The neutron spectrometer TOFOR was installed at JET in 2005 for high-rate observation of neutrons from reactions between two deuterium (D) ions. Neutron spectrometry as a fusion plasma diagnostic technique is invoked to obtain information about the velocity states of fusion fuel ions. Based on neutron spectrometry data, conclusions can be drawn on the efficiency of plasma heating schemes as well as optimization of fuel ion confinement. The quality of TOFOR analysis is found to depend on how well the instrument response function is known; discriminator threshold levels, detector time alignment and electronics broadening are identified as crucial issues. About 19 percent of the neutrons observed with TOFOR have scattered off the JET vessel wall or other structures in the line-of-sight before reaching the instrument, as established through simulations and measurements. A method has been developed to take these neutrons into account in the analysis. TOFOR measurements of fast deuterium distributions are seen to agree with distributions deduced from NPA data, obtained based on an entirely different principle. This serves as validation of the modeling and analysis. Extraordinary statistics in the TOFOR measurements from JET pulses heated with 3rd harmonic RF heating on D beams allow for study of instabilities using neutron emission spectrometry. At ITER, similar studies should be possible on a more regular basis due to higher neutron rates. Observations of neutrons from Be+3He reactions in the TOFOR spectrum from D plasmas heated with fundamental RF tuned to minority 3He raise the question of beryllium neutrons at JET after installation of the ITER-like wall, and at ITER, with beryllium as the plasma facing component. This is especially important for the first few years of ITER operation, where the machine will not yet have been certified as a nuclear facility and should be run in zero-activation mode.

The present thesis describes two experiments performed in the storage ring CELSIUS at The Svedberg Laboratory in Uppsala. In the first experiment the importance of three - nucleon clustering in the six - nucelon system was investigated. The total cross section for the production of the ground state and the 3.56 MeV second excited state of 6Li in the 3He(3He,6Li)π+ reaction has been measured at two beam energies, 261.1 and 262.5 MeV, corresponding to center - of - mass energies 1.2 and 1.9 MeV above the production threshold for the 3.56 MeV state. For the ground state the result was 347 ± 84 ± 42 and 92 ± 84 ± 11 nb respectively. The result for the 3.56 MeV state, 104 ± 23 ± 12 and 56 ± 35 ± 7 nb respectively, is compared to the result of a previous study where the 3.56 MeV state was populated in the d(4He,6Li)π0 reaction. In the second experiment a clean sample of 5×105 eta mesons was prepared by means of the d(p,3He)η reaction. Eta production was tagged by the precise determination of the kinetic energy of the associated 3He ions. In the subsequent decay of eta mesons, channels with lepton - anti - lepton pairs were studied in the WASA detector. In a separate study properties of the WASA deuterium pellet target were investigated and in particular the effects on the beam of the beam - target interactions. In both sets of experiments the fused nuclear system was detected by means of a zero - degree spectrometer with a semiconductor detector telescope. Choosing the detectors to match the rather different requirements, precise information regarding the identity and the momentum of the detected ions could be obtained in both cases.

The Vlasov technique is used to model the electron cooling force. Limitations of the applicability of the method is obtained by considering the perturbations of the electron plasma. Analytical expressions of the electron cooling force, valid beyond the Coulomb logarithm approximation, are derived and compared to numerical calculations using adaptive Monte Carlo integration. The calculated longitudinal cooling force is verified with measurements in CELSIUS. Transverse damping rates of betatron oscillations for a nonlinear cooling force is explored. Experimental data of the transverse monochromatic instability is used to determine the rms angular spread due to solenoid field imperfections in CELSIUS. The result, θrms= 0.16 ± 0.02 mrad, is in agreement with the longitudinal cooling force measurements. This verifies the internal consistency of the model and shows that the transverse and longitudinal cooling force components have different velocity dependences. Simulations of electron cooling with applications to HESR show that the momentum reso- lution ∆p/p smaller than 10−5 is feasible, as needed for the charmonium spectroscopy in the experimental program of PANDA. By deflecting the electron beam angle to make use of the monochromatic instability, a reasonable overlap between the circulating antiproton beam and the internal target can be maintained. The simulations also indicate that the cooling time is considerably shorter than expected.

