Call number: LD2668 .T4 1958 W45

Call number: LD2668 .T4 1985 T53 / Master of Science

The purpose of this experiment was to make positive assignment of the Cs133 energy levels excited by the inelastic scattering of neutrons.

Following a NEA high priority nuclear data request, an experimental campaign to measure the prompt Î3-ray emissions from 235 U has been performed. This has used the STEFF spectrometer at the new Experimental Area 2 (EAR2) within the neutron time- of-flight facility (n_TOF), a white neutron source facility at CERN with energies from thermal to approximately 1 GeV. Prior to the experimental campaign, STEFF has been optimised for the environment of EAR2. The experimental hall features a high background Î3-ray rate, due to the nature of the spallation neutron source. Thus an investigation into reduction of the background Î3-ray rate, encountered by the NaI(Tl) detector array of STEFF, has been carried out. This has been via simulations using the simulation package FLUKA. Various materials and shielding geometries have been investigated but the effects determined to be insufficient in reducing the background rate by a meaningful amount. The NaI(Tl) detectors have been modified to improve their performance in a high count rate environment, and their behaviour characterised to understand the response to higher count rates. Initial testing demonstrated that the modified detectors maintain a potential to measure Î3-ray multiplicities up to 3 counts per microsecond. However, the energy resolution fails somewhere below 1.75 counts per microsecond. The experimental campaign has produced a large amount of data. The preliminary analysis of phase one data has considered incoming neutron energies ranging from thermal to an upper limit of 1 eV, with a minimum Î3-ray energy threshold of 160 keV. Results have been achieved for the prompt fission Î3-ray multiplicity and total energy of M Î3 = 6.3 ± 0.2 and E S,Î3 = 9.0 ± 0.1 MeV respectively. Further work is ongoing by the STEFF team at Manchester to improve upon these results and analyse the remainder of the data set at higher incoming neutron energies.

<p>High-spin states in the oblate deformed odd-odd thallium nucleus ( ) 109 190 81 Tl have been investigated through the reaction 175Lu(20Ne, 5n)190Tl at a beam energy of 115 MeV. The gamma rays emitted from 190Tl nucleus were detected with Ge detectors using the AFRODITE array at iThemba LABS, South Africa. Gamma-gamma coincidence data were obtained and used to construct the level scheme. In this work, Directional Correlations from Oriented (DCO) state ratios and linear polarization anisotropies were measured in order to deduce spin and parity of energy levels in the decay scheme. It was possible to determine the spin and parity of two additional signature-partner bands which decay to the ground-state band.</p>

The Anger camera has been used for the last quarter century in many areas of science to image gamma radiation. Some typical applications include medicine, where functionality of organs are studied in vivo, and industrial inspection of fuel rods for nuclear reactors. The standard Anger geometry includes a large scintillation crystal, light guide, photomultiplier array, and analog processing electronics. Even the most modern gamma cameras built today still use the standard Anger design. The work presented here describes an alternative to the standard gamma-camera design that is flexible enough to be used in a wide variety of applications. Especially in single-photon emmission computed tomography (SPECT) applications, the new design has the potential to be more efficient than the standard design. The new design is modular, that is, several small, separate units comprise a system. Each unit consists of a small gamma camera that is optically and electronically independent from other units. The units, called "modular cameras," can be configured around the region of interest so as to provide the maximum amount of information for reconstruction algorithms or direct information to the operator. The theoretical and experimental investigation of this report focuses on the design and construction of the modular cameras. Each modular camera is, in esscence, a small Anger camera. Components of each module include a scintillation crystal, a light guide, and an array of four photomultiplier tubes. Instead of an analog processing network, each module utilizes fast digital circuitry which includes direct analog-to-digital conversion of the photomultiplier signals, a lookup table which maps detector responses to position estimates of the scintillation flashes in the crystal, and an image memory which accumulates the position estimates and forms an image of the radiation incident on the faceplate of the camera. The digital electronics are necessary because analog techniques fail to give satisfactory estimates of scintillation position when the flashes occur near the sides of the crystal. The contents of the lookup table are determined from the statistical properties of the detected signals as a function of scintillation position. Experiments are described in which "best" estimates of position are found by processing data collected from an array of point-source positions in contact with the crystal. Alternative methods for construction of the lookup table are also discussed, which involve computer generation of the estimates. Both maximum-likelihood and mimimum-mean-square-error estimation rules are used, and the results are compared. A mathematical bound on the performance of the estimators is calculated assuming Poisson statistics for the detection process. The bound, which is a Cramer-Rao lower bound, is used to compare module geometries before lookup tables are constructed. A one-dimensional module, which accumulates information along one axis of the faceplate, is designed first. The one-dimensional module provides proof-of-principle evidence for the estimation techniques and is used to determine critical parameters for modular-camera design. The results of the experiments with the one-dimensional camera are extended to two-dimensional designs, which yield position estimates along both axes of the camera faceplate. Several two-dimensional cameras are tested, and an optimum geometry is constructed and tested for spatial resolution and bias of the estimators.

