The development of compact and low-cost coherent sources in visible and infrared wavelength range can provide indispensible tools for a variety of scientific, technological and industrial applications. Great progress over the last years in material science, crystal growth and semiconductor material processing in combination with recent advances in some of the more traditional technologies, in particular nonlinear frequency conversion and parametric sources, have led to the realisation of a new generation of laser sources. Furthermore, the advent of a new generation of quasi-phase-matched, waveguided and semiconductor nonlinear materials together with novel semiconductor lasers have led to the development of new frequency conversion and parametric sources with previously unattainable performance capabilities. The research described in this thesis relates to the development and characterisation of novel semiconductor based laser sources tunable in the broad spectral ranges which are unattainable for conventional lasers due to a lack of suitable laser gain materials. In the first part of the thesis the subject matter is concerned with the direct emission from laser devices. In particular, a broadly tunable InGaAs/InP strained multi-quantum well external cavity diode laser, operating in the spectral range of 1494 nm – 1667 nm with a maximum CW output power in excess of 81 mW and side-mode suppression ratio higher than 50 dB is demonstrated. This represents the highest output power and side-mode suppression ratio ever to be generated in this spectral region. A record broadly tunable high-power external cavity InAs/GaAs quantum-dot diode laser with a tuning range of 202 nm (1122 nm - 1324 nm), a maximum output power of 480 mW and a side-mode suppression ratio greater than 45 dB, is also demonstrated. This represents a promising achievement for the development of a high-power fast swept tunable laser and compact nonlinear frequency generation schemes for the green-yellow-orange-red spectral range. The second part of the thesis relates to induced nonlinear processes, focusing on frequency doubling and optical parametric oscillation. In particular, an all-room-temperature CW second harmonic generation at 612.9 nm and 591.5 nm in periodically poled potassium titanyl phosphate waveguides pumped by a broadly-tunable quantum-dot external cavity diode laser with a conversion efficiency of 10.5% and 7.9%, respectively, is demonstrated. For the first time, a green-to-red tunable laser source with tunability of over 60 nm (567.7 nm – 629.1 nm) based on frequency doubling in a single periodically poled potassium titanyl phosphate waveguide pumped by a single broadly-tunable quantum dot laser is demonstrated. These results are an important step towards a compact tunable coherent visible light source, operating at room temperature. The possibility of nonlinear frequency conversion in orientation-patterned GaAs waveguides is also investigated. The technology of low-loss periodically poled GaAs waveguided crystals is developed and such crystals are fabricated. Second harmonic generation at 1621 nm in low-loss periodically poled GaAs waveguide is demonstrated. An optical parametric oscillator system used as the pump source for GaAs devices and based on the periodically poled 5 mol% MgO-doped Congruent Lithium Niobate crystal, generating light in the wavelength range between 1430 nm and 4157 nm, is presented. The obtained results show a great promise for realisation of efficient quasi-phase-matched optical parametric oscillator devices based on orientation-patterned GaAs waveguides, which enables the extending generated wavelength up to 16 µm.

In this thesis, the spectral behavior of the fundamental and sum-frequency waves, generated from the surface of a thin metal film in the Kretschmann configuration, is theoretically studied with coherent ultrashort pulses. As a first exploration of considering spectral response in nonlinear plasmonics, it is shown that the spectra of reflected sum-frequency waves exhibit pronounced shifts for the incident fundamental waves close to the plasmon coupling angle, whereas meanwhile those of reflected fundamental waves display energy holes. We also demonstrate that the scale of discovered plasmon-enhanced spectral changes is strongly influenced by the magnitude of the incidentce angle and the source pulse duration, and at a certain angle a spectral switch is observed. The appearance of large sum-frequency wave shifts can serve as an unambiguous plasmon signatur in nonlinear surface spectroscopy. Also, the discovered spectral switch can trigger extremely surface-sensitive nonlinear plasmonic sensors.

