It is widely accepted that the continued increase of processor performance requires at least partial replacement of electronic interconnects with their photonic counterparts. The implementation of optical interconnects requires the realization of a silicon-based light source, which is challenging task due to the low emission efficiency of silicon. One of the main approaches to address this challenge is the use of doping of silicon based matrices with optical centers, including erbium ions. Erbium ions incorporated in various hosts assume the trivalent state (Er3+) and demonstrate a transition at 1.54 μm, coinciding with optical transmission windows in both silicon and silica. Due to the low absorption cross-section and discrete energy levels of the Er3+ ion, indirect excitation is necessary. In late 90s it was demonstrated that the incorporation of excess silicon in erbium-doped silica results in strong erbium sensitization, leading to an increase of the effective absorption cross-section by orders of magnitude. The sensitization was considered to occur via silicon nanocrystals that formed at high annealing temperatures. While a large increase of the absorption cross-section was demonstrated, the incorporation of Si nanocrystals was found to result in a low concentration of excited erbium, as well as silicon related free-carrier absorption. The focus of this dissertation is the investigation of the nature of the sensitization mechanism of erbium in silicon-rich silica. The results presented in the dissertation demonstrate that erbium in silicon-rich silica is predominantly excited by silicon-excess-related luminescence centers, as opposed to the commonly considered silicon nanocrystals. This is a remarkable conclusion that changes the view on the exact origin of erbium sensitization, and that resolves several technical challenges that exist for nanocrystal-based sensitization. The work shows that the density of indirectly excited erbium ions is significantly larger in samples without silicon iii nanocrystals (annealed at T < 1000°C) as opposed to samples with silicon nanocrystals (annealed at T > 1000°C). The density of indirectly excited erbium ions, defining the maximum achievable gain, was demonstrated to be approximately excitation wavelength independent, while the effective erbium absorption cross-section was shown to significantly depend on the excitation wavelength. The excitation mechanism of erbium by luminescence centers was shown to be fast ( < 30 ns) and capable of erbium sensitization to different energy levels. This multilevel nature of erbium excitation was demonstrated to result in two different mechanisms of the excitation of the first excited state of erbium: fast ( < 30 ns) direct excitation by the luminescence centers, and slow ( > 2.3 μs) excitation due to the relaxation of erbium ions excited into higher energy levels to the first excited state. Based on photoluminescence studies conducted in the temperature range 15 - 300K it was shown that the relaxation efficiency of erbium from the second excited state to the first excited state (responsible for the slow excitation mechanism) is temperature independent and approaches unity. The relative stability of the optical properties demonstrated in the temperature range 20 - 200°C, implies that relatively stable optical gain can be achieved under realistic on-chip operating conditions. The optimum Si excess concentration corresponding to the highest density of sensitized Er3+ ions is shown to be relatively insensitive to the presence of Si nanocrystals and is ~ 14.5 at.% and ~ 11.5 at.% for samples without and with Si nanocrystals respectively. The presented results and conclusions have significant implications for silicon photonics and the industrial application of Er doped SiO2. The work shows that in order to sensitize erbium ions in silicon-rich silica there is no need for the presence of silicon nanocrystals, and consequently lower fabrication temperatures can be used. More importantly, the results strongly iv suggest that higher gain values can be acquired in samples annealed at lower temperature (without silicon nanocrystals) as compared to samples annealed at high temperatures (with silicon nanocrystals). In addition, the maximum gain is predicted to be relatively independent of excitation wavelength, significantly relaxing the requirements on the pump source. Based on the experimental results it is predicted that relatively stable performance of erbium-doped siliconrich silica is possible up to typical processor operating temperatures of ~ 80 - 90°C making it a viable material for on-chip devices. The results suggest that low temperature annealed erbiumdoped silicon-rich silica is a preferable material for on-chip photonic devices as compared with its high temperature annealed counterpart.

