Thesis (MSc)--Stellenbosch University, 2012. / ENGLISH ABSTRACT: The experimental observation of the quantum Hall effect in a two-dimensional electron gas posed an intriguing question to theorists: Why is the quantization of conductance so precise, given the imperfections of the measured samples? The question was answered a few years later, when a connection was uncovered between the quantum Hall effect and topological quantities associated with the band structure of the material in which it is observed. The Hall conductance was revealed to be an integer topological invariant, implying its robustness to certain perturbations. The topological theory went further than explaining only the usual integer quantum Hall effect in a perpendicular magnetic field. Soon it was realized that it also applies to certain systems in which the total magnetic flux is zero. Thus it is possible to have a quantized Hall effect without Landau levels. We study a carbon nanotube in a magnetic field perpendicular to its axial direction. Recent studies suggest that the application of an electric field parallel to the magnetic field would induce a gap in the electronic spectrum of a previously metallic carbon nanotube. Despite the quasi onedimensional nature of the carbon nanotube, the gapped state supports a quantum Hall effect and is associated with a non zero topological invariant. This result is revealed when an additional magnetic field is applied parallel to the axis of the carbon nanotube. If the flux due to this magnetic field is varied by one flux quantum, exactly one electron is transported between the ends of the carbon nanotube. / AFRIKAANSE OPSOMMING: Die eksperimentele waarneming van die kwantum Hall effek in ’n twee-dimensionele elektron gas laat ’n interessante vraag aan teoretiese fisikuste: Waarom sou die kwantisasie van die geleiding so presies wees al bevat die monsters, waarop die meetings gedoen word, onsuiwerhede? Hierdie vraag word ’n paar jaar later geantwoord toe ’n konneksie tussen die kwantum Hall effek en topologiese waardes, wat verband hou met die bandstruktuur van die monster, gemaak is. Dit is aan die lig gebring dat die Hall geleiding ’n heeltallige topologiese invariante is wat die robuustheid teen sekere steurings impliseer. Die topologiese teorie verduidelik nie net die gewone kwantum Hall effek wat in ’n loodregte magneetveld waargeneem word nie. Dit is ook moontlik om ’n kwantum Hall effek waar te neem in sekere sisteme waar die totale magneetvloed nul is. Dit is dus moontlik om ’n gekwantiseerde Hall effek sonder Landau levels te hˆe. Ons bestudeer ’n koolstofnanobuis in ’n magneetveld loodreg tot die aksiale rigting. Onlangse studies dui daarop dat die toepassing van ’n elektriese veld parallel aan die magneetveld ’n gaping in die elektroniese spektrum van ’n metaliese koolstofnanobuis induseer. Ten spyte van die een-dimensionele aard van die koolstofnanobuis ondersteun die gapings-toestand steeds ’n kwantum Hall effek en hou dit verband met ’n nie-nul topologiese invariante. Hierdie resultaat word openbaar wanneer ’n bykomende magneetveld parallel tot die as van die koolstofnanobuis toegedien word. Indien die vloed as gevolg van hierdie magneetveld met een vloedkwantum verander word, word presies een elektron tussen die twee kante van die koolstofnanobuis vervoer.

In the first part of this work, we describe a theory of the ground states and charge gaps in the fractional quantum Hall states of graphene. The theory relies on knowledge of these properties for filling fractions smaller than one. Then, by the application of two mapping rules, one is able to obtain these properties for fractional quantum Hall states at arbitrary fillings, by conceiving the quantum Hall ferromagnets as vacua on which correlated electrons or correlated holes are added. The predicted charge gaps and phase transitions between different fractional quantum Hall states are in good agreement with recent experiments. In the second part, we investigate the low energy theory for the neutral Landau level of bilayer graphene. We closely analyze the way different terms in the Hamiltonian transform under the action of particle-hole conjugation symmetries, and identify several terms that are relevant in explaining the lack of such symmetry in experiments. Combining an accurate parametrization of the electronic structure of bilayer graphene with a systematic account of the impact of screening we are able to explain the absence of particle-hole symmetry reported in recent experiments. We also study the energetics of fractional quantum Hall states with coherence between n=0 and n=1 cyclotron quantum numbers, and obtain a general formula to map the two-point correlation function from their well-known counterparts made from only n=0 quantum numbers. Bilayer graphene has the potential for realizing these states which have no analogue in other two-dimensional electron systems such as Gallium Arsenide. We apply this formula to describe the properties of the n=0/n=1 coherent Laughlin state which displays nematic correlations. / text