Interference has long been used for precision measurement of path-length changes. Since the advent of the laser, interference has become one of the most versatile tools in metrology. Specifically, ultra-short laser pulses allow unprecedented resolution in absolute length measurements. While ultra-short laser pulses lead to high resolution, for example in white-light interferometry, they are very susceptible to dispersion. Quantum resources have been proposed to overcome some of the problems related to distortions in the interferometric signal. For example, the Hong-Ou-Mandel (HOM) interferometer relies on frequency-entangled photon pairs and features automatic even-order dispersion cancellation and high interference visibility resilient to unbalanced loss. Quantum-OCT is a technique based on HOM interferometry, that promises to overcome Optical Coherence Tomography (OCT) a classical imaging technique based on low coherence light. Furthermore, straightforward modifications of the HOM interferometer can display several different interferometric signals, including the HOM peak, quantum beating, and phase super-resolution. However, the quantum resources required are hard to produce and dim, leading to long integration times and single-photon counting. In this thesis, we introduce the theory behind Chirped-Pulse Interferometry (CPI), a new technique that combines all the advantages of Q-OCT, including even-order dispersion cancellation, but without the need for any quantum resources. We then experimentally implement CPI and demonstrate all the important characteristics shared by the HOM interferometer, but at dramatically larger signal levels. We show how CPI can be used to measure dispersion cancelled axial profiles of an optical sample and show the improvement in resolution over white-light interferometry. Finally, we show that by modifying CPI in analogous ways to HOM, CPI can also be made to produce interferometric signal identical to the HOM peak, quantum beating, and phase super-resolution.

Interference has long been used for precision measurement of path-length changes. Since the advent of the laser, interference has become one of the most versatile tools in metrology. Specifically, ultra-short laser pulses allow unprecedented resolution in absolute length measurements. While ultra-short laser pulses lead to high resolution, for example in white-light interferometry, they are very susceptible to dispersion. Quantum resources have been proposed to overcome some of the problems related to distortions in the interferometric signal. For example, the Hong-Ou-Mandel (HOM) interferometer relies on frequency-entangled photon pairs and features automatic even-order dispersion cancellation and high interference visibility resilient to unbalanced loss. Quantum-OCT is a technique based on HOM interferometry, that promises to overcome Optical Coherence Tomography (OCT) a classical imaging technique based on low coherence light. Furthermore, straightforward modifications of the HOM interferometer can display several different interferometric signals, including the HOM peak, quantum beating, and phase super-resolution. However, the quantum resources required are hard to produce and dim, leading to long integration times and single-photon counting. In this thesis, we introduce the theory behind Chirped-Pulse Interferometry (CPI), a new technique that combines all the advantages of Q-OCT, including even-order dispersion cancellation, but without the need for any quantum resources. We then experimentally implement CPI and demonstrate all the important characteristics shared by the HOM interferometer, but at dramatically larger signal levels. We show how CPI can be used to measure dispersion cancelled axial profiles of an optical sample and show the improvement in resolution over white-light interferometry. Finally, we show that by modifying CPI in analogous ways to HOM, CPI can also be made to produce interferometric signal identical to the HOM peak, quantum beating, and phase super-resolution.

