A study of ground state binding energy values listed in the Atomic Mass Evaluation 2012 (AME2012) using an interpretive approach, as opposed to the exploratory methods of previous models, is presented. This model is based on a postulate requiring all protons to pair with available neutrons to form bound alpha clusters as the ground state for anN = Z core upon which excess neutrons are added. For each core, the trend of the binding energy as a function of excess neutrons in the isotopic chain can be fit with a three-term quadratic function. The quadratic parameter reveals a smooth decaying exponential function. By re-envisioning the determination of mass excess, the constant-term fit parameters, representing N = Z nuclei, reveal a near-symmetry around Z = 50. The linear fit parameters exhibit trends which are linear functions of core size. A neutron drip-line prediction is compared against current models. By considering the possibility of an alpha-cluster core, a new ground-state structure grouping scheme is presented; nucleon-nucleon pairing is shown to have a greater role in level filling. This model, referred to as the Alpha-Deuteron-Neutron Model, yields promising first results when considering root-mean-square variances from the AME2012. The beta-decay of the neutron-rich isotope 74Cu has been studied using three highpurity Germanium clover detectors at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory. A high-resolution mass separator greatly improved the purity of the 74Cu beam by removing isobaric contaminants, thus allowing decay through its isobar chain to the stable 74Ge at the center of the LeRIBSS detector array without any decay chain member dominating. Using coincidence gating techniques, 121 gamma-rays associated with 74Cu were isolated from the collective singles spectrum. Eighty-seven of these were placed in an expanded level scheme, and updated betaeeding level intensities and log(ft) values are presented based on multiple newly-placed excited states up to 6.8 MeV. The progression of simulated Total Absorption gamma-ray Spectroscopy (TAGS) based on known levels and beta feeding values from previous measurements to this evaluation are presented and demonstrate the need for a TAGS measurement of this isotope to gain a more complete understanding of its decay scheme.

The National Nuclear Data Center (NNDC) contains a compilation of information on the beta decays of Gallium isotopes. In the mass range A = 74 to 77, the Germanium daughters lie close to or at the valley of stability leading us to believe the decays would have been well studied. However, closer inspection indicates significant conflict for placement of gamma rays and energy levels between different measurements, especially for upper-lying states. Detailed beta-decay studies for the 74-77Ga isotopes were performed using a high resolution four clover Hyper-Pure Germanium (HPGe) detector system with two beta scintillators in the Holifield Radioactive Ion Beam Facility (HRIBF) at Oak Ridge National Lab (ORNL) to better understand the structure of the corresponding 74-77Ge daughter nuclei. In our experiments, use of a high-resolution mass separator greatly improved the purity of the samples in comparison to previous measurements. Besides that, the efficiency of the detector system we utilized was much higher than used in previous studies. We also established a method to determine statistically significant gamma gamma coincidence relationships to add reliability to the placement of gamma rays to energy levels and avoid experimental biases. From our analysis, we have established comprehensive decay schemes for all four Germanium nuclei in this study. In most cases, we have extended the energy levels to cover more of the energy window available for beta decay. Our proposed 74Ge decay scheme contains 44 energy levels occupying up to 4.36-MeV with the placement of 99 gamma rays. Similarly, 75Ga decay scheme contains 72 gamma rays with 29 energy levels occupying up to 2.75 MeV. The 76Ga decay scheme has 49 excited states with 100 gamma rays occupying up to 4.81 MeV. And, the 77Ge decay scheme has 68 gamma rays and 34 energy levels occupying up to 3.14 MeV. Based on the expanded level schemes, betaeeding intensity and log(ft) value lower limits were calculated and attempts were made to assign the spin-parity of the observed states. The resulting level schemes were then compared with the Nushellx theoretical predictions.

No description available.

The beta-decay interaction contains two terms which consist of invariant products of two scalars and two tensors respectively. The relative absolute magnitude of these two terms is fairly well established but there has been some controversy over their relative sign. In this thesis the form of the interaction is investigated by means of an analysis of the second-forbidden decay spectrum of Cs137 and it is concluded that the relative sign of the scalar and tensor terms is negative. / Thesis / Master of Science (MS)

SNO+ is a liquid scintillator experiment whose physics goals include measurements of solar neutrinos, reactor anti-neutrinos, geo neutrinos and double beta decay. During an initial water phase, it will also search for invisible modes of nucleon decay. This thesis investigates methods of improving the detector's sensitivity to the baryon and lepton violating processes of neutrinoless double beta decay and invisible nucleon decay. It does this through an improved scintillator model, allowing the sensitivity of the detector with different loading techniques to be evaluated, through a new background rejection technique, capable of increasing the active volume of the detector, and with the development of improved position fitters, achieving resolutions of approximately 10 cm in scintillator and 25 cm in water. The sensitivity of SNO+ to invisible modes of nucleon decay is explored, predicting, after one month of data, a limit of t > 1.38 x 10³⁰ years on the decay of neutrons and of t > 1.57 x 10³⁰ years on the decay of protons.