The two dimensional electron gas subjected to a perpendicular magnetic field is a model system that supports a variety of electronic phases. Perhaps the most well-known are the fractional quantum Hall states, but in recent years there has been an upsurge of interest in the charge ordered phases commonly referred to as electron solids. These solids are a consequence of electron-electron interactions in a magnetic field. While some solid phases form in the lowest Landau level, the charged ordered phases are most abundant in the higher Landau levels. Examples of such phases include the Wigner solids, electronic bubble phases and stripe or nematic phases. Open questions surround the exact role of disorder, confinement potential, temperature and the Landau level index in determining the stability and competition of these phases with other ground states. <div>The interface of GaAs/AlGaAs remains the cleanest host for the two-dimensional electron gas due to the extremely high quality of materials available and the advancement in molecular beam epitaxy growth techniques. As a result, exceptionally high electron mobilities in this system have been instrumental in the discovery of numerous electron solids. </div><div>In this Thesis, I discuss the discovery and properties of several electron solids that develop in such state-of-the-art two dimensional electron gases. These electron solids often develop at ultra low temperatures, in the milliKelvin temperature range. After an introduction to the physics of the quantum Hall effect in two dimensions, in chapter 3, I discuss electron solids developing in the N=1 Landau level. While these solids have been known for some time, details of the competition of these phases xiii with the nearby fractional quantum Hall states remains elusive. A number of reports observe new fractional quantum Hall states at filling factors where electron solids are found in other experiments. We undertook a systematic study to answer some of these unsettled questions. We see evidence for incipient fractional quantum Hall states at 2+2/7 and 2+5/7 at intermediate temperatures which are overtaken by the electronic bubble phases at lower temperatures. Several missing fractional states including those at filling factors 2+3/5, 2+3/7, 2+4/9 highlight the relative stability of the electronic solids called the bubble phases in the vicinity in our sample. </div><div>In chapter 4, I discuss a newly seen electron crystal which manifests itself in transport measurements as a reentrant integer quantum Hall state. Reentrant integer behavior is common in high Landau levels, but so far it was not observed in the lowest Landau level in narrow quantum well samples. In contrast to high Landau levels, where such reentrant integer behavior was associated with electronic bubbles, we believe that the same signature in the N=0 Landau level is due to an electronic Wigner crystal. The filling factors at which we observe such reentrance reveal that it is a crystal of holes, rather than electrons. The discovery of this reentrant integer state paints a complex picture of the interplay of the Wigner crystal and fractional quantum Hall states. </div><div>Finally, in chapter 5, I discuss the observation of a novel phenomenon, that of reentrant fractional quantum Hall effect. In the lowest Landau level, we observe a fractional quantum Hall state, but as the field is increased, we see a deviation and then a return to quantization in the Hall resistance. Such a behavior indicates a novel electron solid. In contrast to the collective localization of electrons evidenced by the reentrant integer quantum Hall effect, such reentrance to a fractional Hall resistance clearly points to the involvement of composite fermion quasiparticles. This property thus distinguishes the ground state we observed as a solid formed of composite fermions. Such a solid phase is evidence for exotic electron-electron correlations at play which are clearly different from those in the traditional Wigner solid of electrons.<br></div>