No description available.

No description available.

<p>High-spin states in the oblate deformed odd-odd thallium nucleus ( ) 109 190 81 Tl have been investigated through the reaction 175Lu(20Ne, 5n)190Tl at a beam energy of 115 MeV. The gamma rays emitted from 190Tl nucleus were detected with Ge detectors using the AFRODITE array at iThemba LABS, South Africa. Gamma-gamma coincidence data were obtained and used to construct the level scheme. In this work, Directional Correlations from Oriented (DCO) state ratios and linear polarization anisotropies were measured in order to deduce spin and parity of energy levels in the decay scheme. It was possible to determine the spin and parity of two additional signature-partner bands which decay to the ground-state band.</p>

Worldwide measurement of radon flux on mine tailing dams has been performed using various instruments. Some of the methods used in South Africa are electrets, alpha tracks, accumulator cans etc. Although these techniques and methods have been used for many years, a number of shortcomings are still evident. The major shortcomings are that, the methods lack spatial representivity that is, they only measure the radon flux at a point where they' are placed and not the whole site in that way, the spatial variation is not shown in a site which is not homogeneous. Another shortcoming is that, they do not show seasonal variation and some have a back diffusion problem, and the time required for the result to be known is too long. For· example it takes several days for electrets to gather sufficient information required, yet it is a single point result. This makes it difficult to steer the measurement. Furthermore, the moisture and atmospheric pressure on the mine dump influence some of the measurements. The above shortcomings led to the investigation of a new· technique based on gamma ray spectrometry to quantitatively assess the radon flux from the mine tailings dam. The system is called Multi Element Detector for Underwater Sediment Activity (MEDUSA). Initially, this technique was uniquely designed to measure the radioactivity on the sea floor where it proved to be successful. The major focus of this research study was, therefore, to critically assess the MEDUSA gamma ray detector system for measurement of radon flux on a tailings dam. The process of determining the radon flux in this work involved field measurements using MEDUSA and laboratory measurements using Hyper Pure Germanium (HPGe} detector. The laboratory measurements were for correcting the field measurements. The HPGe has better advantage over MEDUSA in terms of resolution and this means that the gamma ray energy peaks have better visibility than on the MEDUSA. The field measurements on the tailings dam were done using the MEDUSA mounted on a 4x4 vehicle, and simultaneously sample points were identified and samples collected. The samples were measured for specific activity in the laboratory using gamma spectrometer with HPGe detector. These measurements enabled the determination of a factor that was used to calculate the activity of radium in the field. This activity was found to have an average of 309 Bq.kg"1 with data range of 60 -540 Bq.kg-1.A radon flux equation was then derived and used to calculate the radon flux on the field. Based on the radium content, the radon flux was calculated to average about 0.105 ± 0.023 Bq.m-2 .s-1 The results are within the same range as the previous flux measurement on the same tailings dam but with better statistics. This research work has demonstrated that the MEDUSA can be adapted for radon flux determination from tailings dam. The method promises to address some of the key shortcomings of existing techniques and the usefulness of this method can be extended to measuring radioactivity on contaminated sites for rehabilitation purposes. / Thesis (MSc. ARST) North-West University, Mafikeng Campus, 2003