SuperNEMO est un projet de détecteur de nouvelle génération pour la recherche de la décroissance double bêta sans émission de neutrinos. La technique expérimental déployée est dans la lignée du son prédécesseur NEMO3, combinant un trajectographe et un calorimètre, afin d’identifier non seulement les électrons des décroissances double bêta, mais également pour mesurer l’ensemble des composantes de bruit de fond du détecteur. Le projet vise ainsi une sensibilité de 10^26 ans sur la période du 82Se, ce qui permettrait de sonder une masse effective du neutrino de 50 meV. Pour atteindre cette sensibilité, le projet prévoit notamment de mettre en place un calorimètre composé d’un millier de compteur à scintillation de basse radioactivité, dont la résolution en énergie serait meilleure que 8 % FWHM pour des électrons de 1 MeV.Ce travail de thèse apporte une contribution importante dans les travaux de Recherche et Développements pour améliorer les performances des scintillateurs et photomultiplicateurs, et pour réduire leur radioactivité, avec notamment la conception d’un nouveau photomultiplicateur en collaboration avec Photonis. / SuperNEMO is a next generation double beta decay experiment which will extend the successful “tracko-calo” technique employed in NEMO 3. The main characteristic of this type of detector is to identify not only double beta decays, but also to mesure its own background components. The projet aims to reach a sensitivity up to 1026 years on the half-life of 82Se. One of the main challenge of the Research and Development is to achieve an unprecedented energy resolution for the electron calorimeter, better than 8 % FWHM at 1 MeV.This thesis contributes to improve scintillators and photomultiplicators performances and reduce their radioactivity, including in particular the development of a new photomultiplier in collaboration with Photonis.

This Master thesis aims at designing, assembling and operating a prototypal luminescentbolometer containing a candidate with high Q-value (116Cd and 100Mo)for the study of the neutrinoless double- decay. The crystal is scintillating (with 116CdWO4 and Li2MoO4 compounds). The prototype is designed according to a simple thermal model and cooled down to 18 mK. Data analysis of the 116CdWO4 crystal determines the energy resolution (intrinsicand in the ROI) and the alpha/beta discrimination power. It includes a full interpretation of the background energy spectrum in terms of environmental radioactivity and an evaluation of the crystal radiopurity by the detection of internal contamination of the detector. An evaluation of the potential of a future experiment based on the 116CdWO4developed prototype is performed, ascertaining the feasibility of large scale experiments to search for neutrinoless double beta decay. The use of the thermal model of the detector response to interpret its bolometric behaviour and the study of future optimizations of the detector performance concludes this project.

[pt] Nesta dissertação, estudamos do ponto de vista fenomenológico, os efeitos de neutrinos estéreis para os observáveis de massas de neutrinos baseado nos dados do experimento LSND e nos resultados divulgados recentemente pela colaboração MiniBooNE. Consideramos observáveis de massa as seguintes quantidades: o parâmetro de massa cinemática cuja medida é realizada em experimentos com o decaimento beta do tritium tendo seu valor atual fornecido pelos experimentos Mainz e Troitsk; a massa efetiva de Majorana, que é uma quantidade que pode ser obtida em experimentos com o duplo decaimento beta sem neutrinos; finalmente, a soma de massas dos neutrinos, a qual é vinculada por dados cosmológicos. Nossa análise é realizada considerando os possíveis ordenamentos de massas para o caso em que temos dois neutrinos estéreis além dos três neutrinos ativos usuais, cuja adição é necessária para explicar os resultados de LSND e MiniBooNE ao mesmo tempo. Neste cenário, temos oito possíveis ordenamentos de massas, os quais dividimos em três grupos. No primeiro grupo, temos que os dois neutrinos estéreis são mais pesados que os três neutrinos ativos. No segundo grupo, os dois neutrinos estéreis são mais leves que os três neutrinos ativos. Cada um destes dois grupos tem possibilidades que dependem do ordenamento de massas dos neutrinos ativos que pode ser normal ou invertido. No terceiro e último grupo temos que um neutrino estéril é mais leve e o outro mais pesado que os três neutrinos ativos. Neste grupo, existem quatro possibilidades de ordenamento associada ao posicionamento dos neutrinos estéreis e ao ordenamento dos neutrinos do setor ativo. Investigamos os observáveis de massas em cada um destes cenários. / [en] In this dissertation we study, from the phenomenological point of view, the effects of sterile neutrinos for the observables related to neutrino masses based on the data of the LSND experiment and on the results releasedrecently by the MiniBooNE collaboration. We consider the following mass related obsevables: the kinematic mass parameter which is obtained in tritium beta decay experiments whose current value is provided by Mainzand Troitsk experiments; the Majorana effective mass, it is a quantity that can be obtained in neutrinoless double beta decay experiments. In additionto these quantities, we also consider the sum of neutrinos masses, which isconstrained by cosmological data. Our analysis is performed by considering the possible mass orderings for the cases where we have two sterile neutrinosbeyond the three standard active neutrinos, whose addition is necessary to explain the results of LSND andMiniBooNE simultaneously. In this scenariot here are eight possible mass orderings, which are divided into three groups.In the first group we have two sterile neutrinos which are heavier thanthe three active neutrinos. In the second group the two sterile neutrinosare lighter than the three active neutrinos. Each of these two groups canbe further divided into 2 subgroups depending on the mass ordering ofthe active neutrinos that can be normal or inverted. In the third and lastgroup we have one sterile neutrino lighter and the other heavier than thethree active neutrinos. In this group there are four possibilities of ordering depending on the positioning of the sterile neutrinos with respect to theactive ones and on the mass ordering of the active states. We investigate systematically the masses observable in each of these scenarios.