This thesis contains two major components of research: numerical simulation of optical-parametric amplification cross correlation of Frequency-Resolved Optical Gating (OPA-XFROG) and numerical simulation of GRENOUILLE and its related issues. Recently, an extremely sensitive technique--OPA-XFROG has been developed. A short pump pulse serves as the gate by parametrically amplifying a short segment of the signal pulse in a nonlinear crystal. High optical parametric gain makes possible the complete measurement of ultraweak, ultrashort light pulses. Unlike interferometric methods, it does not carry prohibitively restrictive requirements, such as perfect mode-matching, perfect spatial coherence, highly stable absolute phase, and a same-spectrum reference pulse. We simulate the OPA-XFROG technique and show that by a proper choice of the nonlinear crystal and the noncollinear mixing geometry it is possible to match the group velocities of the pump, signal, and idler pulses, which permits the use of relatively thick crystals to achieve high gain without measurement distortion. Gain bandwidths of ~100 nm are possible, limited by group velocity dispersion. In the second part of the thesis, we numerically simulate the performance of the ultrasimple ultrashort laser pulse measurement device- GRENOUILLE. While simple in practice, GRENOUILLE has many theoretical subtleties because it involves the second-harmonic generation of relatively tightly focused and broadband pulses. In addition, these processes occur in a thick crystal, in which the phase-matching bandwidth is deliberately made narrow compared to the pulse bandwidth. We developed a model that include all sum-frequency-generation processes, both collinear and noncollinear. We also include dispersion using the Sellmeier equation for the crystal BBO. Working in the frequency domain, we compute the GRENOUILLE trace for practical-and impractical-examples and show that accurate measurements are easily obtained for properly designed devices. For pulses far outside a GRENOUILLE's operating range (on the long side), we numerically deconvolve the GRENOUILLE trace with the response function of GRENOUILLE to improve its spectral resolution. In the last part of the thesis, we simulate the second harmonic generation with tightly focused beams by use of lens. Thus, we are able to explain the `weird' focusing effect that has been a `puzzles' for us in the GRENOUILLE measurement.

The ability to perceive the dynamics of nature is ultimately limited by the temporal resolution of the instruments available. With the help of the ultrashort optical pulse, people now are able to observe and steer the electronic dynamics on the atomic scale. Meanwhile, high power attainable in such short time scale helps to boost the study of nonlinear physics. Most commercial femtosecond lasers are based on Ti:sapphire, but such systems can only be tuned in a spectral range around 800 nm. Few applications need only a single wavelength in this spectral region and pulses tunable from the UV to the IR are highly desirable. Based on the soliton characteristics of ultrashort laser pulses, we are the first ones who propose to make use of resonant dispersive waves, which are phase-matched non-solitonic linear waves, to extend the spectral tuning range of ultrashort laser without involving complicated amplifiers. Experimentally, we achieve the tuning of dispersive wave wavelengths by changing the dispersion parameters of the laser cavity, and confirm dispersive waves are ultrashort pulses under appropriate conditions. We successfully apply such a system into a multi-wavelength operation Ti:sapphire laser. The proposed idea is general, and can be applied to systems where solitons dominate, for example fiber lasers. Thanks to the newly developed novel fiber -photonic crystal fiber- we obtain widely tunable and gap-free femtosecond pulse by extending this mechanism to waveguides. This is the largest reported tuning range for efficient nonlinear optical frequency conversion obtained with such a simple and low energy laser. We apply such a Ti:sapphire laser to Raman micro-spectroscopy. Because of the different temporal behaviors of the Raman process and other parametric processes, we can efficiently separate the coherent Raman signal from the unwanted background, and obtain a high chemical contrast and high resolution image. This high repetition rate and low energy laser oscillator makes it very suitable for biological Raman micro-spectroscopy, especially living samples for which damage is a big concern.

The object of the present research is to design and fabricate metal-dielectric thin film multilayer structures that make use of the nonlinear optical (NLO) response of Ag for efficient nonlinear absorption for sensor protection. These structures employ structural resonances to overcome the challenges of reflection and absorption that limit access to this large NLO response. The research consists of three parts: first, we present a comprehensive analysis of the contributions to the nonlinear optical response of Ag. Second, we present a systematic investigation of the linear optical properties of Metal-Dielectric Photonic Band-Gap (MDPBG) structures, including optimization of the structure for a particular transmittance spectrum. Third, we study the linear and nonlinear optical properties of Induced Transmission Filters (ITFs). Each of these parts includes experimental results backed by modeling and simulation.

Includes bibliographical references (p. 74-79).

