Organic semiconductors have recently been found to have a comparably large spin diffusion time and length. This makes them ideal candidates for spintronic devices. However, spin injection, transport and detection properties in organic materials have yet to be fully understood. This work studies spin injection from ferromagnets into organic semiconductors via spin pumping. Furthermore, work towards thermal spin injection, and detection is presented and discussed. The first part of this thesis comprises the spin pumping experiments. Measuring linewidth broadening of the microwave absorption at ferromagnetic resonance due to increase in effective Gilbert damping by spin pumping from a ferromagnetic substrate into an adjacent non-magnetic semiconductor allows us to quantify the spin-mixing conductance. This technique is employed to demonstrate spin injection from a ferromagnetic metal, permalloy (Ni81Fe19), into organic small molecules and conjugated polymers as well as to quantify the spin injection efficiency. The results highlight the importance of structural properties of organic semiconductors at the interface to permalloy. Significant suppression of spin injection due to alkyl side-chains separating the core of the small molecules from the interface is exemplary for this finding. Furthermore, the spin-mixing conductance depends very sensitively on the charge carrier density within a certain range of doping level. This suggests a strong link between spin injection efficiency and spin concentration in the organic semiconductor at the interface to permalloy. The second part of the thesis aims to explore spin caloritronic effects. We study spin injection into organic semiconductors by probing the spin Seebeck effect by making use of the inverse spin Hall effect for spin-to-charge conversion. Moreover, we present experimental work towards observation of a novel effect, the inverse spin Nernst effect, for thermal spin detection.

It has been recognized for some time that the very high fluence of fast (14.1MeV) neutrons produced by deuterium-tritium fusion will represent a major materials challenge for the development of next-generation fusion energy projects such as a fusion component test facility and demonstration fusion power reactor. The best-understood and most promising solutions presently available are a family of low-activation steels originally developed for use in fission reactors, but the ferromagnetic properties of these steels represent a danger to plasma confinement through enhancement of magnetohydrodynamic instabilities and increased susceptibility to error fields. At present, experimental research into the effects of ferromagnetic materials on MHD stability in toroidal geometry has been confined to demonstrating that it is still possible to operate an advanced tokamak in the presence of ferromagnetic components. In order to better quantify the effects of ferromagnetic materials on tokamak plasma stability, a new ferritic wall has been installated in the High Beta Tokamak—Extended Pulse (HBT-EP) device. The development, assembly, installation, and testing of this wall as a modular upgrade is described, and the effect of the wall on machine performance is characterized. Comparative studies of plasma dynamics with the ferritic wall close-fitting against similar plasmas with the ferritic wall retracted demonstrate substantial effects on plasma stability. Resonant magnetic perturbations (RMPs) are applied, demonstrating a 50% increase in n = 1 plasma response amplitude when the ferritic wall is near the plasma. Susceptibility of plasmas to disruption events increases by a factor of 2 or more with the ferritic wall inserted, as disruptions are observed earlier with greater frequency. Growth rates of external kink instabilities are observed to be twice as large in the presence of a close-fitting ferritic wall. Initial studies are made of the influence of mode rotation frequency on the ferritic effect, as well as observations of the effect of the ferritic wall on disruption halo currents.

An electron microscope with electrostatic lenses was used for high resolution studies of magnetic domains in thin iron films. Observation methods used to determine the directions of local magnetization in iron thin films were the Lorentz method and the Foucault method. We studied how Bloch line-crosstie pairs and crosstie main walls behave in applied, in-plane magnetic fields. We found that crosstie main walls remain unchanged until crosstie density goes nearly to zero when the field is applied perpendicular to the main wall. A twisted type of domain appears where crossties disappear.

Arthur F. Kip and Robert D. Arnold. / "December 21, 1948." / Includes bibliographical references. / Supported by the Army Signal Corps. W-36-039-sc-32037 102B Supported by the Dept. of the Army. 3-99-10-022

Charles Kittel. / "May 20, 1948." / Army Signal Corps Contract No. W-36-039 sc-32037. Contract OEMsr-262.

Electrical conductance in the ferromagnetic insulating (FMI) phase of manganites has been experimentally investigated. The investigations were performed on single crystals of compositions La0.82Ca0.18MnO3 and Nd0.7Pb0.3MnO3. The nature of electrical conductance is determined to be Shklovskii–Efros variable range hopping (SE–VRH). Further, at high bias levels, non–linear conductance (NLC) is observed. A “hot electron” model, that quantitatively explains the bias and temperature dependence of the NLC, consistent with the SE–VRH nature of electrical conductance, is presented. The limits of validity of the model are discussed.

We report an intriguing giant dielectric and magnetodielectric (MD) response on double perovskite Pr2CoMnO6(PCMO) system. The Arrhenius plot indicates that the origin of giant dielectric is internal barrier layer capacitance. Meanwhile, at the highest applied magnetic field 9T, the giant dielectric constant around Tm ~ 150 K is enhanced almost ~ 20% (at 10 kHz frequency) compared with that at zero field. The observed positive MD effect is considered to be associated with the direct consequence of negative magnetoresistance changes (~ -20% at 150 K) which was calculated by temperature dependent impedance spectras. Concomitantly, a pronounced ferromagnetic ordering is observed near Tc ~ 150 K coinciding with Tm of £`¡¬(T). These experimental results suggest that the magnetoresistive and MD effect response is very strongly by magnetic property of PCMO.

Thesis (Ph. D.)--University of California, San Diego, 2003. / Vita. Includes bibliographical references.

The primary goal of my dissertation was to build a Scanning Hall Probe Microscope (SHPM) for studying the domain structure of a ferromagnetic semiconductor (Ga[subscript 0.94]Mn[subscript 0.06]). This new semiconductor may be used in the emerging field of spintronics, where both the charge and spin of an electron are utilized. The first part of this dissertation introduces the scanning probe microscopy techniques that are used for our homemade SHPM performance test and images. In chapter 2, general spintronics and ferromagnetic semiconductor are introduced. A compact design of our LT-SHPM is introduced in chapter 3. A unique taper seal based on stainless steel and Cu for opening/closing the vacuum chamber is used for our homemade SHPM. In chapter 4, Hall probes are discussed. In this chapter, ESD (Electrostatic discharge) and its repair work are discussed. Finally, in Chapter 5, SHPM imaging results of Ga[subscript 0.94]Mn[subscript 0.06]As are discussed. We observed stripe domain patterns. We also observed the domain patterns as a function of magnetic field and temperature. / text

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