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  • About
  • The Global ETD Search service is a free service for researchers to find electronic theses and dissertations. This service is provided by the Networked Digital Library of Theses and Dissertations.
    Our metadata is collected from universities around the world. If you manage a university/consortium/country archive and want to be added, details can be found on the NDLTD website.
1

Fission fragment gamma-ray multiplicities

Hook, D. E. January 1987 (has links)
No description available.
2

Characterization of a Stochastic Procedure for the Generation and Transport of Fission Fragments within Nuclear Fuels

Hackemack, Michael Wayne 03 October 2013 (has links)
With the ever-increasing demands of the nuclear power community to extend fuel cycles and overall core-lifetimes in a safe and economic manner, it is becoming more necessary to extend the working knowledge of nuclear fuel performance. From the atomistic to the macroscopic level, great morphological changes occur within the fuel over its lifetime. The main initial damaging events produced by fuel recoils from fast neutrons and fission fragment spiking leads to the onset of grain growths and fuel restructuring. Therefore, it is desirable to have a more detailed understanding of the initial events leading to fuel morphology changes at the atomistic level. However, this is difficult to achieve with the fission fragments due to the wide variability of their species (charge, mass, and energy) and the large averaging of their relative yields in the nuclear data files. This work is our first iteration at developing a general methodology to characterize a procedure, based on Monte Carlo principles, for generating individual fission event result channels and analyzing their specific response in the fuel. We utilized the nuclear reaction simulation tool, TALYS, to generate energy-dependent fission fragment yield distributions for different fissile/fissionable isotopes. These distributions can then be used in conjunction with fuel isotopics and a neutron energy spectrum to generate a fission-reaction-rate-averaged distribution of the fission fragment yields. We then used Monte Carlo sampling to generate the result channels from individual fission events, using the Q-value of the prompt fission system to either accept or reject. The simulation tool: Transport of Ions in Matter (TRIM) was used to characterize the general response of the fission fragment species within Uranium Dioxide (UO2), including the range, energy loss, displacements, recoils, etc. These responses were then correlated which allowed for the quick calculation of the response of the individual fission fragment species generated from the Monte Carlo sampling. As an example of this strategy, we calculated the response on a PWR fuel pin where MCNP was used to generate a high-fidelity neutron energy spectrum.
3

Analysis of a direct energy conversion system using medium energy helium ions

Carter, Jesse James 16 August 2006 (has links)
A scaled direct energy conversion device was built to convert kinetic energy of singly ionized helium ions into an electric potential by the process of direct conversion. The experiments in this paper aimed to achieve higher potentials and higher efficiencies than ever before. The predicted maximum potential that could be produced by the 150 kV accelerator at the Texas A&M Ion Beam Lab was 150 kV, which was achieved with 92% collection efficiency. Also, an investigation into factors affecting collection efficiency was made. It was concluded that charge was being lost due to charge exchange occurring near the surface of the target which caused positive target atoms to be ejected from the face and accelerated away. Introducing a wire mesh near the face of the target with an electric potential, positive or negative, which aimed to control secondary ion emissions, did not have an effect on the collection efficiency of the system. Also, it was found that the gas pressure inside the chamber did not have an effect on the collection efficiency. The goal of achieving higher electric potentials and higher efficiencies than previous direct conversion work was met.
4

Study of fission of exotic actinides by relativistic reactions / Étude de la fission d'actinides exotiques par réaction relativiste

