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Nonlinear Ultrafast Excitation and Two-Dimensional Terahertz Spectroscopy of SolidsKnighton, Brittany E. 27 July 2021 (has links)
Ultrafast spectroscopy allows us to probe and understand material properties. With it, we can measure phonon-polaritons (optical phonons coupled with light) and the resulting dispersion curve in lithium niobate. Customizing the excitation source in ultrafast measurements can excite phonon modes to large amplitudes, allowing the experimental exploration of the Potential Energy Surface in solids. However, stronger pump fluences and bigger signal isn't always the answer in ultrafast spectroscopy. When sample signals and their nonlinear and mechanisms cannot be distinguished with 1D measurements, simple 2D THz measurements are a great place to start searching for distinct factors as was the case in cadmium tungstate. 2D measurements when paired with modeling and first principles calculations can reveal cutting edge information about exciting materials.
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The taiji and infinity-loop microresonators: examples of non-hermitian photonic systemsFranchi, Riccardo 01 June 2023 (has links)
This thesis theoretically and experimentally studies the characteristics of integrated microresonators (MRs) built by passive (no gain) and non-magnetic materials and characterized by both Hermitian and non-Hermitian Hamiltonians. In particular, I have studied three different microresonators: a typical Microring Resonator (MR), a Taiji Microresonator (TJMR), which consists of a microresonator with an embedded S-shaped waveguide, and a new geometry called the Infinity-Loop Microresonator (ILMR), which is characterized by a microresonator shaped like the infinity symbol coupled at two points to the bus waveguide. To get an accurate picture of the three devices, they were modeled using both the transfer matrix method and the temporal coupled mode theory. Neglecting propagation losses, the MR is described by a Hermitian Hamiltonian, while the TJMR and the ILMR are described by a non-Hermitian one. An important difference between Hermitian and non-Hermitian systems concerns their degeneracies. Hermitian degeneracies are called Diabolic Points (DPs) and are characterized by coincident eigenvalues and mutually orthogonal eigenvectors. In contrast, non-Hermitian degeneracies are called Exceptional Points (EPs). At the EP, both the eigenvalues and the eigenvectors coalesce. The MR is at a DP instead, and the TJMR and the ILMR are at an EP. Since the TJMR and ILMR are at an EP, they have interesting features such as the possibility of being unidirectional reflectors. Here, it is shown experimentally how in the case of the TJMR this degeneracy can also be used to break Lorentz reciprocity in the nonlinear regime (high incident laser powers), discussing the effect of the Fabry-Perot of the bus waveguide facets. The effect of backscattering, mainly due to the waveguide surface-wall roughness, on the microresonators is also studied. This phenomenon induces simultaneous excitation of the clockwise and counterclockwise modes, leading to eigenvalue splitting. This splitting makes the use of typical quality factor estimation methods unfeasible. To overcome this problem and mitigate the negative effects of backscattering, a new experimental technique called interferometric excitation is introduced. This technique involves coherent excitation of the microresonator from both sides of the bus waveguide, allowing selective excitation of a single supermode. By adjusting the relative phase and amplitude between the excitation fields, the splitting in the transmission spectrum can be eliminated, resulting in improved quality factors and eigenvalue measurements. It is shown that this interferometric technique can be exploited under both stationary and dynamic conditions of time evolution. The thesis also investigates the sensing performance of the three microresonators as a function of a backscattering perturbation, which could be caused, for example, by the presence of a molecule or particle near the microresonator waveguide. It is shown that the ILMR has better performance in terms of responsivity and sensitivity than the other two microresonators. In fact, it has both the enhanced sensitivity due to the square root dependence of the splitting on the perturbation (characteristic of EPs) and the ability to completely eliminate the region of insensitivity as the backscattering perturbation approaches zero, which is present in both the other two microresonators. To validate the models used, they were compared with experimental measurements both in the linear regime and, for TJMR, also in the nonlinear regime, with excellent agreement.
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