With 663 million people still without access to an improved drinking water source, there is no room for complacency in the pursuit of Sustainable Development Goal (SDG) Target 6.1: “universal and equitable access to safe and affordable drinking water for all” by 2030 (WHO, 2017). All of the current efforts related to water supply service delivery will require continued enthusiasm in diligent implementation and thoughtful evaluation. This cannot be over-emphasized in relation to rural inhabitants of low-income countries (LICs), as they represent the largest percentage of those still reliant on unimproved drinking water sources. In that lies the motivation and value of this thesis research- improving water supply service delivery in LICs. Manually operated suction pumps, being relatively robust, low cost, and feasible to manufacture locally, are an important technology in providing access to improved drinking water sources in LICs, especially in the context of Self-supply. It seems widely accepted that the water-lifting limit of suction pumps as reported in practice is approximately seven meters. However, some observations by our research group of manually operated suction pumps lifting water upwards of nine meters brought this “general rule of thumb” limit into question. Therefore, a focused investigation on the capabilities of a manually operated suction pump (a Pitcher Pump) was conducted in an attempt to address these discrepancies, and in so doing, contribute to the understanding of this technology with the intent of providing results with practical relevance to its potential; that is, provide evidence that can inform the use of these pumps for water supply. In this research, a simple model based on commonly used engineering approaches employing empirical equations to describe head loss in a pump system was used to estimate the suction lift limit under presumed system parameters. Fundamentally based on the energy equation applied to incompressible flow in pipes, the empirically derived Darcy-Weisbach equation and Hydraulic Institute Standards acceleration head equation were used to estimate frictional and acceleration head losses. Considering the theoretical maximum suction lift is limited to the height of a column of water that would be supported by atmospheric pressure, reduced only by the vapor pressure of water, subtracting from this the model was used to predict the suction lift limit, also referred to herein as the practical theoretical limit, assuming a low (4 L/min) and high (11 L/min) flow rate for three systems: 1) one using 1.25-inch internal diameter GI pipes, 2) one using 1.25-inch internal diameter PVC pipes, and 3) one using 2-inch internal diameter PVC pipes. In all considered cases, with an elevation equal to sea level, the suction lift limit was estimated to be over nine meters. At a minimum, the suction lift limit was estimated to be approximately 9.4 meters for systems using 1.25-inch internal diameter pipe and 9.8 meters for systems using 2-inch internal diameter pipe, with essentially no discernable effects noticed between pipe material or pipe age. Additionally, laboratory (field) trials using a Simmons Manufacturing Picher Pump and each of the aforementioned pipe specifications were conducted at the University of South Florida (Tampa, FL, USA) to determine the practical pumping limit for these systems. Results from the pumping trials indicated that the practical pumping limit- the greatest height at which a reasonable pumping rate could be consistently sustained with only modest effort, as perceived by the person pumping- for a Pitcher Pump is around nine meters (9 meters when using 1.25-inch internal diameter GI or PVC pipe and 9.4 meters when using 2-inch internal diameter PVC pipe). Therefore, results from this research present two pieces of evidence which suggest that the practical water-lifting limit of manually operated suction pumps is somewhere around nine meters (at sea level), implying that reconsideration of the seven-meter suction lift limit commonly reported in the field might be warranted.

This thesis discusses rainwater harvesting systems (RWH systems). It particularly focuses on systems collecting rainwater for domestic consumption in rural areas of developing countries. The main aim of the thesis is to identify factors, which influence the willingness and ability of people to adopt and use properly these RWH systems. I began with a brief introduction into the topic of the good-quality drinking water scarcity and with a discussion of relevant information about the RWH systems. The method used for the research was a systematic review. The relevant literature was systematically searched, selected, evaluated, and the relevant material was then processed with regards to the importance of particular factors influencing the RWH systems adption and utilization. Altogether, 26 influential factors were identified and discussed.