Microvasculature can be found in almost every part of the human body, including the internal organs. Importantly, abnormal changes in microvasculature are usually related to pathological development of the tissue cells. Monitoring of changes in blood flow properties in microvasculature, therefore, provides useful diagnostic information about pathological conditions in biological tissues as exemplified in glaucoma, diabetes, age related macular degeneration, port wine stains, burn-depth, and potentially skin cancer. However, the capillary network is typically only one cell in wall thickness with 5 to 10 microns in diameter and located in the dermis region of skin. Therefore, a non-invasive flow imaging technique that is capable of depth sectioning at high resolution and high speed is demanded. Optical coherence tomography (OCT), particularly after its advancement in frequency domain OCT (FD-OCT), is a promising tool for non-invasive high speed, high resolution, and high sensitivity depth-resolved imaging of biological tissues. Over the last ten years, numerous efforts have been paid to develop OCTbased flow imaging techniques. An important effort is the development of phase-resolved Doppler OCT (PR-DOCT). Phase-resolved Doppler imaging using FD-OCT is particularly of interest because of the direct access to the phase information of the depth profile signal. Furthermore, the high speed capability of FD-OCT is promising for real time flow monitoring as well as 3D flow segmentation applications. However, several challenges need to be addressed; 1) Flow in biological samples exhibits a wide dynamic range of flow velocity caused by, for example, the iv variation in the flow angles, flow diameters, and functionalities. However, the improvement in imaging speed of FD-OCT comes at the expense of a reduction in sensitivity to slow flow information and hence a reduction in detectable velocity range; 2) A structural ambiguity socalled 'mirror image' in FD-OCT prohibits the use of maximum sensitivity and imaging depth range; 3) The requirement of high lateral resolution to resolve capillary vessels requires the use of an imaging optics with high numerical aperture (NA) that leads to a reduction in depth of focus (DOF) and hence the imaging depth range (i.e. less than 100 microns) unless dynamic focusing is performed. Nevertheless, intrinsic to the mechanism of FD-OCT, dynamic focusing is not possible. In this dissertation, the implementation of PR-DOCT in a high speed swept-source based FD-OCT is investigated and optimized. An acquisition scheme as well as a processing algorithm that effectively extends the detectable velocity dynamic range of the PR-DOCT is presented. The proposed technique increased the overall detectable velocity dynamic range of PR-DOCT by about five times of that achieved by the conventional method. Furthermore, a novel technique of mirror image removal called ‘Dual-Detection FD-OCT’ (DD-FD-OCT) is presented. One of the advantages of DD-FD-OCT to Doppler imaging is that the full-range signal is achieved without manipulation of the phase relation between consecutive axial lines. Hence the full-range DD-FDOCT is fully applicable to phase-resolved Doppler detection without a reduction in detectable velocity dynamic range as normally encountered in other full-range techniques. In addition, PRDOCT can utilize the maximum SNR provided by the full-range capability. This capability is particularly useful for imaging of blood flow that locates deep below the sample surface, such as v blood flow at deep posterior human eye and blood vessels network in the dermis region of human skin. Beside high speed and functional imaging capability, another key parameter that will open path for optical diagnostics using OCT technology is high resolution imaging (i.e. in a regime of a few microns or sub-micron). Even though the lateral resolution of OCT can be independently improved by opening the NA of the imaging optics, the high lateral resolution is maintained only over a short range as limited by the depth of focus that varies inversely and quadratically with NA. Recently developed by our group, ‘Gabor-Domain Optical Coherence Microscopy’ (GD-OCM) is a novel imaging technique capable for invariant resolution of about 2-3 m over a 2 mm cubic field-of-view. This dissertation details the imaging protocol as well as the automatic data fusion method of GD-OCM developed to render an in-focus high-resolution image throughout the imaging depth of the sample in real time. For the application of absolute flow measurement as an example, the precise information about flow angle is required. GDOCM provides more precise interpretation of the tissue structures over a large field-of-view, which is necessary for accurate mapping of the flow structure and hence is promising for diagnostic applications particularly when combined with Doppler imaging. Potentially, the ability to perform high resolution OCT imaging inside the human body is useful for many diagnostic applications, such as providing an accurate map for biopsy, guiding surgical and other treatments, monitoring the functional state and/or the post-operative recovery process of internal organs, plaque detection in arteries, and early detection of cancers in the gastrointestinal tract. Endoscopic OCT utilizes a special miniature probe in the sample arm to vi access tubular organs inside the human body, such as the cardiovascular system, the lung, the gastrointestinal tract, the urinary tract, and the breast duct. We present an optical design of a dynamic focus endoscopic probe that is capable of about 4 to 6 m lateral resolution over a large working distance (i.e. up to 5 mm from the distal end of the probe). The dynamic focus capability allows integration of the endoscopic probe to GD-OCM imaging to achieve high resolution endoscopic tomograms. We envision the future of this developing technology as a solution to high resolution, minimally invasive, depth-resolved imaging of not only structure but also the microvasculature of in vivo biological tissues that will be useful for many clinical applications, such as dermatology, ophthalmology, endoscopy, and cardiology. The technology is also useful for animal study applications, such as the monitoring of an embryo’s heart for the development of animal models and monitoring of changes in blood circulation in response to external stimulus in small animal brains.

