Diffractive optical elements (DOEs) serve an important function in many dynamic and static optical systems. The theory and design of surface diffractive structures are well understood and practically applied at high spatial and phase resolution for a wide range of optical applications in science and industry. However, these structures normally only harness phase modulation of uniform fields for the beam diffraction and therefore limit their range of application, as well as being susceptible to surface damage. Multilayered volume diffractive elements offer a powerful opportunity to harness both phase and amplitude modulation for benefits in diffraction efficiency and beam shaping. However, multilayered combinations have been difficult to fabricate and provide only weak diffraction for phase gratings with low refractive index contrast. The advent of femtosecond laser writing inside transparent media has enabled the facile embedding of optical devices such as waveguides and diffractive optics into novel three-dimensional geometries that offer advanced functionality with compact design. In this work, femtosecond laser writing is pushed to the limits of forming high resolution phase elements with sufficiently strong refractive index contrast on which to develop volume phase gratings with the highest diffractive efficiency. The formation of both positive and negative zones of refractive index contrast together with rapid Talbot self imaging inside weakly contrasting phase gratings are major challenges here diminish the efficiency of assembled gratings. A method of strategic layering of otherwise weakly diffracting gratings onto Talbot planes is introduced to demonstrate, in FDTD models, the definitive enhancement of overall diffraction efficiency. A systematic optimization of laser writing in fused silica verify this enhancement or diminishment with weak volume gratings assembled on aligned or misaligned on Talbot planes. Advanced laser beam control methods were further demonstrated that underpin new direction for the facile assembly of highly functional DOEs that can exploit coherent light diffraction for opportunities in improving the performance of holographic devices and extend further to the powerful combination of phase and amplitude modulation control that is potentially available in a single optical device, thereby opening new directions for the design and fabrication of robust and strongly diffracting volume optical devices.

Diffractive optical elements (DOEs) serve an important function in many dynamic and static optical systems. The theory and design of surface diffractive structures are well understood and practically applied at high spatial and phase resolution for a wide range of optical applications in science and industry. However, these structures normally only harness phase modulation of uniform fields for the beam diffraction and therefore limit their range of application, as well as being susceptible to surface damage. Multilayered volume diffractive elements offer a powerful opportunity to harness both phase and amplitude modulation for benefits in diffraction efficiency and beam shaping. However, multilayered combinations have been difficult to fabricate and provide only weak diffraction for phase gratings with low refractive index contrast. The advent of femtosecond laser writing inside transparent media has enabled the facile embedding of optical devices such as waveguides and diffractive optics into novel three-dimensional geometries that offer advanced functionality with compact design. In this work, femtosecond laser writing is pushed to the limits of forming high resolution phase elements with sufficiently strong refractive index contrast on which to develop volume phase gratings with the highest diffractive efficiency. The formation of both positive and negative zones of refractive index contrast together with rapid Talbot self imaging inside weakly contrasting phase gratings are major challenges here diminish the efficiency of assembled gratings. A method of strategic layering of otherwise weakly diffracting gratings onto Talbot planes is introduced to demonstrate, in FDTD models, the definitive enhancement of overall diffraction efficiency. A systematic optimization of laser writing in fused silica verify this enhancement or diminishment with weak volume gratings assembled on aligned or misaligned on Talbot planes. Advanced laser beam control methods were further demonstrated that underpin new direction for the facile assembly of highly functional DOEs that can exploit coherent light diffraction for opportunities in improving the performance of holographic devices and extend further to the powerful combination of phase and amplitude modulation control that is potentially available in a single optical device, thereby opening new directions for the design and fabrication of robust and strongly diffracting volume optical devices.