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Le détecteur NEMO3 a été mis en place au Laboratoire Souterrain de Modane, en 2003, afin de rechercher la décroissance double bêta sans émission de neutrinos (ββ0v). La particularité de cette expérience est d’avoir pu étudier plusieurs isotopes dont le 100Mo, le 82Se, le 96Zr ou le 150Nd. En plus d’avoir placé les meilleures limites sur la demi-vie du processus ββ0v pour ces isotopes, ce détecteur a permis des mesures compétitives de leurs désintégrations ββ2v. Le premier objectif de ce travail a été de mesurer les temps de demi-vie des décroissances ββ2v et ββ0v du 82Se vers l’état excité 0+2 du 82Kr grâce aux données de NEMO3. Ces processus n’ayant pas été observés, seules des limites ont été calculées. Les résultats obtenus pour les deux décroissances sont donc T2 1=2(82Se; 0+1 → 0+2) > 1,29 x 1021 ans et T01=2(82Se; 0+1→ 0+2) > 2,31 x 1022 ans, ce dernier étant la première limite sur cette décroissance. SuperNEMO, successeur de NEMO3, cherchera à atteindre une sensibilité de 1026 ans sur la demivie de la décroissance ββ0v du 82Se. Le Radon étant une source de bruit de fond pour la recherche de cette décroissance, sa concentration dans le détecteur doit être inférieure à 0,15 mBq.m-3. Pour parvenir à un tel niveau, l’émanation de Radon des composants de SuperNEMO doit être contrôlée.Le second objectif de cette thèse a donc été de développer deux dispositifs de mesure d’émanation de Radon. Ces deux systèmes, consistants chacun en une chambre d’émanation associée à un détecteur électrostatique, ont par la suite été étalonnés puis leurs bruits de fond ont été caractérisés. Grâce à leurs sensibilités de quelques mBq.m-3, ces dispositifs ont permis de mesurer les taux d’émanation de Radon de plusieurs matériaux destinés à la construction du détecteur SuperNEMO. / The NEMO3 detector was installed in the Laboratoire Souterrain de Modane, in 2003, in orderto search for neutrinoless double beta decay (ββ0v). The specificity of this experiment was the possibility to study several isotopes simultaneously. Among them were 100Mo, 82Se, 96Zr or 150Nd. In addition to setting the best limits on these isotopes half-lives for theββ 0v process, the detector performed precise measurements of their 2v ββdecays. The first point of this work was to measure the half-lives of 2v ββand 0v ββdecays of 82Se to the 0+2 excited state of 82Kr using NEMO3 data. Since those processes have not been observed, only limits were set. The resulting half-life limits are T2 1=2(82Se; 0+1 → 0+2) > 1:29 x 1021 yr and T01=2(82Se; 0+1 → 0+2) > 2:31 x 1022 yr. The latest is the first limit ever measured for this decay. SuperNEMO is the successor to NEMO3 and will aim to reach an half-life sensitivity of 1026 yr for the 0v ββdecay of 82Se. Radon being a source of background for the search of this decay, its concentration inside the detector must be less than 0:15 mBq.m-3. To reach this objective, Radon emanation from the detector componants has to be checked. The second goal of this thesis was thus to develop two setups able to measure Radon emanation. Those two devices, each consisting of an emanation chamber associated to an electrostatic detector, were calibrated before their backgrounds were characterized. With a sensitivity of a few mBq.m-3, these setups measured the Radon emanation rate of several materials which will be used for the construction of the SuperNEMO detector.