Yan, Yiman 28 September 2016 (has links)
SOFIA (Studies On FIssion with Aladin) est un programme expérimental innovant qui a pour objectif la mesure de plusieurs observables de la fission nucléaire : les taux de production isotopiques des fragments de fission, l'énergie cinétique totale des fragments, et la multiplicité des neutrons prompts. Ces informations sont obtenues pour une large variété d'actinides et de pré-actinides. Le recours à la cinématique inverse (le système fissionnant est le faisceau et non pas la cible) est le seul moyen d'identifier les fragments à la fois en charge et en masse. Le travail de doctorat présenté dans cette thèse porte sur l'expérience menée en Octobre 2014 et dédiée à la mesure de la fission de ² ³ ⁶ U induite par excitation coulombienne, soit l'analogue de la fission de ² ³⁵U induite par neutron.Les expériences SOFIA ont lieu à GSI (Darmstadt, Allemagne), la seule installation au monde capable de délivrer un faisceau d'uranium ² ³⁸ de 1 GeV par nucléon. Ce faisceau primaire subit une première fragmentation, dont les produits sont sélectionnés par le FRS (FRagment Separator) afin de former un faisceau secondaire du noyau d'intérêt, en l'occurrence ² ³ ⁶ U, qui est guidé vers l'expérience SOFIA où sa fission est déclenchée.Certains noyaux proches de ² ³ ⁶ U sont également transmis par le FRS : il est donc nécessaire de procéder à l'identification en masse et en charge du système fissionnant, puis d'identifier les deux fragments de fission. Dans les deux cas, l'identification, réalisée événement par événement, repose sur la mesure simultanée de la perte d'énergie dans un gaz, de la rigidité magnétique et du temps de vol. Seules les fissions induites par excitation coulombiennes sont pertinentes : la contribution des réactions nucléaires à la production des fragments doit donc être mesurée et soustraite.L'analyse présentée dans ce document inclut l'identification du faisceau secondaire en masse et en charge, l'identification en charge des fragments de fission, l'estimation de la contribution des réactions nucléaires, et finalement les taux de production des éléments obtenus dans la fission de ² ³ ⁶ U. Ces résultats sont comparés à ceux d'autres mesures réalisées sur SOFIA, et à des résultats antérieurs obtenus par d'autres techniques. / SOFIA (Studies On FIssion with Aladin) is an innovative experimental program which aims to measure several fission observables — the isotopic fission yields, the total kinetic energy of the fragments and the prompt neutron multiplicity, for a wide range of actinides and pre-actinides. The use of inverse kinematics (the fissioning system is the beam instead of the target) is the only way to fully identify fragments in charge and mass. The PhD work presented in this thesis concerns the experiment conducted in October 2014, and is focused on the Coulomb-induced fission of ² ³ ⁶ U, which can be regarded as the analog of the neutron-induced fission of ² ³⁵U.The SOFIA experiments take place in GSI (Darmstadt, Germany) because it is the sole facility in the world which delivers a beam of ² ³⁸U at 1 AGeV. This beam is fragmented and the products are selected by the FRS (FRagment separator) in order to deliver a secondary beam of nuclei of interest - ² ³ ⁶ U in our case, which is then guided to the SOFIA setup where its fission is triggered.Since some nuclides with close atomic and mass numbers to ² ³ ⁶ U are also transmitted by the FRS, it is necessary to identify the fissioning system from the secondary beam first, and then identify both the associated fission fragments. All identifications are performed event by event on the basis of measurements of the energy loss, the magnetic rigidity and the time of flight. Since we are only interested in the Coulomb-induced fission of ² ³ ⁶ U, the contribution of fragmentation fissions on the nuclear charge distribution of fission fragments has to be suppressed.The analysis in this paper involves the isotopic identification of the fissioning system, the nuclear charge identification of the fission fragments, the estimation of the nuclear contribution, and the extraction of the elemental fission yield. The results are then compared to other measurements performed with the SOFIA setup, as well as previous results obtained by other techniques.
5

