A novel broad spectrum neutron spectrometer has been created to extend the useful energy range of existing neutron Bonner Sphere Spectrometers (BSS). Both an active LiI(Eu) scintillator probe and passive gold foil detector were utilized to extend the energy response of the existing BSS. Above 20 MeV the energy structure for the standard polyethylene BSS are poor because the response functions are not unique. MCNPX was used to investigate several modifications to the BSS system which resulted in the Bonner Sphere Extension (BSE). This cost effective extension uses several concentric spheres of copper, lead, and tungsten heavy metal downscatter materials to extend the useful range of the current BSS from 20 MeV to above 1 GeV. Using both a 3" and 5" inner polyethylene spheres, aluminum shell sets were made with a 1" cavity and filled with the high Z materials for six total sets of spheres. a 12" and 8" polyethylene sphere were also milled to accept the heavy metal spheres. The system was validated at the Los Alamos Neutron Science Center (LANSCE) neutron beam. The system was calibrated at LANSCE for neutrons up to 800 MeV on target 4's 15 degree right flightpath (4FP15R) at 90 meters. Detailed models in MCNPX were made of the BSS, BSE and LANSCE facilities. Fine group responses were made and compared to the unfolded data from LANSCE. A vast improvement over the BSS system alone was seen with reasonable agreement with time of flight data measured at LANSCE and MCNPX calculated neutron spectra.

This thesis investigates the differences in Bonner Sphere detector response for anisotropic neutron fields as a function of borehole orientation. Monte Carlo simulations using MCNPX were used to calculate the difference for a borehole oriented directly behind a unidirectional neutron field and one in which the borehole is normal to the neutron flux. The differences in detector response depend on the size of the Bonner Sphere and the energy of the incident flux, which could introduce significant error in the determination of the neutron field’s energy spectrum.

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Ces travaux de thèse sont le fruit d’une collaboration entre le Laboratoire de Métrologie et Dosimétrie des Neutrons de l’Institut de Radioprotection et de Sûreté Nucléaire et le Département d’Environnement Spatial de l’Office National d’Etudes et Recherches Aérospatiales. L’objectif était de caractériser et de mettre en service un système opérationnel de spectrométrie des neutrons, étendu au domaine des hautes énergies afin de mesurer de manière dynamique les variations de l’environnement radiatif naturel atmosphérique en altitude au sommet de l’Observatoire du Pic du Midi de Bigorre dans les Pyrénées. Pour ce faire, les réponses des différents détecteurs ont été calculées par simulations Monte Carlo avant d’être validées expérimentalement jusqu’au domaine des hautes énergies en champs neutroniques de référence. La méthode de reconstruction mathématique du spectre par déconvolution a été étudiée afin de quantifier les incertitudes systématiques. Ensuite, le système a été testé sous la roche au Laboratoire Souterrain à Bas Bruit de Rustrel avant d’effectuer les premières mesures en altitude à +500 m et +1000 m. A la suite de ces expériences, le spectromètre a été installé en mai 2011 au sommet du Pic du Midi à +2885 m. La méthodologie d’analyse en continu des données recueillies a été développée. Des oscillations saisonnières du spectre dont l’amplitude dépend du domaine énergétique ont été mises en évidence. Des décroissances Forbush,caractéristiques d’éruptions solaires, ont également été observées à l’approche du 24ème cycle solaire.Des simulations Monte Carlo ont permis d’analyser ces résultats. Les données ont été valorisées grâce à des applications en dosimétrie personnelle et en fiabilité des composants électroniques vis-à-vis des radiations. / This PhD Thesis has been achieved thanks to the joint effort between two French organizations, the French Institute for Radiological Protection and Nuclear Safety (IRSN/LMDN, Cadarache) and the French Aerospace Lab (ONERA/ DESP, Toulouse). The aim was to develop an operational neutron spectrometer extended to high energies in order to measure the dynamics of the spectral variations of the natural radiative environment at the summit of the Pic du Midi Observatory in the French Pyrenees. Thereby, the fluence responses of each detector were calculated thanks to Monte Carlo simulations. Afterwards, they were validated by means of experimental campaigns up to high energies (>20 MeV) nearby reference neutron fields. The systematic uncertainties were deduced after detailed studies of the mathematic reconstruction of the spectra (i.e. unfolding procedure). Then, the system was tested under rocks at the LSBB of Rustrel before being installed at respectively+500 m and +1000 m above sea level for the first environmental campaigns. Finally, the spectrometer has been operating for two years after its deployment at the summit of the Pic du Midi (+2885 m). The continuous data were analysed thanks to an innovative method. Some seasonal and spectral variations were observed. Some Forbush decreases were also recorded after strong solar flares. These data were further analysed thanks to Monte Carlo simulations. The data were made more attractive thanks toseveral practical applications with personal dosimetry or reliability of submicron electronics components.