Radioactive waste has been accumulated at CERN as unavoidable consequence of the use of particle accelerators. The elimination of this waste towards the final repositories in France and Switzerland requires the determination of the radionuclide inventory. In order to calculate the residual induced radioactivity in the waste, it is necessary to determine the spectra of secondary particles which are responsible for the material activation. In complex irradiation environments like in an accelerator tunnel it is expected that the secondary particle spectra vary with the characteristics of the machine components in a given section of tunnel. In order to obtain the production rates of the radionuclides of interest the spectra of secondary particles are to be folded with the appropriate cross sections. Though technically feasible, it would be impractical to calculate the particle spectra in every area of any machine and for all possible beam loss mechanisms. Moreover, a fraction of the waste has unknown radiological history, which makes it impossible to associate an item of waste to a precise area of the machine. Therefore it is useful to try to calculate “representative spectra”, which shall apply to a relatively large part of the accelerator complex at CERN. This thesis is dedicated to the calculation of representative spectra in the arcs of the 450 GeV proton synchrotron, SPS, at CERN. The calculations have been performed using the Monte Carlo code FLUKA. Extensive simulations have been done to assess the dependence of proton, neutron and pion spectra on beam energy, size of the nearby machine component and position with respect to the beam-loss point. The results obtained suggest that it is possible to define one single set of representative spectra for all the arcs of the SPS accelerator, with a minor error associated with the use of these.

In a nuclear power plant, control rods play a central role to control the reactivity ofthe core. In an inspection campaign of three control rods (CR 99) operated in theKKL reactor in Leibstadt, Switzerland, during 6 respectively 7 consecutive cycles,defects were detected in the top part of the control rods due to swelling caused bydepletion of the neutron-absorbing 10B isotope (Boron-10). In order to correlatethese defects to control rod depletion, the 10B depletion has in this study beencalculated in detail for the absorber pins in the top node of the control rods.Today the core simulator PLOCA7 is used for predicting the behavior of the reactorcore, where the retrievable information from the standard control rod follow-up isthe average 10B depletion for clusters of 19 absorber holes i.e. one axial node.However, the local 10B depletion in an absorber pin may be significantly differentfrom the node average depletion that is re-ceived from POLCA7. To learn more, the 10B depletion has been simulated for each absorber hole in the uppermost node usingthe stochastic Monte Carlo 3D simulation code MCNP as well as an MCNP- based2D-depletion code (McScram). It was found that the 10B depletion is significantly higher for the uppermost absorberpins than the node average. Furthermore, the radial depletion in individual absorberpins was found to be much higher than expected. The results are consistent with theexperimental data on control rod defects.

<p>The application of pulse shape analysis (PSA) and γ-ray tracking techniques has attracted a great deal of interest in the recent years in fields ranging from nuclear structure studies to medical imaging. These new data analysis methods add position sensitivity as well as directional information for the detected γ-rays to the excellent energy resolution of germanium detectors. This thesis focuses on the application of PSA on planar segmented germanium detectors, divided into three separate studies. The pulse shape analysis technique known as the matrix method was chosen due to its ability to treat events with arbitrary number and combinations of interactions within a single detector. It has been applied in two experiments with the 25-fold segmented planar pixel detector -- imaging and polarization measurements -- as well as in a simulation of upcoming detectors for DESPEC at NuSTAR/FAIR.</p><p>In the first experiment, a point source of ¹³⁷Cs was imaged. Events where the 662 keV γ-rays scattered once and were then absorbed in a different segment were treated by the PSA algorithm in order to find the locations of these interactions. The Compton scattering formula was then used to determine the direction to the source. The experiment has provided a robust test of the performance of the PSA algorithm on multiple interaction events, in particular those with interactions in adjacent segments, as well as allowed to estimate the realistically attainable position resolution. In the second experiment, the response of the detector to polarized photons of 288 keV was studied. The polarization of photons can be measured through the observation of the angular distribution of Compton-scattered photons, Hence the ability to resolve the interaction locations had once again proven useful.</p><p>The third study is focused on the performance of the proposed planar germanium detectors for the DESPEC array. As these detectors have not yet been manufactured at the time of this writing, a set of data simulated in GEANT4 was used. The detector response was calculated for two of the possible segmentation patterns -- that with a single pixelated contact and one where both contacts are segmented into mutually orthogonal strips. In both cases, PSA was applied in order to reconstruct the interaction locations from this response. It was found that the double-sided strip detector can achieve an over-all better position resolution with a given number of readout channels. However, this comes at the expense of a small number of complex events where the reconstruction fails. These results have also been compared to the performance of the 25-fold pixelated detector.</p>