Nesta tese, apresentamos estudos de magnetotransporte em poços quânticos duplos (DQWs) a campos magnéticos de baixo e sob a aplicação de um campo elétrico externo (potencial de porta). Medidas de magnetorresistência foram realizadas tanto no regime linear quanto no regime não linear. Relatamos a observação de oscilações magnéticas de inter-sub-banda (MIS) pela primeira vez. Estas oscilações MIS já foram estudadas em poços quânticos simples (QWs) com duas sub-bandas ocupadas; um DQW´e o sistema mais apropriado para o estudo das oscilações MIS. As oscilações MIS são atribuídas ao espalhamento inter-sub-banda, e a intensidade delas depende da largura da barreira (relacionada ao gap de energia entre as duas sub-bandas ocupadas, SAS). O estudo das oscilações MIS é uma ferramenta importante para poder acessar ao tempo de vida quântico dos elétrons a temperaturas onde as oscilações Shubnikov-de Haas (SdH) já não são observadas. Em nossas amostras, as oscilações MIS persistem até 25 K. Explicamos estes resultados num modelo teórico considerando um potencial de espalhamento de curto alcance com uma contribuição significativa do tempo de espalhamento elástico dos elétrons e uma contribuição do espalhamento elétron-elétron (e-e) com o aumento da temperatura. A aplicação de um campo elétrico externo (correntes dc) modifica fortemente as oscilações MIS. Descrevemos este efeito não linear causado pelo campo elétrico dc com uma função de distribuição oscilatória. Considerando o aquecimento dos elétrons pelo campo elétrico, é extraído o tempo de espalhamento inelástico. Para correntes dc grandes são encontradas discrepâncias entre o experimento e a teoria. Finalmente, consideramos medidas de magnetotransporte como função de potenciais de porta (porta na superficie) levando ao desbalance do DQW. Encontramos que as contribuições clássica e quântica são necessárias para a descrição teórica da magnetorresistência. Descrevemos as contribuições da magnetorresistência em termos das taxas de espalhamento inter e intra sub-banda utilizando uma função gaussiana como função da correlação do potencial. / In this thesis we present studies of magnetotransport in double quantum wells (DQWs) in low magnetic fields and under application of an external electric field (gate potential). Measurements of magnetoresistance have been carried out in both linear and non-linear regime. We report on the observation of magneto-intersubband (MIS) oscillations for the first time. These MIS oscillations have been studied already in quantum wells (QWs) with two occupied subbands, DQW is the most convenient system for studies of MIS oscillations. They are attributed to intersubband scattering and the strength of MIS oscillations depends on the barrier width (´delta´SAS). Analysis of MIS oscillations is an important tool to access quantum lifetime of electrons at high temperatures where Shubnikov-de Haas (SdH) oscillations are already absent. For our samples, MIS oscillations still exist up to 25 K. We explain these results in a theoretical model considering short-range scattering potential with a significant contribution of el´astic scattering time of electrons and a contribution of electron-electron (e-e) scattering if one increases temperature. Application of an external electric field (here a dc currents) strongly modifies the MIS oscillations. We describe this non-linear effect caused by a dc electric field with nonequilibrium part of the electron distribution function. Including the heating of electrons by the electric field, we are able to extract inelastic scattering time. For a strong dc current, a discrepancy between experiment and theory is found. Finally, we consider gate-dependent (top gate) magnetotransport measurements and drive de DQWs out of balance. We find that both cl´assical and quantum contributions are necessary for theoretical description of the magnetoresistance. We express both contributions in terms of inter and intrasubband scattering rates using a gaussian function as correlation function of the potential.

Thesis advisor: Ziqiang Wang / Exotic phases and associated phase transitions in low dimensions have been a fascinating frontier and a driving force in modern condensed matter physics since the 80s. Due to strong correlation effect, they are beyond the description of mean-field theory based on a single-particle picture and Landau's symmetry-breaking theory of phase transitions. These new phases of matter require new physical quantities to characterize them and new languages to describe them. This thesis is devoted to the study on exotic phases of correlated electrons in two spatial dimensions. We present the following efforts in understanding two-dimensional exotic phases: (1) Using Zn vertex algebra, we give a complete classification and characterization of different one-component fractional quantum Hall (FQH) states, including their ground state properties and quasiparticles. (2) In terms of a non-unitary transformation, we obtain the exact form of statistical interactions between composite fermions in the lowest Landau level (LLL) with v=1/(2m), m=1,2... By studying the pairing instability of composite fermions we theoretically explains recently observed FQHE in LLL with v=1/2,1/4. (3) We classify different Z2 spin liquids (SLs) on kagome lattice in Schwinger-fermion representation using projective symmetry group (PSG). We propose one most promising candidate for the numerically discovered SL state in nearest-neighbor Heisenberg model on kagome lattice}. (4) By analyzing different Z2 spin liquids on honeycomb lattice within PSG classification, we find out the nature of the gapped SL phase in honeycomb lattice Hubbard model, labeled sublattice pairing state (SPS) in Schwinger-fermion representation. We also identify the neighboring magnetic phase of SPS as a chiral-antiferromagnetic (CAF) phase and analyze the continuous phase transition between SPS and CAF phase. For the first time we identify a SL called 0-flux state in Schwinger-boson representation with one (SPS) in Schwinger-fermion representation by a duality transformation. (5) We show that when certain non-collinear magnetic order coexists in a singlet nodal superconductor, there will be Majorana bound states in vortex cores/on the edges of the superconductor. This proposal opens a window for discovering Majorana fermions in strongly correlated electrons. (6) Motivated by recent numerical discovery of fractionalized phases in topological flat bands, we construct wavefunctions for spin-polarized fractional Chern insulators (FCI) and time reversal symmetric fractional topological insulators (FTI) by parton approach. We show that lattice symmetries give rise to different FCI/FTI states even with the same filling fraction. For the first time we construct FTI wavefunctions in the absence of spin conservation which preserve all lattice symmetries. The constructed wavefunctions also set up the framework for future variational Monte Carlo simulations. / Thesis (PhD) — Boston College, 2011. / Submitted to: Boston College. Graduate School of Arts and Sciences. / Discipline: Physics.