Magister Public Health - MPH / Introduction: In-house contamination of drinking water stored in wide-mouthed buckets (even with lids) has been widely reported in epidemiologic investigations as vehicles for diarrhoea disease transmission. The long handled mukombe cup (LHM cup), recently developed by the National Institute of Health Research (NIHR), a department of the Ministry of Health and Child Care (MoHCC) in Zimbabwe, is a promising low cost dipping devise for extraction of water from wide-mouthed containers. Aim: The study aim was to assess the effectiveness and household acceptability of the long handled mukombe cup in reducing bacteriological contamination of drinking water stored in wide-mouthed vessels in the home in a peri urban settlement in Harare, Zimbabwe. Methodology: A randomised controlled trial of a long handled mukombe cup was conducted in Hatcliffe, Harare. After collecting baseline data on demographics, household water quality, and other sanitation and water handling practices, households were given basic health education before the two selected communities were randomly assigned to one of the two groups of 119 households each. The intervention group received the LHM cup while the control group received no intervention. Households were followed up after two months and assessed effectiveness and user acceptability of the intervention. Data Analysis: Data analysis was conducted using STATA 11. Descriptive statistics were calculated and reported as percentages, proportions, frequencies and measures of central tendency. Bivariate statistics were carried out to test independent associations between use of the LHM cup and E. coli. All analyses were conducted in an intention-to-intervene analysis. Results: A total of 230 households were analysed during follow-up. Samples of stored drinking water from intervention households were significantly lower in E. coli levels than those of control households (geometric mean E. coli of 0.8/100 ml vs 13.0/100 ml, p <0.0001). Overall, 78.4% (987/111) of samples from the intervention households met World Health Organization (WHO) guideline value of 0 cfu/100ml sample, while 52.1% of the 119 samples from control households met such a benchmark (p < 0.0001). In addition, 94.6% of intervention household samples were in compliance with this intervention or presented low risk, 27.7% of samples from control group households presented intermediate or high risk. There was a statistically significant association between LHM cup use and reduced E. coli bacterial contamination in stored drinking water (p < 0.05). There was no statistically significant difference in turbidity in both intervention and control groups, both for turbidity <5 and >5 (p = 0.071). Acceptability of the LHM cup was very high (100%). Conclusion: To our knowledge, this is the first study on the evaluation and acceptability of the LHM cup in the Sub-Saharan Africa. Positive results were recorded that showed that the LHM cup was effective in minimising E. coli contamination in the intervention group as compared to the control group. It is postulated that this is because the LHM cup reduces hand contact with stored water during scooping, thus maintaining improved water quality in communities in Zimbabwe that collect and store drinking water in wide-mouthed containers with lids where extraction is by scooping. However, more research is required to document the LHM cup's continued and effective use, durability and overall sustainability in the absence of any serious sampling or monitoring.

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M.Sc. / Drinking water treatment plants in South Africa rely almost entirely on surface water sources, which are often compromised due to high return flows and indirect reuse. The typical treatment plants focus on the removal of physical and microbial contaminants which include turbidity, colour, chemical compounds and micro-organisms. A relatively new alarm to this list is natural organic matter (NOM) which has become a major concern in potable water treatment due to its recent regulation. Conventionally, the drive to remove NOM from potable water would be the desire to remove colour from public water supplies. However, more problems in drinking water treatment associated with NOM have been recently identified. These include taste and odour, its tendency to foul membranes, interference with the removal of other contaminants and its potential to contribute to corrosion and slime growth in distribution systems. Moreover, it causes high demands for coagulants and disinfectants. The NOM is also the main precursor for disinfection by-products (DBPs) formed when it interacts with disinfectants such as chlorine during water disinfection. In this study, different raw water samples, of different NOM composition were collected from selected sources across the country and assessed for the removal of dissolved organic carbon (DOC) and UV absorbance at a wavelength of 254 nm (UV 254) using enhanced coagulation (EC). The efficacy of EC, which can be employed as a practical technology in the removal of both turbidity and NOM, was evaluated in these raw water sources. Jar tests were conducted with ferric chloride as the coagulant, and specific pH values were chosen as target values guiding the different coagulant dosages for the jar tests. The pH of the low-alkalinity (<60 mg/ℓ CaCO3) raw waters were adjusted and raised by the addition of sodium carbonate. Algorithms for finding the optimum coagulant dosage for both turbidity and UV 254 removal were developed and consistently applied to all the results in independent v batch tests, in which residual amounts of UV 254, DOC and turbidity were measured. The raw water parameters and results obtained from these tests were used to develop feed-forward multiplicative models predicting the performance of EC using ferric chloride. The results showed that the raw waters chosen were, indeed, representative of the different water types present in South Africa, and that the general water characteristics were affected by seasonal variations. The EC procedure developed was able to reduce turbidity to levels low enough for removal by subsequent treatment steps in the water treatment train. The residual UV 254 values were in all cases lower than 6 m-1, which theoretically corresponds to about 3.5 mg/ℓ DOC. This was confirmed by the residual DOC values which were found to be lower than 4 mg/ℓ. Generally, the waters of South Africa were found to be amenable to coagulation. In almost all cases, the costs for EC were comparable to those for conventional coagulation, hence EC could be employed as a NOM removal strategy in the South African context.

This research investigated using a life cycle environmental and economic approach to evaluate IX technology for small potable water systems, allowing for the identification and development of process and design improvements that reduce environmental impacts and costs. The main goals were to evaluate conventional IX in terms of life cycle environmental and economic sustainability, develop a method for improving designs of IX systems from a environmental and economic sustainability standpoint, evaluate potential design improvements, and make the research findings accessible to water professionals through user-friendly tools and frameworks that take into account their feedback. This research provides an understanding, from the perspective of life cycle environmental impacts and costs, of the tradeoffs between various reactor designs of IX, the effects of scale, key contributors to impact and cost, design trends that improve sustainability, and how combined cation anion exchange compares to conventional IX. Furthermore, tools were developed that can be used to identify design choices that improve sustainability of IX systems. These tools were made into a user-friendly format to better bridge the gap between research and practice.