The inference of massive neutrino states through the observation of flavor oscillations boosted the importance of direct and indirect mass searches, including the search for the hypothesized neutrinoless double beta decay (0νββ-decay). Nowadays, the search for this ultra-rare nuclear transition is one of the most active research fields at the intersection of nuclear, particle and astroparticle physics. Its main and evident feature is the explicit violation of the total lepton number, which is an accidentally conserved quantity in the Standard Model of particle physics, and would prove the Majorana nature of neutrinos. This, in turn, would support the theoretical explanation of the origin of the observed baryon asymmetry in the universe through the process of leptogenisis and could shed light on the role of neutrinos in the early universe’s structure formation. For the theoretical description of the 0νββ-decay, nuclear structure effects play an important role as they may affect considerably the decay rate. These nuclear effects are summarized as the nuclear matrix elements (NMEs), containing information about the initial and final states of the involved atomic nuclei and the decay mechanism. Under the assumption of light Majorana neutrino exchange, the inverse half-life is proportional to the effective Majorana neutrino mass, a kinematic phase-space factor, the involved NMEs and the fourth power of the weak axial-vector coupling gA. The search for the 0νββ-decay is driven by experiments and an accurate description of the nuclear structure effects is essential to estimate the required sensitivity to cover a certain mass range. In order to match theoretical calculations and the results of β-decay and ββ-decay studies, there is a scientific discussion regarding quenching effects of gA in nuclear media. Different methods are being investigated to determine an effective gA at the energy scale of nuclear transitions. One of those recently proposed methods exploits the dependency of the spectrum-shape of highly forbidden β-decays on gA. An ideal candidate for such an investigation is the fourfold forbidden non-unique β-decay of Cd-113, which is the most prominent signal in the current stage of the COBRA experiment searching for 0νββ-decays with cadmium zinc telluride (CZT) solid state detectors. The detector material CZT acts as a semiconductor at room temperature and contains intrinsically several candidates for rare nuclear transitions. The experiment is located at the LNGS underground facility in Italy, which is shielded against cosmic rays by a mean rock coverage of about 1400 m. In the present demonstrator phase, it consists of 64 coplanar grid (CPG) detectors that are arranged in four layers of 4 x 4 crystals. In the scope of this thesis, conventional and novel prototype CPG-CZT detectors, which are the basis for an anticipated large-scale experiment, are characterized by evaluating homogeneous and localized γ-ray irradiation measurements. Moreover, a novel pulse-shape discrimination (PSD) technique is established, optimized and applied in the analysis of the physics data obtained with the demonstrator array. The PSD optimization is complemented by dedicated laboratory measurements with the aim to create a pulseshape library of signal-like single-site events and high-energy cosmic muon interactions for which an analytic reconstruction model has been developed. For the first time, the COBRA demonstrator’s full exposure from Sept.’11 to Nov.’19 is analyzed, including a detailed background characterization as well as an automatized data partitioning to identify periods with increased backgrounds. The main subject is the study of the Cd-113 β-decay’s spectrum-shape to address the quenching of gA in lowmomentum exchange nuclear processes. The analysis of the experimental data is carried out in the context of three nuclear frameworks and confirms the idea of a significantly quenched gA. Furthermore, the data are analyzed with respect to the 2νββ-decay of Cd-116 and the long-lived α-decay of Pt-190 as a localized contaminant in the CZT detectors’ electrode metalization. Finally, the prospects of a search for excited state transitions of the ββ-nuclides Cd-116 and Te-130 are studied with elaborate Monte-Carlo simulations. The analysis section is concluded with an estimate of the achievable 0νββ-decay half-life sensitivity for multiple ββ-nuclides given the full exposure of the COBRA demonstrator and the recently achieved upgrade to the COBRA eXtended DEMonstrator (XDEM).

The Cadmium-Zinc-Telluride 0-Neutrino-Double-Beta Research Apparatus (COBRA-Experiment) investigates the theoretically predicted neutrinoless double beta decay (0νββ-decay) to indirectly determine the effective Ma- jorana mass of the electron-neutrino by a measurement of the half-life of the 0νββ-decay using room-temperature semiconducting Cadmium-Zinc- Telluride-detectors (CZT). The detectors are made of elements containing several isotopes that decay via double beta decay (ββ-decay). In such a con- figuration the detector itself becomes the source of the decay and, hence, the efficiency for the detection of such events rises. This work covers the investigations and characterizations made on the CZT detectors used in the COBRA-Experiment, currently running. Prior to in- stallation the physical properties of the detectors are analyzed and during operation the stability of the detectors is monitored. For the laboratory analysis three dedicated setups are developed that allow for detailed inves- tigations of different properties of the detectors. Beside the working point determination and the analysis of the temperature dependence of the de- tector performance, the spatial detector response to localized irradiation is analyzed and a setup to generate a library of specific pulse shapes is designed and operated. Furthermore, an investigation for a possible discrimination of α- and β-decay events based on pulse shape discrimination is performed as well as an analysis of the long term stability of underground operated CZT detectors.

Experiments with polarized "ultracold neutrons" (UCN) offer a new way to measure the decay correlations of neutron beta decay; these correlations can be used to test the completeness of the Standard Model and predict physics beyond it. Ultracold neutrons are very low energy neutrons that can be trapped inside of material and magnetic bottles. The decay correlations in combination with the neutron and muon lifetimes experimentally find the first element (Vud) of the Cabibbo-Kobayashi-Maskawa (CKM) quark mixing matrix. The CKM matrix is a unitary transform between the mass and weak eigenstates of the d, s and b quarks; if the matrix is not unitary this would imply that the Standard Model is not complete. Currently the first row of the CKM matrix is over 2 sigma from unitarity and Vud is the largest component of the row. The UCNA experiment looks at the correlation between the polarization of the neutron and the momentum of the electron resulting from the beta decay of the neutron (the A-correlation). The keys to making a high precision measurement of A-correlation are a near 100% polarization of the neutrons that decay, low"backscatter electron detectors, and small, well characterized backgrounds. UCN can be 100% polarized by passing them through a seven Telsa magnetic field. The key to the UCNA experiment is keeping them polarized until they decay or are lost. This dissertation covers the development of guides that are minimally depolarizing and efficient transporters of UCN and their use in the UCNA experiment. The entire guide development process is covered from conception to manufacturing and testing. This process includes development of a pulsed laser deposition, diamond-like carbon coating system and materials studies of the resulting coatings. After the initial studies of the guide coating, meter"long sections of guide are tested with UCN to determine their depolarization and transport properties. The guide technology developed in this dissertation has been used in the entire UCNA experiment. Also, this technology is currently the state of the art for polarized and non-polarized UCN guide systems and it is being implemented in several new UCN experiments. / Ph. D.