High precision data from household travel survey (HTS) is extremely important for the transportation research, traffic models and policy formulation. Traditional methods of data collection were imprecise because they relied on people’s memories of trip information, such as date and location, and the remainder data had to be obtained by certain supplemental tools. The traditional methods suffered from intensive labor, large time consumption, and unsatisfactory data precision. Recent research trends to employ smartphone apps to collect HTS data. In this study, there are two goals to be addressed. First, a smartphone app is developed to realize a smartphone-based method only for data collection. Second, the researcher evaluates whether this method can supply or replace the traditional tools of HTS. Based on this premise, the smartphone app, TravelSurvey, is specially developed and used for this study. TravelSurvey is currently compatible with iPhone 4 or higher and iPhone Operating System (iOS) 6 or higher, except iPhone 6 or iPhone 6 plus and iOS 8. To evaluate the feasibility, eight individuals are recruited to participate in a pilot HTS. Afterwards, seven of them are involved in a semi-structured interview. The interview is designed to collect interviewees’ feedback directly, so the interview mainly concerns the users’ experience of TravelSurvey. Generally, the feedback is positive. In this study, the pilot HTS data is successfully uploaded to the server by the participants, and the interviewees prefer this smartphone-based method. Therefore, as a new tool, the smartphone-based method feasibly supports a typical HTS for data collection.