Generation and detection of circularly-polarized (CP) radiation in the 8- to 12-μm band of the infrared (IR) spectrum is crucial for polarization sensing and imaging scenarios. There is very little naturally occurring CP radiation in the long-wave IR band, so that useful functionalities may be obtained by exploiting preferential radiation and transmission characteristics of engineered metamaterials. Conventional CP devices in the IR utilize birefringent crystals, which are typically bulky and expensive to manufacture. The operation of these devices is generally optimized at a single wavelength. Imaging in the long-wave IR is most often broadband, so that achromatic CP-device behavior is highly desirable from a fluxtransfer viewpoint. Also, size, weight and cost are significant drivers in the design of practical IR systems. Thus a solution is sought with a convenient thin planar form factor. This dissertation will demonstrate a novel planar periodic subwavelength-microstructured approach derived from classical radiofrequency meanderline designs that are able to generate CP radiation over a broad IR band while maintaining a low fabrication profile. We investigate issues regarding efficiency as a function of the number of layers in the device structure; reflective, transmissive, and emissive behavior; strategies for broadband achromatization; and thermal-isolation requirements between the active blackbody reservoir and the top of the planar device, to achieve a given degree of polarization. Theoretical, numerical, and experimental findings are presented that confirm the feasibility of this class of devices for use in a wide variety of situations, from polarization imaging and spectroscopy to industrial laser processing and machining.

High power lasers with diffraction limited beam quality are desired for many applications in defense and manufacturing. A lot of applications require laser beams at the 100 kW power level along with divergence close to the diffraction limit. The figure of merit for a beam used in such applications should be radiance which determines the laser power delivered to a remote target. One of the primary limiting factors is thermal distortion of a laser beam caused by excessive heat generated in the laser media. Combination of multiple laser beams is usually considered as a method to mitigate these limitations. Spectral beam combining (SBC) by volume Bragg gratings (VBGs) is a very promising method for the future of high radiance lasers that needs to achieve 100 kW-level power. This work is dedicated to development of methods to increase spectral density of combined beams keeping their divergence at an acceptably low level. A new figure of merit for a beam combining system is proposed, the Beam Combining Factor (BCF), which makes it possible to distinguish the quality of the individual beams from the quality of beam combining. Also presented is a method of including the effect of beam divergence and spectral bandwidth on the performance of VBGs, as well as a method to optimize VBG parameters in terms of thickness and refractive index modulation for an arbitrary number of beams. A novel thermal tuning technique and apparatus is presented with which the SBC system can be tuned for peak efficiency from low to high power without the need for mechanical re- iv alignment. Finally, a thermally tuned SBC system with five beams, with a spectral separation between beams of 0.25 nm at a total power of 685 W is presented. The results show the highest power spectral density and highest spectral radiance of any SBC system to date. Recent demonstrations in SBC by multiplexed VBGs and the use of super Gaussian beams for beam quality improvement are also discussed.

The topic of this dissertation is the development of low repetition rate and low noise semiconductor-based laser sources with a focus on linearly chirped pulse laser sources. In the past decade chirped optical pulses have found a plethora of applications such as photonic analogto-digital conversion, optical coherence tomography, laser ranging, etc. This dissertation analyzes the aforementioned applications of linearly chirped pulses and their technical requirements, as well as the performance of previously demonstrated chirped pulse laser sources. Moreover, the focus is shifted to a specific application of the linearly chirped pulses, timestretched photonic analog-to-digital conversion (TS ADC). The challenges of surpassing the speeds of current electronic converters are discussed, while the need for low noise linearly chirped pulse lasers becomes apparent for the realization of TS ADC. The experimental research addresses the topic of low noise chirped pulse generation in three distinct ways. First, a chirped pulse (Theta) laser with an intra-cavity Fabry-Pérot etalon and a long-term referencing mechanism is developed that results in the reduction of the pulse-topulse energy noise. Noise suppression of > 15 times is demonstrated. Moreover, an optical frequency comb with spacing equal to the repetition rate (≈100 MHz) is generated using the etalon, resulting in the first reported demonstration of a system operating in the sub-GHz regime based on semiconductor gain. The path for the development of the Theta laser was laid by the precise characterization of the etalon used in this laser cavity design. A narrow linewidth laser is used in conjunction with an acousto-optic modulator externally swept for measuring the etalon's iv free spectral range with a sub-Hz precision, or 10 parts per billion. Furthermore, the measurement of the etalon long-term drift and birefringence lead to the development of a modified intra-cavity Hänsch-Couillaud locking mechanism for the Theta laser. Moreover, an external feed-forward system was demonstrated that aimed at increasing the temporal/spectral uniformity of the optical pulses. A complete characterization of the system is demonstrated. On a different series of experiments, the pulses emitted by an ultra-low noise but high repetition rate mode-locked laser were demultiplexed resulting in a low repetition rate pulse train. Experimental investigation of the noise properties of the laser proved that they are preserved during the demultiplexing process. The noise of the electrical gate used in this experiment is also investigated which led into the development of a more profound understanding of the electrical noise of periodical pulses and a mechanism of measuring their noise. The appendices in this dissertation provide additional material used for the realization of the main research focus of the dissertation. Measurements of the group delay of the etalon used in the Theta laser are presented in order to demonstrate the limiting factors for the development of this cavity design. The description of a balancing routine is presented, that was used for expanding the dynamic range of intra-cavity active variable delay. At last, the appendix presents the calculations regarding the contribution of various parameters in the limitations of analog-todigital conversion.