Le sujet de cette thèse concerne le transport en alternatif à basse fréquence dans les états de bords de l'effet Hall quantique. L'objet d'étude est la partie imaginaire de l'admittance, inductive ou capacitive, des échantillons de Hall. Dans un gaz d'électrons bidimensionnel, le transport à très basse température sous champ magnétique quantifiant, se fait dans des canaux de bord unidimensionnels. Ces canaux ont une capacité quantique propre et sont par ailleurs couplés par l'interaction électrostatique.Nos échantillons sont fabriqués à partir d'hétérojonctions GaAlAs/GaAs et n'ont pas de grille pour n'exhiber que leur propriétés capacitives intrinsèques. Deux topologies sont étudiées dans cette thèse : les barres de Hall et les Corbinos, de géométrie circulaire. La topologie permet de distinguer 2 comportements dans le transport en alternatif.Sont d'abord présentées les mesures à l'impédancemètre de la partie imaginaire de l'impédance et les spectres de réactance, pour les barres de Hall en fonction de la fréquence. Nous utilisons des mesures 3 points ou bien 2 points, mais toujours en 4 fils, et révélons la nature inductive des état de bords. Nous montrons que l'inductance est inversement proportionnelle à la densité d'état, comme le prévoit le calcul de l'inductance quantique d'un canal 1D. Le formalisme de Buttiker permet en outre de comprendre cette dépendance en terme de capacité mutuelle des états de bords.Nous mesurons également la partie imaginaire de l'admittance et traçons les spectres de susceptance des Corbinos, qui s'avèrent être des capacités parfaites. Nos résultats s'interprètent en faisant intervenir la capacité quantique des états de bords.Enfin, nous montrons que l'effet Hall dans un échantillon type barre, peut être vu comme l'effet d'apparition d'une inductance, et ceci même à haute température. Cette inductance cinétique est le résultat de l'augmentation du temps de dissipation de l'énergie sur les phonons, avec le champ magnétique. / In a two dimensional electron gas, low energy transport in presence of a magnetic field occurs in chiral 1D channels located on the edges of the sample. In the Buttiker’s description of a.c. quantum transport, the “emittance” determines the amplitude of the imaginary part of the admittance, whose sign and physical meaning are determined by the topology: in the case of an Hall bar the emittance is an inductance, while it is a capacitance in the case of a corbino sample.Emittance is related to the density of states and to the drift velocity of carriers. So quantum capacitances and inductances give access to the velocity of the charge carriers through the transit time/dwell time of charges in the quantum circuit.We performed systematic studies on samples with different topologies : Hall bars and Corbino disks. Our samples have no gate, which makes us able to observe the inner properties of the quantum states. We have measured the ac admittance of quantum Hall samples using standard electrical techniques in the [0.1-100] kHz frequency range, at low temperature under high magnetic field.We measured kinetic inductances of Hall bars with three contacts and showed the perfect inductive nature of edge states. We measured quantum capacitances of Corbino disks as well. In both topologies we observed the close relation between the emittance and the density of states. We show also the proportionality between the emittance and the length of the circuit. We obtain the transit time of electrons through the device, and finally the drift velocity on edge states.At high temperature we still observe an inductive behavior of Hall bars, induced by increase of energy relaxation time with magnetic field.

