Ces dernières décennies ont vu apparaître de nombreuses innovations dans le domaine de la combustion afin de réduire la consommation et les émissions polluantes. De nouveaux types d'injecteur, de type LPP - Lean Premixed Prevaporized, ont été mis au point permettant de diminuer le rapport combustible/air et visent à pré-vaporiser le carburant en amont de la combustion afin de mieux le mélanger à l'air issu du compresseur. Cette architecture permet une amélioration de la consommation et des émissions polluantes, mais rend les foyers annulaires plus sensibles à des phénomènes instationnaires qui perturbent le fonctionnement du système, accroissent les flux de chaleur vers les parois de la chambre, induisent des vibrations de structures, entrainent une fatigue cyclique des pièces mécaniques et dans des cas extrêmes conduisent à des dommages irréversibles. L'objectif est de poursuivre l'effort engagé au laboratoire EM2C sur ce thème et plus particulièrement sur celui de la dynamique de la combustion dans les chambres annulaires. La thèse concerne plus spécialement le cas où l'injection du combustible s'effectue sous forme liquide. La configuration reproduit sous forme idéalisée celle que l'on trouve en pratique dans les moteurs aéronautiques. La chambre, désignée sous le nom de MICCA-Spray, est équipée de 16 injecteurs swirlés pouvant être alimentés par un combustible liquide ou gazeux, permettant ainsi une combustion diphasique ou prémélangée. Le système possède des parois en quartz donnant un accès optique à la zone de flamme. Il est aussi équipé d'un ensemble de diagnostics tels des microphones, des photomultiplicateurs ainsi que des systèmes d'imagerie à haute cadence. / These last decades have seen many innovations in the field of combustion to reduce fuel consumption and pollutant emissions. New types of injector, for example LPP - Lean Premixed Prevaporized, have then been developed to reduce the fuel / air ratio and aim to pre-vaporize the fuel upstream of the combustion in order to mix it better with the air coming from the compressor. Unfortunately this architecture makes annular chambers more sensitive to unsteady phenomena which disturb the functioning of the system, increase the heat flows towards the walls of the chamber, induce vibrations of structures, cause cyclic fatigue of mechanical parts and in extreme cases lead to irreversible damage. The objective of this thesis is to continue the effort undertaken at the EM2C laboratory on this topic and more particularly on the dynamics of combustion in annular chambers comprising a set of injectors. The thesis concerns more particularly the case where the injection of the fuel takes place in liquid form. This configuration reproduces, in idealized form, what can be found in practice in aeronautical engines. It is also a configuration studied at the fundamental level. The chamber, known as MICCA-Spray, is equipped with 16 swirled injectors that can be powered by liquid or gaseous fuel, thus enabling two-phase or fully premixed combustion. The system has quartz walls giving optical access to the flame zone. It is also equipped with a set of diagnostics such as microphones, photomultipliers and high-speed imaging systems.

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High-intensity pyrolysis, rapid heating in an inert gas atmosphere at up to 20 atm pressure, of 6 Australian coals was examined to gain further insight into high-intensity processes such as Integrated Gasification Combined Cycles (IGCC). Experiments focussed on pyrolysis in a specially developed Wire Mesh Reactor (WMR). The particle temperature lagged that of the mesh by 0.2 seconds at a heating rate of 100??~C s -1 and was predicted by modelling. This is part of the reason the volatile yield (VY) results for 10 s hold-time at ???b1.7 wt% daf of coal, is much more reproducible than 1 s hold-time experiments at ???b4.2 wt% daf of coal. Four coals of the same rank did not behave identically when heated. Three of the coals had a pyrolysis VY the same as the proximate VM when heated to 100??~C at 1 atm but the fourth, higher inertinite coal had a 1 atm pyrolysis VY 90% of its proximate VM. All four coals of similar rank had a significant decrease in VY, between 10 and 20 wt% daf of coal, with pressure increasing from 1 to 20 atm. The two lower rank coals showed less decrease in VY with increasing pressure than the higher rank and higher inertinite coals. The lower decrease in VY with increased pressure was mostly attributed to the lower inertinite levels for both the coals of similar rank and VM, and the coals of lower rank. Char characteristics examined focussed on pore Surface Area (SA). For high intensity WMR and Drop Tube Furnace (DTF) pyrolysis experiments CO2 SA for char from a particular coal was similar but the BET SA different. This was due to the char in the WMR experiments having longer to form larger pores determined by BET N2 SA. Both the N2 and CO2 SA was more than an order of magnitude greater than for low intensity pyrolysis char. This highlights that the WMR can be used to attain char with similar CO2 SA characteristics as other high intensity pyrolysis experiments and to provide a more meaningful insight into char reactivity than low intensity chars do.

