerges. We use phase-sensitive analysis of atomic-resolution STM topographs to measure the strain locally, and spatially-resolved quasiparticle interference imaging to compare the Dirac point positions in regions with different types of strain, quantifying for the first time the effect of anisotropic strain on the surface states of a topological crystalline insulator. / Thesis (PhD) — Boston College, 2016. / Submitted to: Boston College. Graduate School of Arts and Sciences. / Discipline: Physics.

The existence of the exact commensurability between the periods of rotation and revolution of a satellite orbiting a planet is not a rare phenomenon in the Solar system. In fact, there are several examples of such resonances with the Earth-Moon system being the most familiar example of a 1:1 (synchronous) resonance. In this report, I will discuss the questions of stability of five resonant systems (Moon – Earth, Enceladus - Saturn, Dione - Saturn, Rhea – Saturn, and Mercury – Sun (the only non – synchronous resonance among the evolved spin – orbit resonances in the Solar system). Several authors have investigated the stability of spin-orbit resonances, and, in this report, I will concentrate on the two most recent investigations. / text

A derivation of the elastic scattering differential cross section, within a three-body eikonal model, that treats both central and spin-orbit interactions between the constituent projectile clusters and the target is presented. This formalism is then used in the theoretical study of the scattering of 8B from 12C at 40 MeV/nucleon. The proton halo candidate, 8B, is taken to consist of a single valence proton orbiting a 7Be core cluster. Calculation of the elastic scattering amplitude relies upon determining the phase shifts caused as the projectile passes through the region of interaction with the target. A form for the orbital angular momentum operator of each projectile cluster about the target is obtained that allows a relatively simple form for the spin-orbit phase shift functions, analogous to those for the central interactions, to be deduced. The study of the angular distribution of the elastic scattering differential cross section is carried out in two parts. Initially the effect of elastic break-up and recombination of the projectile during the scattering process, only taking into account central interactions, is studied. To gauge the magnitude of these effects, within the three-body model, the elastic scattering differential cross section, in the limit of no projectile break-up, is derived. Despite the very small binding energy of 8B it is shown that these effects are quite small. It is also shown, however, that these effects become more conspicuous as the valence proton becomes less localised about the core. Finally the effect of including spin-orbit interactions is studied. In the system under study these effects are shown to have an almost negligible effect on the angular distribution of the differential cross section. However, increasing the projectile kinetic energy to the region of hundreds of MeV/nucleon is seen to increase their significance. Future calculations hope to look at the angular distribution of the elastic scattering differential cross section and vector and tensor analysing powers of polarised beams of deuterons as these systems are expected to show more sensitivity to spin- orbit interactions. Furthermore, with the possibility of polarised beams of halo nuclei, the three-body Glauber model would be an ideal theoretical tool with which to study certain of their spin-related phenomena too.

Since the discovery of giant magnetoresistance in 1980s, Spintronics became an exciting field which studies numerous phenomena including the spin transport in magnetic heterostructures, magnetization dynamics and the interplay between them. I have investigated different topics during my graduate research. In this dissertation, I summarize all my projects including spin pumping, spin convertance and spin injection into ballistic medium. First, we develop a linear response formalism for spin pumping effect. Spin pumping refers that a precessing emits a spin current into its adjacent nonmagnetic surroundings, which was originally proposed using scattering theory. The newly developed formalism is demonstrated to be identical the early theory in limiting case. While our formalism is convenient to include the effects of disorders and spin-orbit coupling which can resolve the quantitative controversies between early theory and experiments. Second, the spin pumping experiments indicates a much smaller spin Hall angle compared with the results obtained via the spin transfer torque measurements. We found that such issues can be resolved when taking into consideration the effects of non-local conductivity. And we conclude neither of the two methods measures the real spin Hall angle while the spin pumping methods provides much accurate estimations. Third, we developed the spin transport equations in weak scattering medium in the presence of spin-orbit coupling. Before this, all spin dependent electron transport has been modeled by the conventional spin diffusion equation. While recent spin injection experiments have seen the failure of spin diffusion equation. As the experimental fitting using spin diffusion models led to unrealistic conclusions. At last, we study the spin convertance in anti-ferromagnetic multilayers, where the spin information can be mutually transferred between ferromagnetic/anti-ferromagnetic and conduction electrons. Our theory successfully explained the experiment results that the insertion of thin NiO film between YIG/Pt largely enhances the spin Seebeck currents.