Recently optical frequency combs and low noise RF tones are drawing increased attention due to applications in spectroscopy, metrology, arbitrary waveform generation, optical signal processing etc. This thesis focuses on the generation of low noise RF tones and stabilized optical frequency combs. The optical frequency combs are generated by a semiconductor based external cavity mode-locked laser with a high finesse intracavity etalon. In order to get the lowest noise and broadest bandwidth from the mode-locked laser, it is critical to know the free spectral range (FSR) of the etalon precisely. First the etalon FSR is measured by using the modified Pound-Drever-Hall (PDH) based method and obtained a resolution of 1 part in 106 , which is 2 order of magnitude better than the standard PDH based method. After optimizing the cavity length, RF driving frequency and PDH cavity locking point, the mode-locked laser had an integrated timing jitter of 3 fs (1 Hz- 100 MHz) which is, to the best of our knowledge, the lowest jitter ever reported from a semiconductor based multigigahertz comb source. The modelocked laser produces ~ 100 comb lines with 10 GHz spacing, a linewidth of ~500 Hz and 75 dB optical signal-to-noise ratio. The same system can also be driven as a regeneratively modelocked laser with greatly improved noise performance. Another way of generating a low noise RF tone is using an opto-electronic oscillator which uses an optical cavity as a high Q element. Due to the harmonic nature of OEOs, a mode selection element is necessary. Standard OEOs use an RF filter having drawbacks such as broad pass band, high loss, and high thermal noise. In our work, a novel optoelectronic scheme which uses an optical filter (Fabry-Perot etalon) as the mode filter instead of an RF filter is demonstrated. This method has the advantage of having ultra-narrow filtering bandwidths ( ~ 10 iv kHz for a 10 GHz FSR and 106 finesse) and an extremely low noise RF signal. Experimental demonstration of the proposed method resulted in a 5-10 dB decrease of the OEO noise compared to the conventional OEO setup. Also, by modifying the etalon-based OEO, and using single side band modulation, an optically tunable optoelectronic oscillator is achieved with 10-20 dB lower noise than dual side band modulation. Noise properties of the OEO as a function of optical frequency detuning is also analyzed theoretically and the results are in agreement with experimental results. The thesis concludes with comments on future work and directions.

Infrared (IR) dipole antenna-coupled metal-oxide-metal (MOM) tunnel diodes provide a unique detection mechanism that allows for determination of the polarization and wavelength of an optical field. By integrating the MOM diode into a phased-array antenna, the angle of arrival and degree of coherence of received IR radiation can be determined. The angular response characteristics of IR dipole antennas are determined by boundary conditions imposed by the surrounding dielectric or conductive environment on the radiated fields. To explore the influence of the substrate configuration, single dipole antennas are fabricated on both planar and hemispherical lens substrates. Measurements demonstrate that the angular response can be tailored by the thickness of the electrical isolation stand-off layer on which the detector is fabricated and/or the inclusion of a ground plane. Directional detection of IR radiation is achieved with a pair of dipole antennas coupled to a MOM diode through a coplanar strip transmission line. The direction of maximum angular response is altered by varying the position of the diode along the transmission line connecting the antenna elements. By fabricating the devices on a quarter wave layer above a ground plane, narrow beam widths of 35° full width at half maximum and reception angles of ± 50° are achievable with minimal side-lobe contributions. Phased-array antennas can also be used to assess the degree of coherence of a partially coherent field. For a two-element array, the degree of coherence is a measure of the correlation of electric fields received by the antennas as a function of the element separation.

