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  • About
  • The Global ETD Search service is a free service for researchers to find electronic theses and dissertations. This service is provided by the Networked Digital Library of Theses and Dissertations.
    Our metadata is collected from universities around the world. If you manage a university/consortium/country archive and want to be added, details can be found on the NDLTD website.
1

The Absolute Yields of Xenon and Krypton in U 238 Spontaneous Fission

Young, Beverly George 10 1900 (has links)
The absolute abundances of fission-product xenon and krypton isotopes in six uranium minerals were determined mass spectrometrically using the isotope dilution technique. The fission products were resolved into a U spontaneous fission component, a U 235 neutron-induced fission component, and a U 238 neutron-induced fission component. The presence of U 238 of neutron-induced fission indicated that t he neutron energies in uranium minerals were higher than had been suspected. Internal consistency in the analysis was achieved only when the I 29 yield in u235 thermal neutron fission reported by Purkayastha and Martin was lowered by 20%. The number of U 238 spontaneous fissions was calculated from the lead age, U 238 content, and the U 238 pontaneous fission half life. A comparison of the number of fission products from U 238 spontaneous fission and the number of spontaneous fissions in each of the six minerals showed that five of the six minerals had lost large portions of their noble gases. A fractionation of krypton relative to xenon accompanied this loss. The results obtained for the sixth mineral indicated little or no loss of xenon and krypton. Absolute yields for U 238 spontaneous fission were therefore determined from an analysis of this mineral. / Thesis / Doctor of Philosophy (PhD)

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