The development and application of portable LCD (Liquid crystal display) technology is the main trend on the market. The goal of this study is to fabricate a compound optical film, and we focus on the design and fabrication of a new type backlight module for side-LED (Light emitting diode) display. The optical efficiency can be improved via the compound optical film. The profile of optical film was determined using commercial optical software, FRED. The mold with multi aspect ratio and multi fill-factor microlens array by LIGA-like process (Lithographie galvanoformung abformung) was produced using THB-126N negative photoresist and AZ-4620 positive photoresist. The study presents many innovative processes, such as the homemade gray scale mask, and multi-step electroforming method, which both produces the microlens array with variable size and aspect ratio. In addition, the embedded micro-void caused light guide and diffusion under the quantitative control during the PDMS (Polydimethylsiloxane) optical film fabrication. The compound optical film with embedded micro-voids, multi aspect ratio and variable size microlens array can be fabricated quickly without substrate. Then the optical properties were analyzed by BM-7A to characterize the luminance, uniformity and optical efficiency.