Experimental studies at CERN-nTOF of the 230Th(n,f) reaction

Lapinski, Felicia January 2020 (has links)
This work investigates the feasibility to perform an experiment at CERN n_TOF to study the fission cross section and fission fragment angular distribution (FFAD) of the 230Th(n,f) reaction. An analysis of fission fragment energy losses in the experimental target resulted in a choice of target thickness of 0.1 µm (100 µg/cm2 ), which yields good transmission out of the target at up to 45° emission angles from the target normal. A detection setup using ten PPAC detectors with nine thorium targets interleaved in between them was investigated, where the detectors and targets were tilted 45° with respect to the neutron beam. This makes it possible to measure all emission angles needed with respect to the neutron beam in order to determine the FFAD. For the experimental area EAR2 at n_TOF, a prediction of the count rate in the experiment resulted in low statistical uncertainties after a few weeks of beam time, which indicates that an experiment like this is feasible. / Detta projekt undersöker genomförbarheten av ett experiment vid CERN n_TOF för att mäta tvärsnittet och fördelningen av emissionsvinklar av fissionsfragment (FFAD) från 230Th(n,f)-reaktionen. En analys av energiförlusterna av fissionsfragment inuti torium-provet resulterade i en optimal provtjocklek på 0.1 µm (100 µg/cm2 ), vilket medför att fissionsfragment som emitteras i vinklar upp till 45° från provets normal har hög sannolikhet att transmitteras ut ur provet. En detektionsuppställning med tio PPAC-detektorer med nio toriumprov mellan dem undersöktes, där detektorerna och proven antogs vara snedställda med 45° från neutronstrålens riktning. Detta möjliggör detektion av fissionsfragment i alla vinklar som är nödvändiga för att kunna mäta hela FFAD. För experimentanläggningen EAR2 vid n_TOF, resulterade en uppskattning av antalet detekterade fissionsevent per sekund i låga mätosäkerheter efter ett par veckor av mättid, vilket antyder att experimentet är görbart.
6

Determination of binary fission-fragment yields in the reaction 251Cf(nth, f) and Verification of nuclear reaction theory predictions of fission-fragment distributions in the reaction 238U(n, f)

Birgersson, Evert January 2007 (has links)
Neutron-induced fission has been studied at different excitation energies of the compound nucleus by measurements on the two fissioning systems, 252Cf* and 239U*. For the first time, the light fission fragment yields from the reaction 251Cf(nth, f) have been measured with high resolution. This experiment was performed with the recoil mass spectrometer LOHENGRIN at ILL in Grenoble, France. When the results from this work, where the compound nucleus is at thermal excitation, are compared to the spontaneous fission of 252Cf, enhanced emission yields as well as an increased mean kinetic energy is observed around A = 115. This suggests the existence of an additional super-deformed fission mode in 252Cf. The reaction 238U(n, f) was studied using the 2E-technique with a double Frisch grid ionization chamber. Fission fragment mass, energy and angular distributions were determined for incident neutron energies between 0.9 and 2.0 MeV. The experiments were performed at the Van de Graaff accelerator of IRMM in Geel, Belgium. This is the first measurement of the mass distribution for incident neutron energies around 0.9 MeV. The motivation for studying 238U(n, f) was to verify theoretical predictions of the mass distribution at the vibrational resonance in the fission cross section at 0.9 MeV. However, the predicted changes in fission fragment distributions could not be confirmed. A precise modelling of the fission process for the minor actinides becomes very important for future generation IV and accelerator driven nuclear reactors. Since fission fragment distributions depend on the excitation of the fissioning system, so does the number of delayed neutrons, which are one of the safety parameters in a reactor.
7

Fission fragment angular distribution and fission cross section validation

Leong, Lou Sai 27 September 2013 (has links) (PDF)
The present knowledge of angular distributions of neutron-induced fission is limited to a maximal energy of 15 MeV, with large discrepancies around 14 MeV. Only 238U and 232Th have been investigated up to 100 MeV in a single experiment. The n_TOF Collaboration performed the fission cross section measurement of several actinides (232Th, 235U, 238U, 234U, 237Np) at the n_TOF facility using an experimental set-up made of Parallel Plate Avalanche Counters (PPAC), extending the energy domain of the incident neutron above hundreds of MeV. The method based on the detection of the 2 fragments in coincidence allowed to clearly disentangle the fission reactions among other types of reactions occurring in the spallation domain. I will show the methods we used to reconstruct the full angular resolution by the tracking of fission fragments. Below 10 MeV our results are consistent with existing data. For example in the case of 232Th, below 10 MeV the results show clearly the variation occurring at the first (1 MeV) and second (7 MeV) chance fission, corresponding to transition states of given J and K (total spin and its projection on the fission axis), and a much more accurate energy dependence at the 3rd chance threshold (14 MeV) has been obtained. In the spallation domain, above 30 MeV we confirm the high anisotropy revealed in 232Th by the single existing data set. I'll discuss the implications of this finding, related to the low anisotropy exhibited in proton-induced fission. I also explore the critical experiments which is valuable checks of nuclear data. The 237Np neutron-induced fission cross section has recently been measured in a large energy range (from eV to GeV) at the n TOF facility at CERN. When compared to previous measurements, the n TOF fission cross section appears to be higher by 5-7 % beyond the fission threshold. To check the relevance of n TOF data, we simulate a criticality experiment performed at Los Alamos with a 6 kg sphere of 237Np. This sphere was surrounded by enriched uranium 235U so as to approach criticality with fast neutrons. The simulation predicts a multiplication factor keff in better agreement with the experiment (the deviation of 750 pcm is reduced to 250 pcm) when we replace the ENDF/B- VII.0 evaluation of the 237Np fission cross section by the n TOF data. We also explore the hypothesis of deficiencies of the inelastic cross section in 235U which has been invoked by some authors to explain the deviation of 750 pcm. The large distortion that should be applied to the inelastic cross sections in order to reconcile the critical experiment with its simulation is incompatible with existing measurements. Also we show that the nubar of 237Np can hardly be incriminated because of the high accuracy of the existing data. Fission rate ratios or averaged fission cross sections measured in several fast neutron fields seem to give contradictory results on the validation of the 237Np cross section but at least one of the benchmark experiments, where the active deposits have been well calibrated for the number of atoms, favors the n TOF data set. These outcomes support the hypothesis of a higher fission cross section of 237Np.
8