Neste trabalho foram estudados os níveis excitados do 193Ir produzidos a partir do decaimento β do 193Os (T1/2 ~ 30h). Para a obtenção das amostras radioativas, ~ 5mg de Ósmio metálico (99% enriquecido em 192Os) foram irradiados no reator IEA-R1, sob um fluxo de nêutrons da ordem de 1012cm2 s1 e depois analisadas, empregando-se a técnica de espectroscopia γ simples (unidimensional) com espectrômetro γ de alta resolução, bem como as técnicas de espectroscopia de coincidência γγ e de correlação angular direcional γγ (θ) usando um sistema de aquisição multiparamétrica composto por 4 detectores HPGe. A partir destes dados, foi possível adicionar 28 transições a este esquema de decaimento, 11 das quais já eram conhecidas de outros estudos envolvendo reações nucleares, além de 17 observadas pela primeira vez. Também foram acrescentados 8 níveis excitados ao esquema de decaimento, sendo 3 conhecidos por outras reações e 5 completamente novos. Além disso, foi possível confirmar a suspeita encontrada na literatura de que os níveis a 848,93keV e 849,093keV são o mesmo, além de confirmar a existência de um nível excitado a 806,9keV. A análise de correlação angular direcional permitiu a definição do spin de do nível excitado a 874kev (5/2+), além de propor uma probabilidade de 79% do nível a 1078keV ter spin 5/2, e de restringir as possibilidades de spin para o nível novo a 960keV para duas (1/2 ou 3/2). Também foi possível determinar a razão de mistura multipolar (δLn+1/Ln) para 43 transições, sendo 19 pela primeira vez e praticamente todas as restantes com precisão melhor que a encontrada na literatura. Finalmente, foi feita uma tentativa de compreender o núcleo através de um modelo teórico, o qual reproduziu muito bem o estado fundamental e os dois primeiros estados excitados do 193Ir. / In this work, the excited levels of 193Ir populated by the β decay of 193Os (T1/2 30h) were investigated. For that purpose, 5mg samples of 99%-enriched 192Os were irradiated under a thermal neutron flux of 1012s1 and then analysed both using single gamma spectroscopy and a 4-detector multiparametric acquisition facility, which provided data for both a γγ coincidence analysis and a directional angular correlation γγ (θ) study. From these data, 28 transitions were added to this decay scheme, 11 of which were previously known from nuclear reactions and 17 observed for the first time. Eight excited levels were also added to the decay scheme, 3 of which were known from nuclear reaction studies the remaining 5 are suggested for the first time. Moreover, it was possible to confirm suspicions found in reference that the levels at 848.93keV and 849.093keV are indeed the same; it was also possible to confirm the existence of an excited level at 806.9keV, which had been inferred, but not experimentally confirmed in β decay studies to date. The angular correlation analysis allowed for the definition of the spin of the excited level at 874keV as 5/2+; moreover, the results showed a 79% probability that the spin of the 1078keV level is 5/2, and also restricted the spin possibilities for the new excited level at 960keV to two values (1/2 or 3/2). It was also possible to measure the multipolarity mixing ratio (δLn+1/Ln) for 43 transitions 19 of them for the first time and most of the others with a better precision than previously known. Finally, an attempt was made to understand the low-lying levels structure for this nucleus using a theoretical model, which reproduced the ground state and the two lowest-lying excited levels in 193Ir.