A LLE-GC-MS method was developed to detect PPCPs in surface water samples from Big Cypress National Park, Everglades National Park and Biscayne National Park in South Florida. The most frequently found PPCPs were caffeine, DEET and triclosan with detected maximum concentration of 169 ng/L, 27.9 ng/L and 10.9 ng/L, respectively. The detection frequencies of hormones were less than PPCPs. Detected maximal concentrations of estrone, 17β-estradiol, coprostan-3-ol, coprostane and coprostan-3-one were 5.98 ng/L, 3.34 ng/L, 16.5 ng/L, 13.5 ng/L and 6.79 ng/L, respectively. An ASE-SPE-GC-MS method was developed and applied to the analysis of the sediment and soil area where reclaimed water was used for irrigation. Most analytes were below detection limits, even though some of analytes were detected in the reclaimed water at relatively high concentrations corroborating the fact that PPCPs do not significantly partition to mineral phases. An online SPE-HPLC-APPI-MS/MS method and an online SPE-HPLC-HESI-MS/MS method were developed to analyze reclaimed water and drinking water samples. In the reclaimed water study, reclaimed water samples were collected from the sprinkler for a year-long period at Florida International University Biscayne Bay Campus, where reclaimed water was reused for irrigation. Analysis results showed that several analytes were continuously detected in all reclaimed water samples. Coprostanol, bisphenol A and DEET’s maximum concentration exceeded 10 µg/L (ppb). The four most frequently detected compounds were diphenhydramine (100%), DEET (98%), atenolol (98%) and carbamazepine (96%). In the study of drinking water, 54 tap water samples were collected from the Miami-Dade area. The maximum concentrations of salicylic acid, ibuprofen and DEET were 521 ng/L, 301 ng/L and 290 ng/L, respectively. The three most frequently detected compounds were DEET (93%), carbamazepine (43%) and salicylic acid (37%), respectively. Because the source of drinking water in Miami-Dade County is the relatively pristine Biscayne aquifer, these findings suggest the presence of wastewater intrusions into the delivery system or the onset of direct influence of surface waters into the shallow aquifer.

Rainwater harvesting, the act of capturing and storing rain, is an ancient practice that is increasingly utilized today by communities to address water supply needs. This thesis examines whether domestic rainwater harvesting systems (DRWHS) can be a sustainable solution as defined by social, water quality, and technical feasibility for water security in semi-arid, rural environments. For this study, 50 surveys and 17 stored rainwater analyses were conducted in San Jose Xacxamayo, Mexico, in conjunction with my Peace Corps work of implementing 82 DRWHS. Results showed that all DRWHS were socially feasible because of cultural acceptance and local capacity. Water quality analyses showed that four DRWHS contained coliform bacteria; deeming water unfit for human consumption. Technical feasibility, examined through climate analyses, showed an average year-round reliability of 20-30% under current and future rainfall regime. The DRWHS can be a sustainable water supply option with roof expansion and treatment prior to consumption.

Water supply systems aim, among other objectives, to protect public health by reducing the concentration of, and potentially eliminating, microorganisms pathogenic to human beings. Yet, because water supply systems are engineered systems facing variable conditions, such as raw water quality or treatment process performance, the quality of the drinking water produced also exhibits variability. The reliability of a treatment system is defined in this context as the probability of producing drinking water that complies with existing microbial quality standards. This thesis examines the concept of reliability for two physicochemical treatment technologies, conventional rapid granular filtration and ultrafiltration, used to remove the protozoan pathogen Cryptosporidium parvum from drinking water. First, fault tree analysis is used as a method of identifying technical hazards related to the operation of these two technologies and to propose ways of minimizing the probability of failure of the systems. This method is used to compile operators’ knowledge into a single logical diagram and allows the identification of important processes which require efficient monitoring and maintenance practices. Second, an existing quantitative microbial risk assessment model is extended to be used in a reliability analysis. The extended model is used to quantify the reliability of the ultrafiltration system, for which performance is based on full-scale operational data, and to compare it with the reliability of rapid granular filtration systems, for which performance is based on previously published data. This method allows for a sound comparison of the reliability of the two technologies. Several issues remain to be addressed regarding the approaches used to quantify the different input variables of the model. The approaches proposed herein can be applied to other water treatment technologies, to aid in prioritizing interventions to improve system reliability at the operational level, and to determine the data needs for further refinements of the estimates of important variables. / Applied Science, Faculty of / Civil Engineering, Department of / Graduate

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