Despite mounting concerns of looming global warming and fuel shortages, combustion will remain the predominant source of fulfilling the world’s ever-increasing demand for energy in the foreseeable future. In light of these issues, the combustion regime known as Moderate and Intense Low oxygen Dilution (MILD) combustion has the potential of offering increased efficiency whilst lowering pollutant emissions. Essentially, MILD combustion relies on the reuse of the exhaust gases from the combustion process to simultaneously dilute the oxygen concentration of the oxidant stream, and increase its temperature. The benefit of this technique is that it results in a vast reduction in emissions, especially oxides of nitrogen. In addition, the thermal efficiency of the combustion process is increased, reducing fuel demands, as well as producing a more uniform heating profile and subsequently better product quality for many applications. The recirculation of exhaust gas and heat has been utilised for applications in the past. MILD combustion aims to extend the advantages of heat recovery and exhaust gas recirculation beyond the boundaries that are otherwise possible using conventional techniques. The relatively new concept of MILD combustion is a major advancement to the previous technology, and many fundamental issues have not yet been resolved. In a furnace environment, the dilution and preheating of the reactants generate a unique “distributed” reaction zone. There is a need to better understand the structure of this combustion regime and the parameters which control it. To emulate MILD combustion conditions in a controlled experimental environment, a Jet in Hot Coflow (JHC) burner is used in this study. The MILD combustion regime is examined using laser diagnostic techniques. The two key flame intermediates hydroxyl radical (OH) and formaldehyde (H2CO), as well as temperature, are imaged simultaneously to reveal details relating to the reaction zone. Simultaneous imaging enables not only the spatial distribution of each scalar to be investigated, but also the combined effect of the interactions of the three measured scalars. The role of four key variables are investigated as part of this work, namely; the coflow oxygen (O2) level, the jet Reynolds number, fuel dilution and fuel type. Also considered is the effect of surrounding air entrainment into the hot and diluted coflow, which causes a deviation from MILD combustion conditions. The local oxygen (O2) concentration is a key parameter in the establishment of MILD combustion conditions. The effect of lowering the O2 level is to lead to reductions in the OH and temperature in the reaction zone, in effect leading to a less intense reaction. When comparatively high oxygen laden, cold surrounding air mixes with the hot and low O2 coflow, MILD combustion conditions no longer exist. In this case, the flame front can become locally extinguished and subsequent premixing with the high O2 concentrations can lead to increased reaction rates and hence higher temperatures. It is therefore essential that fresh air must be excluded from a MILD combustor to maintain the stable reaction which typifies MILD combustion. It is found that the flame structure is relatively insensitive to both the type of hydrocarbon fuel and the Reynolds number. Each of these parameters can lead to changes in some intermediate species, namely formaldehyde, yet the OH and temperature measurements show comparatively minor variation. Nevertheless, fuel type and Reynolds number, in the form of increased flow convolution, can lead to striking differences in the flame structure. One of the most prominent effects is noted with the dilution of the fuel with various diluents. Some of the flames visually appear lifted, whereas the measurements reveal the occurrence of pre-ignition reactions in the “lifted” region. The unique characteristics of the stabilisation for these particular cases has lead to the term transitional flames. The fundamental aspects discovered by this study shed new light on the reaction zone structure under MILD combustion conditions. By advancing understanding of MILD combustion, future combustion systems will be able to better utilise the efficiency increases and lower pollutant benefits it offers. / http://proxy.library.adelaide.edu.au/login?url= http://library.adelaide.edu.au/cgi-bin/Pwebrecon.cgi?BBID=1293788 / Thesis (Ph.D.) -- University of Adelaide, School of Mechanical Engineering, 2007.