L’observation de la double désintégration bêta sans neutrinos (0ν2β) impliquerait la violation de la conservation du numéro leptonique, signe d’une nouvelle physique au-delà du Modèle Standard, et permettrait d’établir la nature de Majorana des neutrinos. Les bolomètres scintillants cryogéniques sont parmi les détecteurs les plus prometteurs pour rechercher ce processus nucléaire extrêmement rare dans des noyaux qui sont théoriquement entre les plus favorables.Des scintillateurs de ZnMoO₄ ayant une masse de ∼ 0.3 kg, ainsi que des cristaux de Zn¹⁰⁰ MoO₄ enrichi dans l’isotope ¹⁰⁰Mo, ont été produits pour la première fois en utilisant la technique de Czochralski à faible gradient thermique. Les propriétés optiques et de luminescence des cristaux produits ont été étudiées pour évaluer le progrès de la qualité de la croissance des cristaux. Des tests à basse température avec un scintillateur de 313 g de ZnMoO₄et deux scintillateurs de Zn¹⁰⁰ MoO₄ enrichis ont été réalisées en surface au Centre de Sciences Nucléaires et de Sciences de la Matière. On a aussi mené des mesures à faible fond radioactif avec trois cristaux de ZnMoO₄ naturels et deux détecteurs enrichis, installés dans le setup d’ EDELWEISS au Laboratoire Souterrain de Modane.Pour optimiser la collecte de la lumière dans des bolomètres scintillants cryogénique de ZnMoO₄, nous avons simulé par une méthode Monte Carlo la collecte des photons de scintillation dans un module de détection pour différentes géométries, en utilisant le logiciel GEANT4. La réponse à la désintégration 2ν2β de ¹⁰⁰Mo a été simulée pour des détecteurs enrichis de Zn¹⁰⁰ MoO₄ avec forme et masse différente, avec le but de comprendre la structure des spectres 2ν2β en fonctionne de la forme des cristaux. Nous avons simulé aussi la performance de 48 cristaux de Zn¹⁰⁰ MoO₄ ayant une taille de Ø60 × 40 mm et installés dans le cryostat d’EDELWEISS. La contribution au fond de la contamination radioactive interne des cristaux, l’activation cosmogénique et la contamination radioactive du setup ont été simulées.Tenant compte de la modeste résolution temporelle des bolomètres à basse température, nous avons également étudié la contribution au fond à l'énergie Q₂β déterminé par des coïncidences aléatoires de signaux, en particulier du à la décroissance 2ν2β, qui est l'une des sources de fond les plus dangereuses dans les bolomètres cryogéniques. Des méthodes pour le rejet d’événements coïncidant par hasard ont été développées et comparées. Nous avons également analysé la dépendance de l'efficacité de rejet à l’égard des performances du détecteur cryogénique. / Observation of neutrinoless double beta (0ν2β) decay would imply the violation of lepton number conservation and definitely new physics beyond the Standard Model, establishing the Majorana nature of neutrinos. Cryogenic scintillating bolometers look the most promising detectors to search for this extremely rare nuclear process in a few theoretically the most favorable nuclei.ZnMoO₄ scintillators with a mass of ∼ 0.3 kg, as well as Zn¹⁰⁰ MoO₄ crystals enriched in the isotope ¹⁰⁰Mo were produced for the first time by using the low-thermal-gradient Czochralski technique. The optical and luminescent properties of the produced crystals were studied to estimate the progress in crystal growth quality. The low-temperature tests with a 313 g ZnMoO₄ scintillator and two enriched Zn¹⁰⁰ MoO₄ were performed aboveground in the Centre de Sciences Nucléaires et de Sciences de la Matière. The low background measurements with a three ZnMoO₄ and two enriched detectors installed in the EDELWEISS set-up at the Laboratoire Souterrain de Modane were carried out.To optimize the light collection in ZnMoO₄ cryogenic scintillating bolometers, we have simulated the collection of scintillation photons in a detector module for different geometries by Monte Carlo method using the GEANT4 package. Response to the 2ν2β decay of ¹⁰⁰Mo was simulated for the enriched Zn¹⁰⁰ MoO₄ detectors of different shape and mass to understand the dependence of 2ν2β decay spectra on crystal shape. We have simulated 48 Zn¹⁰⁰ MoO₄ crystals with a size of Ø60 × 40 mm installed in the EDELWEISS cryostat. The contribution to background from the internal radioactive contamination of the crystals, cosmogenic activation and radioactive contamination of the set-up were simulated.Taking into account the poor time resolution of the low temperature bolometers, we also studied contribution to background at the Q₂β energy of random coincidences of signals, in particular of 2ν2β decay, which is one of the most valuable sources of background in cryogenic bolometers. Methods of the randomly coinciding events rejection were developed and compared. We have also analyzed dependence of the rejection efficiency on a cryogenic detector performance.