Etude de la fission nucléaire par spectrométrie des rayons gamma prompts / Study of nuclear fission by spectrometry of the prompt gamma rays

Rąpała, Michał 15 October 2018 (has links)
La volonté d'améliorer l'efficacité énergétique des réacteurs nucléaires a motivé de nouvelles solutions dans leur conception. L'une d'elles est l’utilisation d’un réflecteur lourd dans les réacteurs de génération III+ et les futurs réacteurs de génération IV. Lorsque la matière est traversée par des rayons γ, les excitations induites entraînent une élévation de sa température. Ce processus, appelé échauffement γ, est responsable de plus de 90% de la production de chaleur dans la région hors combustible d'un réacteur nucléaire. C’est également le cas dans le réflecteur. Pour simuler l'effet de l’échauffement γ en fonction de la composition du combustible, il faut disposer de données précises sur les γ prompts émis par les différents fragments produits dans le processus de fission. En 2012, une campagne d’expériences inédite, EXILL, a été menée au réacteur de recherche de l'ILL. Un grand nombre de détecteurs HPGe a été placé autour d’une cible fissile et a mesuré les rayons γ émis par la cible alors qu’elle était irradiée par un faisceau intense de neutrons froids. Dans ce travail, nous avons analysé les données obtenues avec des cibles ²³⁵U. Elles nous ont permis d’étudier la désexcitation de plusieurs fragments de fission et plus globalement le processus de fission induite par des neutrons. Dans un premier temps, nous avons utilisé la méthode standard d'analyse par coïncidence γ-γ-γ. Nous avons pu filtrer les données expérimentales, identifier les transitions γ dans des fragments bien produits et calculer leur intensité relative. Les problèmes que nous avons rencontrés concernent le bruit de fond. Les résultats obtenus dépendent de ce choix et présentent donc des problèmes de reproductibilité. Nous avons développé et testé une nouvelle méthodologie d'analyse. Son principe est un balayage des portes de coïncidence selon trois directions, ce qui permet de trouver le bruit de fond le mieux adapté. L'idée principale était finalement de passer d'une méthode "spectroscopique", dont le but est de trouver de nouvelles transitions et des états excités dans un noyau, à une méthode "spectrométrique", qui nous permet d'obtenir plus précisément l’intensité de transitions γ connues, avec une meilleure estimation de leur incertitude. Cela nous a amené à développer un logiciel d'analyse semi-automatique d'ajustement des pics. Divers schémas de calcul de l'intensité des transitions γ ont été également élaborés pour tenir compte des contaminations possibles, selon leur emplacement dans la matrice de coïncidence et leur intensité. La méthode standard et la nouvelle méthode d'analyse ont été comparées pour l'analyse du ¹⁴²Ba. Dans ce travail, nous avons également comparé nos résultats sur quelques noyaux, tel que le ¹⁰⁰Zr, avec des simulations réalisées avec le code FIFRELIN. Ce dernier est un code Monte-Carlo qui simule le processus de fission et la désexcitation des fragments de fission. FIFRELIN utilise plusieurs modèles différents pour décrire ces processus. Nous avons testé le comportement des différents modèles, trouvé les valeurs optimales des paramètres de simulation et testé comment ces configurations reproduisaient les résultats expérimentaux. FIFRELIN n'a pas été en mesure de reproduire simultanément les intensités des transitions γ émises par les fragments de ¹⁰⁰Zr et la multiplicité de neutrons prompts moyennée sur tous les fragments de fission. Cependant, avec des paramètres modifiés, FIFRELIN a fourni localement une multiplicité de neutrons prompts correcte pour les fragments de masse atomique A=100 et des intensités de transition γ bien reproduites pour le noyau de ¹⁰⁰Zr. Nous avons également comparé nos résultats expérimentaux sur les fragments