In the present thesis we introduce the reader to the field of spintronics and explore new phenomena, such as spin transfer torques, spin filtering, and three types of spin-orbit torques, Rashba, spin Hall, and spin swapping, which have emerged very recently and are promising candidates for a new generation of memory devices in computer technology. A general overview of these phenomena is presented in Chap. 1. In Chap. 2 we study spin transfer torques in tunnel junctions in the presence of spin filtering. In Chap. 3 we discuss the Rashba torque in ferromagnetic films, and in Chap. 4 we study spin Hall effect and spin swapping in ferromagnetic films, exploring the nature of spin-orbit torques based on these mechanisms. Conclusions and perspectives are summarized in Chap. 5.

No description available.

This thesis uses ferromagnetic resonance to explore the current-induced torques (CITs) in two different systems, namely YIG/heavy metal bilayers and bulk NiMnSb, at room temperature. We apply a microwave current to the sample while sweeping the external magnetic field, and measure the longitudinal DC voltage. From a symmetry analysis of the ferromagnetic resonance lineshape, the amplitudes and directions of the CITs parameterised by an effective magnetic field are accurately estimated. In Chapter 4, YIG samples of different thickness, capped by either Pt or Ta, are studied. The resonance is driven by both spin-transfer torque and Oersted field, and the DC voltage is attributed to both spin rectification and spin pumping. The CITs can be well analysed from the lineshape of the voltage and its dependence on YIG thickness, from which we deduce that the Oersted field dominates over the spin-transfer torque in driving magnetization dynamics. In Chapter 5, we characterise the CITs in bulk NiMnSb induced by the relativistic spin-orbit coupling effect. Both field-like and antidamping-like spin-orbit torques are observed and analysed in detail. At the end of this chapter, we study the spin-wave resonance driven by the CITs, from which the exchange stiffness of NiMnSb is determined. In Chapter 6, we extrapolate a new form of magnetoresistance in NiMnSb: unidirectional spin-orbit magnetoresistance (USOMR). USOMR scales linearly with the current and has opposite sign when the magnetization is reversed. Similar to the giant magnetoresistance in magnetic multilayers, USOMR can be used to distinguish between two opposite magnetization directions directly in the bulk of the ferromagnet.

<p>The spin of an electron often misleadingly interpreted as the classical rotationof a particle. The quantum spin distinguishes itself from classicalrotation by possessing quantized states and can be detected by its magneticmoment. The properties of spin and its collective behavior with otherfundamental properties are fascinating in basic sciences. In many aspectsit offers scope for designing new materials by manipulating the ensemblesof spin. In recent years attention towards high density storage devices hasdriven the attention to the fundamental level were quantum physics rules.To understand better design of molecule based storage materials, studies onspin degrees of freedom and their coupling properties can not be neglected.</p><p>To account for many body effect of two or more electrons consistent withrelativity, an approximation like the Breit Hamiltonian(BH) is used in modernquantum chemical calculations, which is successful in explaining the splitin the spectra and corresponding properties associated with it. Often differenttactics are involved for a specific level of computations. For example themulti-configurational practice is different from the functional based calculations,and it depends on the size of the system to choose between resourcesand accuracy. As the coupling terms offers extra burden of calculating theintegrals it is literally challenging.</p><p>One can readily employ approximations as it suits best for the applicationoriented device computations. The possible methods available in the literatureare presented in chapter 2. The theoretical implementations of couplingfor the multi-reference and density functional method are discussed in detail.The multi-reference method precedes the density functional methodin terms of accuracy and generalizations, however it is inefficient in dealingvery large systems involving many transition elements, which is vital formolecule based magnets as they often possess open shell manifolds. On theother hand existing density functional method exercise perturbations techniqueswhich is extremely specialized for a specific system - highly coupledspins.</p><p>The importance of spin-spin coupling(SSC) in organic radical-Oxyallyl(OXA)was systematically studied with different basis sets and compared with asimilar isoelectronic radical(TMM). The method of spin-spin coupling implementationsare also emphasized. Similar coupling studies were carriedivout for the species HCP and NCN along with spin-orbit coupling(SOC).The splitting of the triplet states are in good agreement with experiments</p>

This thesis analyses the effect spin-orbit coupling has on the dispersion of Langmuir waves in magnetized plasmas, using recently developed kinetic theories of plasmas including quantummechanical and relativistic effects. Two new wave modes appearclose to the resonance <img src="http://www.diva-portal.org/cgi-bin/mimetex.cgi?%5CDelta%20%5Comega_%7Bc%7D" /> = ( g/2 − 1)<img src="http://www.diva-portal.org/cgi-bin/mimetex.cgi?%5Comega_%7Bc%7D" /> , where <img src="http://www.diva-portal.org/cgi-bin/mimetex.cgi?%5Comega_%7Bc%7D" /> is the cyclotron frequency and g is the electron gyromagnetic ratio. Forconsidered long wave lengths the deviation from this resonanceis very small. The wave modes are also very weakly damped.