Since its discovery, the phenomenon of nuclear fission is the object of extensive theoretical and experimental studies. However, we are still far from a complete understanding of the fission process. Nuclear theory can satisfactorily explain the process of neutron-induced fission at thermal neutron energies, but it meets problems at high neutron energies. However, new applications are nowadays developed involving neutron-induced fission in this energy domain. An example of such an application is accelerator-driven systems (ADS) which are dedicated to transmutation of highly radioactive nuclear waste. Conceptual studies of ADS require new nuclear data on neutron-induced reactions within a wide incident energy range. Along with structural, spallation target and other materials, data on neutron-induced fission are especially required for two nuclides, 232Th and 238U. At present, however, there are no published neutron-induced fission yield data for either 232Th or 238U at energies above 20 MeV. In this thesis, I present measurements of fission fragment mass yields at neutron energies from 10 to 60 MeV for 232Th and 238U. The experiment was done at the Louvain-la-Neuve quasi-monoenergetic neutron beam facility. A multi-section Frisch-gridded ionization chamber was used as the fission fragment detector. The fission fragment mass yields were measured at peak neutron energies of 33, 45, and 60 MeV. In addition, data for the neutron-energy intervals 9-11, 16-18, and 24-26 MeV were also extracted from the low-energy tail. The measurement results show that the symmetric fission component increases with incident neutron energy for both uranium and thorium, but it is more enhanced for thorium. The uranium results were compared to the only existing set of experimental data for neutron energies above 20 MeV. Reasonable agreement was found. However, our data show a lower symmetric fission component. For thorium, the present data are the first above 20 MeV. Model calculations with the TALYS code have also been done. This code is based on the multi-modal random neck-rupture model extended for higher excitation energies. We included a phenomenological model into the code and achieved a good description of our experimental results. / Felaktigt tryckt som Digital Comprehensive Summaries of Uppsala Dissertations from the Faculty of Science and Technology 723

This report describes investigations of the NE213-detector and the possibility to utilize pulse shape analysis to separate neutrons and gammas in a mixed emission field. Neutron fluxes are often contaminated with gammas, to which the detectors are sensitive. Sorting out the unwanted gamma pulses from the interesting neutrons is therefore crucial in many situations, for instance in fusion reactor diagnostics, such as for neutron cameras. This can be done based on pulse shapes, which differ for gammas and neutrons interacting in the NE213-detector. By analyzing the pulse shapes from a digital transient recorder, neutrons can be distinguished from gammas. An experiment with a Cf-252 neutron source was set up and provided data. The separation algorithm was based on charge comparison and gave good results. Furthermore the results of the pulse shape analysis were verified by TOF-measurements. The lowest permissible energy for a reasonable separation was found to be around 0.5 MeV. Some conclusions on the limitations of the equipment were also made.

The study of high power fusion plasmas at the JET tokamak has been further enhanced through the development of instrumentation for neutron emission spectroscopy (NES) measurements. This has involved the upgrade of the magnetic proton recoil (MPR) spectrometer used for deuterium-tritium plasmas earlier so that the MPRu can now be also employed for deuterium (D) plasmas. A neutron time-of-flight (TOF) spectrometer designed for optimized rate (TOFOR) has been constructed and put into operation. The MPRu and TOFOR spectrometers were carried out as part of the JET enhanced performance program and represent the most advanced instrumentation for NES diagnosis of both D and DT tokamak plasmas setting a central platform for R&amp;D direct to the next step in fusion research to be carried out with ITER. The MPRu work presented in this thesis concerns the development of a new focal plane detector based on the phoswich scintillator technique. The main objective of this sub-project was to increase the signal-to-background ratio to permit measurement of the 2.5-MeV neutron emission from d+d--&gt;3He+n reactions and, hence, allow NES diagnosis of D plasmas. The objective was achieved as demonstrated in preliminary measurements at JET. The development of TOFOR from concept to construction is presented in the thesis including, in particular, the commissioning of the instrument at JET. The objective of the TOFOR project was to achieve the same high performance in the NES diagnosis of D plasmas as had earlier been demonstrated by the MPR for DT plasmas. TOFOR has been used in the first plasma physics experiments reported in this thesis. These demonstrate that the performance objectives have been achieved as tested, in particular, in the observation of auxiliary heating effects on velocity distribution of the deuterium population.

In this project, the homogeneity of the detection efficiency of two silicon detectors were examined using a radioactive alpha-source, 241Am, to study the surfaces of the detectors by exposing a small part of the detector at a time. By then observing the variations of the deposited alpha-energies at different positions on the detector, one can map the differences in the homogeneity of the surface. Many variations of different magnitudes were found; some variations can reasonably be represented by either variations in the dead layer or residue glue along the edges. Some variations seemed best explained by pieces of dust or dirt on the surface. The possibility of using heavy fission fragments from the decay of 252Cf to compare the effects was explored but shown to be non-feasible in the scope of this project. Finally, proposals for further work and improvements are discussed.