de ¹⁰⁰Zr provenant du processus ²³⁵U(n,f) avec les autres données expérimentales disponibles provenant des expériences sur ²⁴⁸Cm(sf) et ²⁵²Cf(sf), et une autre expérience sur ²³⁵U(n,f). / The desire to improve the fuel efficiency of nuclear reactors has motivated new solutions in their design. One of them is the heavy reflector used in the generation III+ and in the future generation IV reactors. γ-rays passing through matter cause its excitation and temperature rise. It is a process called γ-heating, and it is responsible for more than 90% of the heat production in the non-fuel region of the nuclear reactor. This is also the case of the heavy reflector. To simulate the γ-heating effect in every state of the nuclear reactor it is necessary to have precise data on the prompt γ-rays emitted by different fission fragments produced in the course of the nuclear chain reaction. In 2012, at the research reactor of the ILL, an innovative experiment, called EXILL, was conducted. It produced a large amount of useful data on the de-excitation of the fission fragments. A large number of HPGe detectors were used to study the neutron induced fission process by measuring the emitted γ-rays. Fissile targets were irradiated by an intense cold neutron beam. In this work we analyzed the ²³⁵U targets. We studied several fission fragments and more generally the fission process by using high-resolution γ-ray spectroscopy. At the beginning, we used the standard γ-γ-γ coincidence analysis method. We were able to filter experimental data, identify the well produced γ-rays, and calculate their relative intensities. The problems we have encountered are related to the background. The results obtained with this method were background dependent and thus presented some problems with reproducibility. We therefore developed and tested a new analysis methodology. Its crucial feature is a coincidence gates scanning in three directions which helps to find the most suitable background. The idea was to move from a “spectroscopic” method, which main purpose is finding new transitions and excited states in a nucleus, to a “spectrometric” method, which allows us to obtain more precise γ-ray intensities. We developed a semi-automatic analysis software which facilitates fitting of the chosen γ-ray peak, the contamination and the background. Various γ-ray intensity calculation schemes were derived to take into account different contamination strengths and placements. The results of the analysis with the new technique are reproducible and more reliable. The standard and the new analysis method were compared in the ¹⁴²Ba analysis. In this work, we also compared our experimental results on some nuclei, such as ¹⁰⁰Zr, with the simulation results performed with the FIFRELIN code. It is a Monte-Carlo code which simulates the fission process and the de-excitation of the fission fragments. It uses various models to describe these processes. We were able to test the behavior of different models implemented in FIFRELIN to find the optimal simulation parameter values and to test how well these setups reproduce the experimental results. FIFRELIN was unable to simultaneously reproduce the γ-ray intensities of ¹⁰⁰Zr and the prompt-neutron multiplicity averaged over all fission fragments. However, with modified simulation parameters, FIFRELIN locally provided correct prompt-neutron multiplicity for the fission fragment with the atomic mass A=100 and well reproduced γ-ray intensities of ¹⁰⁰Zr. We also compared our experimental results on ¹⁰⁰Zr coming from the ²³⁵U(n,f) process with the other available experimental data coming from the experiments on ²⁴⁸Cm(sf) and ²⁵²Cf(sf), and another experiment on ²³⁵U(n,f).
9

Fission fragment angular distribution and fission cross section validation / Distributions angulaires de fragments de fission et validation de sections efficaces de fission

