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COMPUTATIONAL DESIGN AND EXPERIMENTAL VALIDATION OF DIAMOND-BASED QUANTUM EMITTERSOluseye Akomolede (11706230) 15 November 2021 (has links)
<p>The enhancement of the emission from nitrogen vacancy color
centers will help facilitate advancements in quantum information technology. To
this end, the reduction of the excited state lifetimes of NVs as well as the
design of devices which support electroluminescence of nitrogen vacancies, as
well as the broadband enhancement of the emission from these centers is of
great importance.</p>
<p> </p>
<p>In this study, we create diamond thin films containing
nitrogen vacancy color centers using salt-assisted ultrasonic disaggregation
techniques and electrophoretic deposition. These films are implanted with xenon
atoms and the resulting structures are characterized optically. We report a
reduction in the bulk emission lifetime of nitrogen vacancy color centers of
two orders of magnitude. A coupled-mode theory approach is used to analyze the
emission from the xenon-doped nanodiamond species. It is determined that the
lifetime reduction occurs due to coupling between nitrogen vacancy color
centers and xenon color centers within the diamond lattice.</p>
<p> </p>
<p>A diamond field effect transistor is investigated via
simulations utilizing Sentaurus TCAD software. The device is scaled by three
orders of magnitude from previous experiments involving the same structure.
Transport characteristics are obtained from simulation results. We confirm the
existence of a decreasing saturation voltage with a decrease in gate length in
the diamond field effect transistor. Further investigation into the device’s
viability as a quantum emitter is conducted. </p>
<p> </p>
<p>The design of a single photon source utilizing plasmonic
structures to enhance emission from nitrogen vacancy color centers is proposed.
The plasmonic structure is investigated to extract operating parameters and to
quantify the optical coupling and propagation characteristics for various
physical dimensions</p>
<p> </p>
The design of a plasmonic device which features
both electroluminescence via nitrogen vacancy color centers and their
enhancement via plasmonic effects is numerically simulated. The device features
large Purcell enhancement factor and good photon emission rate. In summary,
this work paves the way towards the advancement of the nitrogen vacancy color center
as a stable source of room temperature photons for quantum information
applications.
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DIPOLE-DIPOLE INTERACTIONS IN ORDERED AND DISORDERED NANOPHOTONIC MEDIAThrinadha Ashwin Kumar Boddeti (16497417) 06 July 2023 (has links)
<p>Dipole-dipole interactions are ubiquitous fundamental physical phenomena that govern physical effects such as Casimir Forces, van der Waals forces, collective Lamb shifts, cooperative decay, and resonance energy transfer. These interactions are associated with real and virtual photon exchange between the interacting emitters. Such interactions are crucial in realizing quantum memories, novel super-radiant light sources, and light-harvesting devices. Owing to this, the control and modification of dipole-dipole interactions have been a longstanding theme. The electromagnetic environment plays a crucial role in enhancing the range and strength of the interactions. This work focuses on modifying the nanophotonic environment near interacting emitters to enhance dipole-dipole interactions instead of spontaneous emission. To this end, we focus on engineering the nanophotonic environment to enhance the strength and range of dipole-dipole interactions between an ensemble of emitters. We explore ordered and disordered nanophotonic structures. We experimentally demonstrate long-range dipole-dipole interactions mediated by surface lattice resonances in a periodic plasmonic nanoparticle lattice. Further, the modified electromagnetic environment reduces the apparent dimensionality of the interacting system compared to non-resonant in-homogeneous and homogeneous environments. We also develop a spectral domain inverse design technique for the accelerated discovery of disordered metamaterials with unique spectral features. </p>
<p>Further, we explore the novel regimes of light localization at near-zero-index in such disordered media. The disordered near-zero-index medium reveals enhanced localization and near-field chirality. This work paves the way to engineer the electromagnetic nanophotonic environment to realize enhanced long-range dipole-dipole interactions.</p>
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