The emergence of mode-locked oscillators providing pulses with durations as short as a few electric-field cycles in the near infra-red has paved the way toward electric-field sensitive physics experiments. In addition, the control of the relative phase between the carrier and the pulse envelope, developed in the early 2000’s and rewarded by a Nobel price in 2005, now provides unprecedented control over the pulse behaviour. The amplification of such pulses to the millijoule level has been an on-going task in a few world-class laboratories and has triggered the dawn of attoscience, the science of events happening on an attosecond timescale. This work describes the theoretical aspects, modeling and experimental implementation of HERACLES, the Laser Plasma Laboratory optical parametric chirped pulse amplifier (OPCPA) designed to deliver amplified carrier-envelope phase stabilized 8-fs pulses with energy beyond 1 mJ at repetition rates up to 10 kHz at 800 nm central wavelength. The design of the hybrid fiber/solid-state amplifier line delivering 85-ps pulses with energy up to 10 mJ at repetition rates in the multi-kHz regime tailored for pumping the optical parametric amplifier stages is presented. The novel stretcher/compressor design of HERACLES, suitable for handling optical pulses with spectra exceeding 300 nm of bandwidth with unprecedented flexibility, is fully modeled and also presented in the frame of this thesis. Finally, a 3D model of the multistage non-collinear optical parametric amplifier is also reported. The current and foreseen overall performances of HERACLES are presented. This facility is designed to enable attosecond physics experiments, high-harmonic generation and physics of plasma studies.

Non-reciprocal wave transmission is a phenomenon witnessed in certain photonic devices when the wave propagation dynamics through the device along one direction differs greatly from the dynamics along the counter-propagating direction. Specifically, it refers to significant power transfer occurring in one direction, and greatly reduced power transfer in the opposite direction. The resulting effect is to isolate the directionality of wave propagation, allowing transmission to occur along one direction only. Given the popularity of photonic integrated circuits (PIC), in which all the optical components are fabricated on the same chip so that the entire optical system can be made more compact, it is desirable to have an easily integrated optical isolator. Common free-space optical isolator designs, which rely on the Faraday effect, are limited by the availability of suitable magnetic materials. This research proposes a novel integrated optical isolator based on an array of closely spaced, identical waveguides. Because of the nonlinear optical properties of the material, this device exploits the differing behaviors of such an array when illuminated with either a high power or a low power beam to achieve non-reciprocal wave transmission in the forwards and backwards directions, respectively. The switching can be controlled electro-optically via an integrated gain section which provides optical amplification before the input to the array. The design, fabrication, characterization and testing of this optical isolator are covered in this dissertation. We study the switching dynamics of this device and present its optimum operating conditions.

With exploding growth of information exchanges between people, display has become indispensable in our daily lives. After decades of intensive research and development in materials and devices, and massive investment in manufacturing technologies, liquid crystal display (LCD) has overcome various obstacles and achieved the performance we need, such as wide viewing angle, high contrast ratio, and high resolution, etc. These excellent performances make LCD prevailed in every perspective. Recently, with the demands of energy conservation, a greener LCD with lower power consumption is desired. In order to achieve this goal, new energy-effective driving methods, such as field sequential color display, have been proposed. However, in order to suppress color breakup the LC response time should be faster than 1 ms. To overcome this challenge, various fast-response liquid crystal modes, such as thin cell gap, low viscosity materials, overdrive and undershoot voltages, polymer stabilization, and ferroelectric liquid crystal, are under active investigations. Among these approaches, blue phase liquid crystal (BPLC) shows a greater potential with less fabrication limitations. In this dissertation, the feasibility of polymer-stabilized blue phase liquid crystal for display applications is explored starting from the building blocks of the material system, polymer-stabilization processes, test cell preparations, electro-optical (EO) properties, to suggested approaches for further improvements. iv Because of the nature of blue phase liquid crystals, delicate balance among system components is critically important. Besides the properties of each composition, the preparation process also dictates the EO performance of the self-assembled nano-structured BPLC composite. After the preparation of test cells, EO properties for display applications are investigated and results described. Approaches for further improvements of the EO properties are also suggested in the final part of this dissertation.