<p>This thesis describes new results obtained from experimental studies of the extremely neutron-deficient isotopes ¹⁶⁹Ir and¹¹⁰Xe, close to the proton drip-line. The experiments use state-of-the-art equipment for nuclear spectroscopy where a large high-resolution Germanium-detector array is coupled to a high-transmission recoil separator and using the highly selective recoil-decay tagging technique. The work is based on two experiments performed at the Accelerator Laboratory of the University of Jyväskylä, Finland. The experimental techniques used are described as are the experimental set-ups. Comparison between experimental results and theoretical predictions are made. The thesis also briefly summarises the theoretical models employed to interpret the experimental results. The results for 169Ir point to a rotational-like behaviour of a moderately deformed nucleus exhibiting triaxial shape. The experimental results do not fully agree with theoretical predictions for the shape evolution of the neutron-deficient iridium isotopes, approaching the proton drip-line. The results for ¹¹⁰Xe indicate an emergence of enhanced collectivity near the N=Z line in the region of the nuclear chart above ¹⁰⁰Sn. These findings are interpreted as a possible effect of increased neutron-proton isoscalar pair correlations, a residual interaction effect not accounted for in present-day nuclear models.</p>

<p>Vapor explosion as a result of Molten Fuel-Coolant Interactions (MFCI) postulated to occur in certain severe accident scenarios in a nuclear power plant presents a credible challenge on the plant containment integrity. Over the past several decades, a large body of literature has been accumulated on vapor explosion phenomenology and methods for assessment of the related risk. Vapor explosion is driven by a rapid fragmentation of high-temperature melt droplets, leading to a substantial increase of heat transfer areas and subsequent explosive evaporation of the volatile coolant. Constrained by the liquid-phase coolant, such rapid vapor production in the interaction zone causes pressurization and dynamic loading on surrounding structures. While such a general understanding has been established, the triggering mechanism and subsequent dynamic fine fragmentation have yet not been clearly understood. A few mechanistic fragmentation models have been proposed, however, computational efforts to simulate such phenomena generated a large scatter of results.</p><p>In order to develop a mechanistic understanding of thermal-hydraulic processes in vapor explosion, it is paramount to characterize dynamics of fragmentation of the hot liquid (melt) drop and vaporization of the volatile liquid (coolant). In the present study, these intricate phenomena are investigated by performing well-controlled, externally triggered, single-drop experiments, using advanced diagnostic techniques to attain visual information of the processes. The methodology’s main challenge stemming from the opaqueness of the molten material surrounded by the vapor film and rapid dynamics of the process, was overcome by employing a high-speed digital visualization system with synchronized cinematography and X-ray radiography system called SHARP (Simultaneous High-speed Acquisition of X-ray Radiography and Photography).</p><p>The developed image processing methodology, focus on a separate quantification of vapor and molten material dynamics and an image synchronization procedure, consists of a series steps to reduce the effect of uneven illumination and noise inherited of our system, further segmentation, i.e. edge detection, and extraction of image features, e.g. area, aspect ratio, image center and image intensity (radiography).</p><p>Furthermore, the intrinsic property of x-ray radiation, namely the differences in linear mass attenuation coefficients over the beam path through a multi-component system, which translates the image intensity to a transient projection of the molten material morphology, was exploited. A methodology for the quantitative analysis of the x-ray images, i.e. transient maps of the fragmented melt, was developed. Its uncertainties were evaluated analytically and experimentally pointing towards the need to minimize the X-ray scattering and noise inherited from the optical system, for a more accurate quantification and a larger calibrated thickness range.</p><p>Analysis of the data obtained by the SHARP system and image processing procedure developed provided new insights into the physics of the vapor explosion phenomena, as well as, quantitative information of the associated dynamic micro-interactions.</p><p>The qualitative analysis, based on the matched radiograph and photographic images, describe the bubble and melt interrelated progression granting information on the phenomenological micro-interaction of the vapor explosion process. The dynamics of the initially disturbed vapor film is composed by multiple cycles, where the vapor bubble grows to a maximum diameter and collapses. X-ray radiographs show that during the first bubble expansion, the melt undergoes deformation/pre-fragmentation but does not follow the bubble interface during the subsequent expansion; suggesting no mixing between coolant and melt. Coolant entrainment occurs when the expanded bubble collapses leading to fine fragmentation of the molten material due to explosive evaporation. The vapor bubble expansion, fed by these fragments at the boundary, reaches its critical size, and start collapsing. The remaining melt is accountable for the following cycle.</p><p>Bubble dynamics analysis shows a strong correlation between energetics of the subsequent explosive evaporation and the high temperature molten material drop (tin) deformation/partial fragmentation during the first bubble growth. The data suggest that this pre-fragmentation may have been responsible in providing an adequate mixing condition that promotes coolant entrainment during the bubble collapse stage. The SHARP observations followed by further analysis leads to a hypothesis about a novel phenomenon called <b>pre-conditioning</b>, according to which dynamics of the first bubble-dynamics cycle and the ability of the melt drop to deform/pre-fragment dictate the subsequent explosivity of the so-triggered drop.</p>

<p>One of the most important affairs in the nuclear industry is the fuel cycle situation prediction. It affects the energy company’s profit, environment and even the safety of reactor operation. For these reasons, a series of computer codes have been generated to simulate the fuel cycle scenario including NFCSim, ORION and so on. At the Department of Reactor Physics, a new fuel cycle simulation code is under development and this code will be used in the present thesis.In order to simulate the nuclides transmutation chains, MCNP was first used to calculate the neutron spectrum and cross section data for the reactor cores, using JEF 3.0 and EAF 99 data libraries.The main task of this project is to simulate the present and future status of all the facilities in Chinese reactor park. Three consecutive scenarios (present, near-term and long-term) are defined for this comparison, simulation time scale is set to be 208 years (1992~2200) and four groups of nuclides (major actinides, minor actinides, major fission products and safety related nuclides) are defined and presented.Power balance scenario, plutonium self-sustained scenario and CIAE proposals are discussed individually as choices of reactor parks’ future development. The result is that at least 70 years (cooling storage time is not included) are needed to transmute the minor actinides inventory after the large-scale FBR (Fast Breeder Reactor) technology is mature enough for large scale commissioning in plutonium-sustained scenario.</p>

Thesis (Ph. D.)--University of Texas at Austin, 2001. / Vita. Includes bibliographical references. Available also from UMI/Dissertation Abstracts International.

Thesis (Ph. D.)--University of Hawaii at Manoa, 2004. / Includes bibliographical references (leaves 117-119). Also available via World Wide Web.

Thesis (Ph.D.)--University of Illinois at Urbana-Champaign, 2009. / Source: Dissertation Abstracts International, Volume: 70-06, Section: B, page: 3759. Adviser: Roy A. Axford. Includes bibliographical references (leaves 309-311) Available on microfilm from Pro Quest Information and Learning.

Thesis (Ph. D.)--Ohio State University, 2004. / Title from first page of PDF file. Document formatted into pages; contains xxvi, 249 p.; also includes graphics (some col.). Includes abstract and vita. Advisor: Anil K. Pradhan, Dept. of Astronomy. Includes bibliographical references (p. 237-249).

Proefschrift--Utrecht. / Summary in English. Bibliography: p. 65-67.

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