High power thulium fiber lasers are useful for a number of applications in both continuous-wave and pulsed operating regimes. The use of thulium as a dopant has recently gained interest due to its large bandwidth, possibility of high efficiency, possibility of high power and long wavelength ~1.8 – 2.1 μm. The longer emission wavelength of Tm-doped fiber lasers compared to Yb- and/or Er-doped fiber lasers creates the possibility for higher peak power operation due to the larger nonlinear thresholds and reduced nonlinear phase accumulation. One primary interest in Tm-doped fiber lasers has been to scale to high average powers; however, the thermal and mechanical constraints of the fiber limit the average power out of a single-fiber aperture. One method to overcome the constraints of a single laser aperture is to spectrally combine the output from multiple lasers operating with different wavelengths into a single beam. In this thesis, results will be presented on the development of three polarized 100 W level laser systems that were wavelength stabilized for SBC. In addition to the development of the laser channels, the beams were combined using bandpass filters to achieve a single near diffraction-limited output. Concurrently, with the development of high average power systems there is an increasing interest in femotosecond pulse generation and amplification using Tm- doped fiber lasers. High peak power sources operating near 2 µm have the potential to be efficient pump sources to generate mid-infrared light through supercontinuum generation or optical parametric oscillators. This thesis focuses on the development of a laser system utilizing chirped pulse amplification (CPA) to achieve record level energies and peak powers for ultrashort pulses in Tm-doped fiber. iv A mode-locked oscillator was built to generate femtosecond pulses operating with pJ energy. Pulses generated in the mode-locked oscillator were limited to low energies and contained spectral modulation due to the mode-locking mechanism, therefore, a Raman-soliton self-frequency shift (Raman-SSFS) amplifier was built to amplify pulses, decrease the pulse duration, and spectrally clean pulses. These pulses were amplified using chirped pulse amplification (CPA) in which, limiting factors for amplification were examined and a high peak power system was built. The primary limiting factors of CPA in fibers include the nonlinear phase accumulation, primarily through self-phase modulation (SPM), and gain narrowing. Gain narrowing was examined by temporally stretching pulses in a highly nonlinear fiber that both stretched the pulse duration and broadened the spectrum. A high peak power CPA system amplified pulses to 1 µJ energy with 300 fs compressed pulses, corresponding to a peak power >3 MW. High peak power pulses were coupled into highly nonlinear fibers to generate supercontinuum

The thulium fiber laser has gained interest due to its long emission wavelength, large bandwidth (~1.8 – 2.1 µm), high efficiencies (~60 %), and high output power levels both in cw as well as pulsed regimes. Applications like remote sensing, machining, medical tissue ablation, and mid-infrared generation benefit from high peak power thulium laser sources. Pulsed thulium fiber laser systems are advancing rapidly towards higher peak power levels and are becoming the preferred sources for these applications. This dissertation work describes the development of novel nanosecond pulsed thulium fiber laser systems with record high peak power levels targeting mid-infrared generation. The peak power scaling in thulium fiber lasers requires new fiber designs with larger mode field area (MFA) than commercially available step index large mode area (SI-LMA) fibers. Two different prototypes of thulium doped photonic crystal fibers (PCF) were investigated for high peak power generation. The first prototype is a flexible-PCF with MFA twice as large as SILMA fiber and the second prototype is a PCF-rod with six times larger MFA. A robust single stage master oscillator power amplifier (MOPA) source based on flexible-PCF was developed. This source provided narrow linewidth, tunable wavelength, variable pulse duration, high peak power, and high energy nanosecond pulses. The PCF-rod was implemented as a second stage power amplifier. This system generated a record level of ~1 MW peak power output with 6.4 ns pulse-duration at 1 kHz repetition rate. This thulium doped PCF based MOPA system is a state of the art laser source providing high quality nanosecond pulses. iv The single stage MOPA system was successfully implemented to pump a zinc germanium phosphide (ZGP) crystal in an optical parametric oscillator (OPO) cavity to generate 3 - 5 µm wavelengths. The MOPA source was also used to demonstrate backside machining in silicon wafer. The PCF based laser system demonstrated an order of magnitude increase in the peak power achievable in nanosecond thulium doped fiber laser systems, and further scaling appears possible. The increase in peak power will enable additional capabilities for mid-infrared generation and associated applications.

High power thulium fiber lasers are interesting for a myriad of applications due to their potential for high average output power, excellent beam quality, compactness, portability, high operating efficiency and broad, eye-safe spectral range from 1.8-2.1 microns. Currently, the majority of thulium laser research effort is being invested into scaling average output powers; however, such output powers are being scaled with no degree of control on laser system output spectrum or temporal behavior. Thulium fiber laser technology is not useful for many of its most important applications without implementation of techniques enabling tunable, narrow spectral widths with appropriate pulse durations for particular applications. This work outlines several techniques for spectral control of thulium fiber lasers and investigates scaling of average laser powers while using these techniques to maintain a desired spectral output. In addition, an examination of operation in both nanosecond and picosecond pulsed regimes and scaling of average powers and pulse energies in these regimes to useful power levels is conducted. The demonstration of thulium fiber laser systems for applications in frequency conversion and spectral beam combination is also discussed. In addition to the experimental results, theoretical modeling of thulium fiber amplifier operation, simple thermal management analysis, as well as practical fiber and system design considerations for future power scaling are presented. Experimental and theoretical results of this work will enable the successful design of future extremely high power spectrally and temporally controlled thulium fiber laser systems.