Leong, Lou Sai 27 September 2013 (has links)
La connaissance actuelle de la distribution angulaire de la fission induite par neutrons est limitée à une énergie maximum de 15~MeV, avec de grands écarts autour de 14~MeV. Seulement 238U et 232Th ont été étudiés jusqu'à 100 MeV et un seul jeu de données existe. Nous avons réalisé une expérience à n_TOF au CERN pour mesurer les distributions angulaires de fragments de fission jusqu'à 1~GeV pour les isotopes 232Th, 235U , 238U , 237Np.L'expérience a été réalisée à l'aide d'un dispositif expérimental à base de compteurs à avalanche à plaques parallèles (PPAC). La méthode basée sur la détection des 2 fragments en coïncidence permet d'identifier sans ambiguïté la fission des autres réactions, notamment dans le domaine de spallation. Au-dessous de 10 MeV nos résultats sont cohérents avec les données existantes. Par exemple, dans le cas de 232Th , en dessous de 10 MeV ils montrent clairement la variation d'anisotropie se produisant dans les résonances vibrationnelles (1.6 MeV) correspondant à des états de transition de J et K donnés (spin total et sa projection sur l'axe de fission), et après l'ouverture de la deuxième chance de fission (7 MeV). Ils apportent une meilleure précision autour de la troisième chance de fission (14 MeV). Aux énergies intermédiaires, au-dessus de 20 MeV nous avons constaté une anisotropie significative mais bien inférieure à l'unique résultat antérieur. Notre résultat est en accord avec la systématique en fissilité du système composite et avec un modèle incluant les phénomènes essentiels, en particulier le preéquilibre. Dans le cadre de cette comparaison l'anisotropie plus grande que pour la fission induite par protons s'explique parfaitement. J'ai par ailleurs exploré et simulé les expériences de criticité qui permettent de tester la précision des données nucléaires. La section efficace de fission de 237Np induite par neutrons avait été mesurée sur l'installation n_TOF au CERN. Par rapport aux résultats antérieurs la section efficace de fission n_TOF était apparue plus élevée de 6-7% au-delà du seuil de fission. Pour vérifier la pertinence des données de n_TOF, nous avons simulé une expérience de criticité effectuée à Los Alamos avec une sphère contenant 6 kg de 237Np. Cette sphère est entourée par de l'uranium hautement enrichi en 235U de façon à approcher la criticité avec des neutrons rapides. La simulation prédit un facteur de multiplication keff en meilleur accord avec l'expérience (l'écart de -0.75% est réduit à +0.25%) quand on remplace la section efficace de fission de 237Np des bibliothèques évaluées par celle de n_TOF. Nous avons également exploré d'autres effets pouvant expliquer l'écart qui existait entre la mesure de criticité et sa prédiction par les simulations, en particulier nous avons testé la section inélastique de 235U et la multiplicité de neutrons de fission de 237Np. Dans les 2 cas la modification requise pour réconcilier l'écart de criticité n'est pas en accord avec les mesures. Des mesures de taux de fission dans des flux de neutrons dont le spectre est connu indiquent également que la section de fission du 237Np pourrait être plus grande de 4 à 5% par rapport à ce qui était admis aujourd'hui. / The present knowledge of angular distributions of neutron-induced fission is limited to a maximal energy of 15 MeV, with large discrepancies around 14 MeV. Only 238U and 232Th have been investigated up to 100 MeV in a single experiment. The n_TOF Collaboration performed the fission cross section measurement of several actinides (232Th, 235U, 238U, 234U, 237Np) at the n_TOF facility using an experimental set-up made of Parallel Plate Avalanche Counters (PPAC), extending the energy domain of the incident neutron above hundreds of MeV. The method based on the detection of the 2 fragments in coincidence allowed to clearly disentangle the fission reactions among other types of reactions occurring in the spallation domain. I will show the methods we used to reconstruct the full angular resolution by the tracking of fission fragments. Below 10 MeV our results are consistent with existing data. For example in the case of 232Th, below 10 MeV the results show clearly the variation occurring at the first (1 MeV) and second (7 MeV) chance fission, corresponding to transition states of given J and K (total spin and its projection on the fission axis), and a much more accurate energy dependence at the 3rd chance threshold (14 MeV) has been obtained. In the spallation domain, above 30 MeV we confirm the high anisotropy revealed in 232Th by the single existing data set. I'll discuss the implications of this finding, related to the low anisotropy exhibited in proton-induced fission. I also explore the critical experiments which is valuable checks of nuclear data. The 237Np neutron-induced fission cross section has recently been measured in a large energy range (from eV to GeV) at the n TOF facility at CERN. When compared to previous measurements, the n TOF fission cross section appears to be higher by 5-7 % beyond the fission threshold. To check the relevance of n TOF data, we simulate a criticality experiment performed at Los Alamos with a 6 kg sphere of 237Np. This sphere was surrounded by enriched uranium 235U so as to approach criticality with fast neutrons. The simulation predicts a multiplication factor keff in better agreement with the experiment (the deviation of 750 pcm is reduced to 250 pcm) when we replace the ENDF/B- VII.0 evaluation of the 237Np fission cross section by the n TOF data. We also explore the hypothesis of deficiencies of the inelastic cross section in 235U which has been invoked by some authors to explain the deviation of 750 pcm. The large distortion that should be applied to the inelastic cross sections in order to reconcile the critical experiment with its simulation is incompatible with existing measurements. Also we show that the nubar of 237Np can hardly be incriminated because of the high accuracy of the existing data. Fission rate ratios or averaged fission cross sections measured in several fast neutron fields seem to give contradictory results on the validation of the 237Np cross section but at least one of the benchmark experiments, where the active deposits have been well calibrated for the number of atoms, favors the n TOF data set. These outcomes support the hypothesis of a higher fission cross section of 237Np.
10

