Future magnetic fusion reactors such as tokamaks will need innovative, fast, deep-fueling systems to inject frozen deuterium-tritium pellets at high speeds and high repetition rates into the hot plasma core. There have been several studies and concepts for pellet injectors generated, and different devices have been proposed. In addition to fueling, recent studies show that it may be possible to disrupt edge localized mode (ELM) formation by injecting pellets or gas into the fusion plasma. The system studied is capable of doing either at a variety of plasma and pellet velocities, volumes, and repetition rates that can be controlled through the formation conditions of the plasma. In magnetic or inertial fusion reactors, hydrogen, its isotopes, and lithium are used as fusion fueling materials. Lithium is considered a fusion fuel and not an impurity in fusion reactors as it can be used to produce fusion energy and breed fusion products. Lithium hydride and lithium deuteride may serve as good ablating sleeves for plasma formation in an ablation-dominated electrothermal plasma source to propel fusion pellets. Previous studies have shown that pellet exit velocities, greater 3 km/s, are possible using low-z propellant materials. In this work, a comprehensive study of solid lithium hydride and deuteride as a pellet propellant is conducted using the ETFLOW code, and relationships between propellants, source and barrel geometry, pellet volume and aspect ratio, and pellet velocity are determined for pellets ranging in volume from 1 to 100 mm3. / Master of Science