Despite mounting concerns of looming global warming and fuel shortages, combustion will remain the predominant source of fulfilling the world’s ever-increasing demand for energy in the foreseeable future. In light of these issues, the combustion regime known as Moderate and Intense Low oxygen Dilution (MILD) combustion has the potential of offering increased efficiency whilst lowering pollutant emissions. Essentially, MILD combustion relies on the reuse of the exhaust gases from the combustion process to simultaneously dilute the oxygen concentration of the oxidant stream, and increase its temperature. The benefit of this technique is that it results in a vast reduction in emissions, especially oxides of nitrogen. In addition, the thermal efficiency of the combustion process is increased, reducing fuel demands, as well as producing a more uniform heating profile and subsequently better product quality for many applications. The recirculation of exhaust gas and heat has been utilised for applications in the past. MILD combustion aims to extend the advantages of heat recovery and exhaust gas recirculation beyond the boundaries that are otherwise possible using conventional techniques. The relatively new concept of MILD combustion is a major advancement to the previous technology, and many fundamental issues have not yet been resolved. In a furnace environment, the dilution and preheating of the reactants generate a unique “distributed” reaction zone. There is a need to better understand the structure of this combustion regime and the parameters which control it. To emulate MILD combustion conditions in a controlled experimental environment, a Jet in Hot Coflow (JHC) burner is used in this study. The MILD combustion regime is examined using laser diagnostic techniques. The two key flame intermediates hydroxyl radical (OH) and formaldehyde (H2CO), as well as temperature, are imaged simultaneously to reveal details relating to the reaction zone. Simultaneous imaging enables not only the spatial distribution of each scalar to be investigated, but also the combined effect of the interactions of the three measured scalars. The role of four key variables are investigated as part of this work, namely; the coflow oxygen (O2) level, the jet Reynolds number, fuel dilution and fuel type. Also considered is the effect of surrounding air entrainment into the hot and diluted coflow, which causes a deviation from MILD combustion conditions. The local oxygen (O2) concentration is a key parameter in the establishment of MILD combustion conditions. The effect of lowering the O2 level is to lead to reductions in the OH and temperature in the reaction zone, in effect leading to a less intense reaction. When comparatively high oxygen laden, cold surrounding air mixes with the hot and low O2 coflow, MILD combustion conditions no longer exist. In this case, the flame front can become locally extinguished and subsequent premixing with the high O2 concentrations can lead to increased reaction rates and hence higher temperatures. It is therefore essential that fresh air must be excluded from a MILD combustor to maintain the stable reaction which typifies MILD combustion. It is found that the flame structure is relatively insensitive to both the type of hydrocarbon fuel and the Reynolds number. Each of these parameters can lead to changes in some intermediate species, namely formaldehyde, yet the OH and temperature measurements show comparatively minor variation. Nevertheless, fuel type and Reynolds number, in the form of increased flow convolution, can lead to striking differences in the flame structure. One of the most prominent effects is noted with the dilution of the fuel with various diluents. Some of the flames visually appear lifted, whereas the measurements reveal the occurrence of pre-ignition reactions in the “lifted” region. The unique characteristics of the stabilisation for these particular cases has lead to the term transitional flames. The fundamental aspects discovered by this study shed new light on the reaction zone structure under MILD combustion conditions. By advancing understanding of MILD combustion, future combustion systems will be able to better utilise the efficiency increases and lower pollutant benefits it offers. / http://proxy.library.adelaide.edu.au/login?url= http://library.adelaide.edu.au/cgi-bin/Pwebrecon.cgi?BBID=1293788 / Thesis (Ph.D.) -- University of Adelaide, School of Mechanical Engineering, 2007.

Homogeneous Charge Compression Ignition (HCCI) is a promising method for combustion engines to provide a substantial reduction in fuel consumption and formation of both nitrogen oxides and soot pollutants in automotive and stationary engines. Control of HCCI combustion timing is essential for the successful integration of the HCCI concept in real applications. This thesis concentrates on control oriented modeling and experimental study of HCCI combustion for control of ignition timing in HCCI engines. A detailed experimental study of HCCI with over 600 operating points on two different engines is done to characterize the complex relationship among the engine variables, the ignition timing and the exhaust temperature. This leads to identifying regions with distinct patterns of cyclic variation for HCCI ignition timing. In addition, main influential factors on the variations of ignition timing and exhaust temperature in HCCI engines are determined. A dynamic full-cycle physics based Control Oriented Model(COM) is derived from using the experimental data and simulations from an HCCI thermo-kinetic model. The COM is validated with a large number of transient and steady-state experimental points. The validation results show that the COM captures the key HCCI dynamics with a high degree of accuracy for control applications. The COM is computationally efficient and all inputs of the model can be readily measured or estimated on a real engine. This makes the COM simple and fast enough for use as an off-line simulation bed to design and evaluate different strategies for physics-based control of combustion timing in HCCI engines.