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Experimental study of nanoscale metal clusters using synchrotron radiation excited photoelectron spectroscopyMikkelä, M.-H. (Mikko-Heikki) 21 January 2013 (has links)
Abstract
In this work an experimental study of size varied, neutral, and free metal clusters using synchrotron radiation excited photoelectron spectroscopy was performed. The combined core-level and valence photoelectron spectroscopic investigation indicates metallic properties for nanoscale Rb, K, Sn, and Bi clusters. In the case of Sn the experimental results suggest a metal-to-insulator transition occurring at the studied size range. In addition to the experimental results the technical implementation of the cluster production set-up is presented and jellium-model-based simulations are compared with the experimental results of the Rb and K clusters.
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