Microplastics (MPs) constitute a risk to both human and environmental health. It is vital to identify sources and pathways to take the necessary action and limit the number of MPs in our environments. However, we currently have a limited understanding regarding MPs' variation with time in urban environments in an indoor setting. This knowledge gap is partly due to the absence of standard sampling procedures, and there is a need to develop reliable sampling techniques. This study evaluates the effectivity of a novel tape-lifting method developed for sampling MPs from various urban surfaces and applies this technique to measure weekly trends in artificial polymer deposition within an indoor environment at Umeå University. Two stone floor surfaces were sampled repeatedly on eight occasions over three weeks. Recovered MPs were identified in a microscope and categorized after shape: fibers or fragments. My developed tape-lifting method showed high MP recoveries (on average 100 ±4%) for the majority of the tested indoor surfaces (floors and tables). However, the method proved less functional for outdoor substrates (asphalt), where the recovery was significantly lower (on average, 48% ± 17). In my monitoring of MPs, I found that the deposition rate of fibers did not significantly differ between the two sampling sites or change over the three weeks. In contrast, MPs of fragment-type varied both between sampling sites and as a function of time. Here, the MP deposition rate was, on average, nearly two times higher at one of the sites, indicating substantial spatial variation. Regarding temporal variation, fragmented MPs showed an overall decrease in the number of deposited fragments over the three-week period. Interestingly the lack of variation in fibrous MPs indicates a dominating input source of fibers that is both homogenous for the room and static with time. In contrast, a specific source that is also time-sensitive appears to influence the dispersal pattern of fragmented MPs. My findings highlight the need to consider the temporal dimension of MP contamination and for research focusing on the relationship between fragmented MPs and their sources in indoor environments.

Le 36Cl est utilisé dans les études hydrologiques en raison de son caractère conservatif. Il apparaît cependant que le Cl- participe à un cycle biogéochimique complexe associé au turnover de la matière organique. Le flux de 36Cl atmosphérique a été déterminé (suivi mensuel des eaux de pluie sur deux ans) et varie saisonnièrement avec des valeurs accrues au printemps - été. L'importance de la période d'échantillonnage a été mise en évidence indiquant qu'une période de 6 mois est recommandée afin de lisser les variations saisonnières et les pics sporadiques du flux de 36Cl. Le flux atmosphérique moyen du 36Cl à notre site, constituant le flux d'entrée majoritaire dans son cycle biogéochimique, est de (75±6) atoms.m-2.s-1.La distribution du Cl et du 36Cl a été étudiée dans l’écosystème forestier grâce au développement des protocoles adéquats. 72% du Cl et 80% du 36Cl sont présents sous forme organique dans le sol alors qu'ils sont principalement sous forme inorganique dans la végétation. Les rapports mesurés dans la végétation (~ 200 x 10-15 at.at-1) sont similaires à ceux provenant des apports atmosphériques (~ 180 x 10-15 at.at-1) et ceux mesurés dans le sol sont un ordre de grandeur supérieur. Ces derniers augmentent significativement à 5-15 cm dans la fraction organique du profil de sol alors que dans la fraction inorganique une faible augmentation apparaît à 15-30 cm. Nous attribuons ces observations au recyclage du 36Cl du pic nucléaire des années 1950-1960. Ces résultats indiquent que la distribution du 36Cl diffère de celle du Cl suggérant des processus dynamiques d’immobilisation et de remobilisation du 36Cl liés au renouvellement de la matière organique. / 36Cl is widely used in hydrological studies since it is considered as a conservative tracer. However it appears that Cl- participates in a complex biogeochemical cycle linked to the organic matter turnover. The 36Cl atmospheric fallout rate has been determined (monthly record of rainwater samples during two years) and varies seasonally with higher values during spring – summer. The sampling period should at least span 6 months to avoid any biais in the fallout rate determination due to the monthly variations or any sporadic bursts of 36Cl. The mean 36Cl fallout rate at our site, corresponding to the main input of its biogeochemical cycle, equals (75±6) atoms.m-2.s-1. The distribution of Cl and 36Cl has been studied into the ecosystem thanks to the development of appropriate protocols.72% of the Cl and 80% of the 36Cl are contained in the organic fraction in soil while they are mainly in inorganic form in the vegetation. 36Cl/Cl measured in vegetation (~200 x 10-15 at.at-1) are within the range of the ones measured in the rainwater samples (~180 x 10-15 at.at-1), while the 36Cl/Cl ratios are 10 times higher in soil. 36Cl/Cl in soil increase significantly at a depth of 5-15 cm in the organic fraction while a slight increase is observed in the inorganic fraction at 15-30 cm deep. This suggests that 36Cl originating from the massive input of 36Cl introduced in the atmosphere more than 50 years as a consequence of nuclear tests, might still be recycling.These results emphasize that the distribution of 36Cl and Cl are not similar suggesting a possible occurrence of dynamic processes of 36Cl accumulation and release associated with the turnover of the organic matter.