<div>Since the debut of graphene, many 2D materials have emerged as promising candidates for silicon alternatives to extend Moore’s Law, such as MoS₂ and phosphorene. However, some common shortcomings such as low mobility, instability and lack of massive production methods limit the exploration and applications of these materials. Here, we introduce a novel member to the 2D category – high-mobility air-stable 2D tellurium film (tellurene).</div><div><br></div><div>Tellurium (Te) is a narrow bandgap semiconductor with unique one-dimensional chiral structure. Recently, a hydrothermal synthesizing method was developed to produce large-area tellurene nanofilms with thickness ranging from tens of nanometers down to few layers. In this thesis, a thorough investigation of Te properties in 2D quantum region was first carried out by various material characterization techniques including TEM and Raman spectroscopy. Potential applications of Te-based electronics, optoelectronic and thermoelectric devices were explored, and high-performance Te FETs were achieved with record-high drive current over 1 A/mm via device scaling and contact engineering. Magneto-transport, including weak anti-localization and Shubnikov-de-Haas oscillations was studied at cryogenic temperature. Quantum Hall effect was observed for the first time in both 2D electron and hole gases with mobility of 6,000 and 3,000 cm²/Vs, and non-trivial Berry phase in Te 2D electron system was detected as the first experimental evidence of massive Weyl fermions. This work not only demonstrates the great potential of tellurene films for electronics and quantum device applications, but also expands the spectrum of topological matters into a new material species - Weyl semiconductors.</div>

The fractional quantum Hall (FQH) effect harbors a wealth of unique phenomena, many of which remain mysterious. Of particular interest is the predicted existence of quasi-particles with unusual topological properties, especially in light of recent proposals to observe these properties using electronic interferometers. An introduction to quantum Hall physics and electronic interferometry is given in Chapter 1 of this thesis. The remaining chapters, summarized below, describe a set of experiments in which FQH systems are studied using electronic Fabry-Perot interferometry and related techniques. Since prior studies of electronic Fabry-Perot interferometers revealed unexpected behavior even in the integer quantum Hall (IQH) regime, we began our measurements there. Our initial experiment, presented in Chapter 2, disentangles signatures of Coulomb interaction effects from those of Aharonov-Bohm (AB) interference and provides the first measurement of pure AB interference in these devices. In our next experiment, presented in Chapter 3, we measure AB interference oscillations as a function of an applied dc bias, use their period to study the velocity of the interfering electrons, and study how the oscillations decay as a function of bias and magnetic field. Moving to the FQH regime, applying a similar-sized bias to a quantum point contact leads to long-lasting changes in the strengths and positions of FQH plateaus. The involvement of lattice nuclear spins in this effect, suggested by the long persistence times, is confirmed using NMR-type measurements. Although the exact physical process responsible for the effect remains unclear, its filling-factor dependence provides a striking illustration of composite fermion physics. These measurements are described in Chapter 4. In certain devices, interference oscillations associated with several FQH states are observed. Interpretation of their magnetic-field and gate-voltage periods provides a measurement of quasi-particle charge, and temperature dependence measurements suggest differences between the edge structure of IQH and FQH states. These measurements are described in Chapter 5. Finally, Chapter 6 presents some recent, not-yet-published observations that may shed light on ways to improve the visibility of existing oscillations and potentially observe interference at additional FQH states. This chapter concludes with a discussion of possible next steps toward achieving these goals. / Physics

This thesis is a study of three categories of problems in fermionic systems for which topology plays an important role: (i) The properties of zero modes arising in systems of fermions interacting with a bosonic background, with a special focus on Majorana modes arising in the superconductor state. We propose a method for counting Majorana modes and we study a mechanism for controlling their number parity in lattice systems, two questions that are of relevance to the protection of quantum bits. (ii) The study of dispersionless bands in two dimensions as a platform for correlated physics, where it is shown the possibility of stabilizing the fractional quantum Hall effect in a flat band with Chern number. (iii) The extension of the hierarchy of quantum Hall fluids to the case of time-reversal symmetric incompressible ground states describing a phase of strongly interacting topological insulators in two dimensions. / Physics

This thesis describes electronic transport experiments in graphene from the hopping to the ballistic regime. The first experiment studies dual-gated bilayer graphene devices. By applying an electric field with these dual gates, we can open a band gap in bilayer graphene and observe an increase in resistance of over six orders of magnitude as well as a strongly non-linear behavior in the transport characteristics. A temperature-dependence study of resistance at large electric field at the charge neutrality point shows the change in the transport mechanism from a hopping dominated regime at low temperature to a diffusive regime at high temperature. / Physics