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TOTAL SYNTHESES OF BERGAMOTANE SESQUITERPENES AND LYCOPODIUM ALKALOIDS AND COMPUTATIONAL STUDY TOWARD DIAMINATION OF ALLENES AND [2+2] SELECTIVITY

<p>Total synthesis of massarinolin A, purpurlides B, D, E, 2,3-deoxypurpurolide C, phleghenrines A and B were finished. A halogen bond promoted michael addiation was discovered during mechanism study toward diamination of allenes. Computational chemsitry study conducted toward the selectivity of 2+2 reaction supported the proposed key reaction during total synthesis of gibberellic acid 18.</p>

  1. 10.25394/pgs.21397566.v1
Identiferoai:union.ndltd.org:purdue.edu/oai:figshare.com:article/21397566
Date27 October 2022
CreatorsYe-Cheng Wang (14009903)
Source SetsPurdue University
Detected LanguageEnglish
TypeText, Thesis
RightsCC BY 4.0
Relationhttps://figshare.com/articles/thesis/TOTAL_SYNTHESES_OF_BERGAMOTANE_SESQUITERPENES_AND_LYCOPODIUM_ALKALOIDS_AND_COMPUTATIONAL_STUDY_TOWARD_DIAMINATION_OF_ALLENES_AND_2_2_SELECTIVITY/21397566

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