Simulations And Experiments Of Plasma-Induced Effects In Silicon Detectors

Gomez L, Ana Maria January 2023 (has links)
When an atomic nucleus undergoes fission, two fragments with different mass and kinetic energy are emitted. The highly unstable fission fragments (FFs) evaporate prompt neutrons soon after the nucleus splits. A precise measurement of both, the mass yield distribution of the FFs and the average prompt neutron emission, $\bar{\nu}$, is important not only for current nuclear technologies but also for the development of future technologies such as Generation IV nuclear power plants. Moreover, the experimental determination of the mass yield distributions, both pre- and post-neutron emission, is valuable for testing fission models. Additionally, a precise measurement of the average neutron multiplicity as a function of the FFs mass, <img src="http://www.diva-portal.org/cgi-bin/mimetex.cgi?$%5Cbar%7B%5Cnu%7D(A)$" data-classname="equation" data-title="" />, is crucial in the understanding of how the excitation energy is shared between nascent FFs.  The VElocity foR DIrect particle identification spectrometer (VERDI) is designed to achieve pre- and post-fission mass distributions with resolutions between 1-2 u. VERDI is a double-energy double-velocity instrument that consists of two arms. On each arm is operated one Microchannel Plate detector (MCP) for the collection of the FFs start time and up to 32 Passive Implanted Planar Silicon (PIPS) detectors for the stop time and energy detection of the FFs. However, challenges in the experimental measurements with VERDI arise due to the high degree of ionization (plasma) in the detector material from the interaction with the FFs. The plasma causes a delay in the charge carriers' migration for the signal start, known as the plasma delay time effect (PDT). Furthermore, the recombination of charge carriers in the plasma causes a shrinking in the signal's height, known as pulse height defect (PHD). This phenomenon leads to inaccuracies in the measurement of FFs mass distributions and increased systematic uncertainties.  Previous studies on PDT and PHD have shown varying behaviors across different detector types, which motivated dedicated studies in the type of PIPS detectors used in VERDI. An experimental campaign to characterize the PDT and PHD in PIPS detectors was conducted in the LOHENGRIN recoil separator, which is part of the ILL nuclear facility in Grenoble, France. Measurements of FFs in a range of masses between 80 u and 149 u, with energies between 20 MeV to 110 MeV, were taken to fully characterize six PIPS detectors. The resulting PDT and PHD values were 1 ns to 4 ns and 2 MeV to 10 MeV respectively. The PDT and PHD exhibited consistent energy and mass dependencies across the detectors, which enables the possibility of an event-by-event correction of VERDI data. In this thesis, the basis for discussing the results of the studies of the PDT and PHD effects will be presented.

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