Several significant wave propagation problems in the fields of nonlinear optics and hydrodynamics are studied in this thesis. In optics, the physical model considered is the two-core optical fiber (TCF), which is an essential component of lightwave technology. In hydrodynamics, the motion of a wave packet on the free surface of water of finite depth allowing modulations from two mutually perpendicular and horizontal directions, governed by the famous Davey-Stewartson (DS) equations, is taken into account. The main contributions of this thesis are: In optics, the effects of the intermodal dispersion (IMD) and the birefringence induced effects, both of which always exist in the TCFs, have been ignored in the previous studies of the modulation instability (MI) of continuous waves (CWs) in the TCFs. In this thesis, a detailed analysis of these effects on the MI spectra has been done. It is found that IMD does not seriously affect the MI spectra of the symmetric/antisymmetric CW states, but can significantly modify the MI spectra of the asymmetric CW states. In exploring the birefringence induced effects, a particular class of asymmetric CW states, which admits analytical solutions and has no counterpart in the single-core fibers, is focused on. It is found that the MI spectra of a birefringent TCF in the normal dispersion regime can be distinctively different from those of a zero-birefringence TCF especially for the circular-birefringence TCF. All the findings of MI analysis can be well verified by the wave propagation dynamics. Another contribution of this thesis is that we find the dramatic pulse distortion and even pulse splitting phenomenon due to IMD in TCFs, which is unexpected in many situations, can be effectively suppressed and even avoided by Kerr nonlinearity, which has never been reported in the literatures in the studies of TCFs. In hydrodynamics, DS equations describe the evolution of weakly nonlinear, weakly dispersive wavepackets with slow spanwise dependences on a fluid of finite depth. Generally, DS equations are divided into two types e, i.e. DSI and DSII equations, depending on the specific fluid configurations (fluid depth, wavelength of the water wave, surface tension etc). Due to the importance of DS equations, many exact solutions have been derived by different nonlinear wave methods over the years in the literature. In this thesis, two new exact doubly periodic wave patterns of DS equations are derived by the use of properties of the theta functions, or equivalently, the Jacobi elliptic functions, and the corresponding solitary waves are also deduced in the long wave limits. The new feature of the two wave patterns found is that they can be applied to both DSI and DSII systems at the same time. / published_or_final_version / Mechanical Engineering / Doctoral / Doctor of Philosophy

This thesis reports on ultrafast linear and nonlinear optical probing of nanometer thick films. Exfoliated graphene and few-layer graphite are probed through optical second harmonic generation (SHG) with 800 nm, 150 fs pulses. Samples of varying thickness from 1 carbon layer to bulk graphite are deposited onto an oxidized silicon substrate. SHG measurements are taken as a function of azimuthal rotation angle of the films. It is found that the SHG from graphene is much weaker than that from bilayer graphene, and has a qualitatively different azimuthal pattern. As the sample thickness increases from bilayer graphene to bulk graphite, the SHG yield generally decreases. Both of these effects are explained in terms of the symmetry of graphene and graphite, and modeled using multilayer optical transfer matrices, and an identical set of nonlinear susceptibility tensor elements for the front and back surfaces. These tensors are independent of sample thickness. MnAs films of 150 and 190 nm thickness on (001)GaAs are optically excited with 775 nm, 200 fs pump pulses. Specular SHG at 388 nm and first order optical diffraction at ∼ 400 nm are used to probe the samples on timescales up to 2 μs. It is found that the SHG probes the temperature-dependent, spatially averaged, surface strain. This strain reaches a maximum deviation in ∼ 6–100 ps after optical excitation depending on the pump fluence and initial temperature. The strain then recovers in hundreds of picoseconds, a timescale consistent with heat diffusion. The optical diffraction probes the first Fourier component of the paramagnetic–ferromagnetic stripes inherent to MnAs films in the 10–40◦C temperature range. After optical excitation, the diffraction data show highly nonthermal behaviour in the MnAs films. If a sample is excited from the coexistence phase, the diffraction signal shows decaying oscillations with a period of ∼ 335±4 (408±4) ps for the 150 (190) nm films; this is consistent with the release of a standing acoustic wave. Decay occurs on a timescale of ∼ 2 ns consistent with local diffusion through the films. The stripes are restored on a timescale of hundreds of nanoseconds, with a temporal behavior consistent with a diffusion process, possibly thermal in origin.