In spite of the failures to find an ultimate theory of unconventional superconductivity, after many years of research the scientific community possesses a considerable store of theoretical knowledge about the problem. Over time, the focus is gradually shifted from finding a theoretical description of an experimentally observed phenomenon to distinguishing between multiple models that offer comparably reasonable descriptions. From the point of view of an experimentalist, this means that any qualitative under-standing of an experimental observation would no longer suffice. Instead, the empha-sis in the experimental research should be shifted to accurate quantification of obser-vations, which becomes possible only if the results available from all the available ex-perimental methods are connected together by the theoretical glue. Among the meth-ods that are to be unified, ARPES plays a central role. The reason for this is that it gives access to the single-particle excitation spectrum of the material as a function of both momentum and energy with very high resolution. Other experimental techniques, such as inelastic neutron scattering (INS), Raman spectroscopy, or the newly estab-lished Fourier-transform scanning tunneling spectroscopy (FT-STS) probe more com-plicated two-particle spectra of the electrons and up to now can not achieve the mo-mentum resolution comparable with that of ARPES. Such reasoning serves as the mo-tivation for the present work, in which some steps are done towards understanding the anomalous effects observed in the single-particle excitation spectra of cuprates and relating the ARPES technique to other experimental methods. First, the electronic properties of BSCCO are considered — the superconducting cuprate most studied by surface-sensitive methods. The recent progress in un-derstanding the electronic structure of this material is reported, focusing mainly on the many-body effects (renormalization) and their manifestation in the ARPES spectra. The main result of this part of the work is a model of the Green’s function that is later used for calculating the two-particle excitation spectrum. Then, the matrix element effects in the photoemission spectra of cuprates are discussed. After a general introduction to the problem, the thesis focuses on the recently discovered anomalous behavior of the ARPES spectra that partially originates from the momentum-dependent photoemission matrix element. The momentum- and excitation energy dependence of the anomalous high-energy dispersion, termed “waterfalls”, is covered in full detail. Understanding the role of the matrix element effects in this phenomenon proves crucial, as they obstruct the view of the underlying excitation spectrum that is of indisputable interest. Finally, the work describes the relation of ARPES with other experimental methods, with the special focus on the INS spectroscopy. For the optimally doped bilayer Bi-based cuprate, the renormalized two-particle correlation function in the superconducting state is calculated from ARPES data within an itinerant model based on the random phase approximation (RPA). The results are compared with the experimental INS data on BSCCO and YBCO. The calculation is based on numerical models for the normal and anomalous Green’s functions fitted to the experimental single-particle spectra. The renormalization is taken into account both in the single-particle Green’s function by means of the self-energy, and in the two-particle correlation function by RPA. Additionally, two other applications of the same approach are briefly sketched: the relation of ARPES to FT-STS, and the nesting properties of Fermi surfaces in two-dimensional charge density wave systems.
| Identifer | oai:union.ndltd.org:DRESDEN/oai:qucosa:de:qucosa:23643 |
| Date | 27 June 2008 |
| Creators | Inosov, Dmytro |
| Contributors | Büchner, Bernd, Eremin, Ilya, Patthey, Luc |
| Publisher | Technische Universität Dresden, Leibniz-Institut für Festkörper- und Werkstoffforschung Dresden |
| Source Sets | Hochschulschriftenserver (HSSS) der SLUB Dresden |
| Language | English |
| Detected Language | English |
| Type | doc-type:doctoralThesis, info:eu-repo/semantics/doctoralThesis, doc-type:Text |
| Rights | info:eu-repo/semantics/openAccess |
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